Carbon‐Based Metal‐Free ORR Electrocatalysts for Fuel Cells: Past, Present, and Future
Replacing precious platinum with earth‐abundant materials for the oxygen reduction reaction (ORR) in fuel cells has been the objective worldwide for several decades. In the last 10 years, the fastest‐growing branch in this area has been carbon‐based metal‐free ORR electrocatalysts. Great progress ha...
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| Veröffentlicht in: | Advanced materials (Weinheim) 2019-03, Vol.31 (13), p.e1804799-n/a |
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| creator | Yang, Lijun Shui, Jianglan Du, Lei Shao, Yuyan Liu, Jun Dai, Liming Hu, Zheng |
| description | Replacing precious platinum with earth‐abundant materials for the oxygen reduction reaction (ORR) in fuel cells has been the objective worldwide for several decades. In the last 10 years, the fastest‐growing branch in this area has been carbon‐based metal‐free ORR electrocatalysts. Great progress has been made in promoting the performance and understanding the underlying fundamentals. Here, a comprehensive review of this field is presented by emphasizing the emerging issues including the predictive design and controllable construction of porous structures and doping configurations, mechanistic understanding from the model catalysts, integrated experimental and theoretical studies, and performance evaluation in full cells. Centering on these topics, the most up‐to‐date results are presented, along with remarks and perspectives for the future development of carbon‐based metal‐free ORR electrocatalysts.
Replacing precious platinum with earth‐abundant materials in fuel cells for the oxygen reduction reaction (ORR) has been a worldwide objective for several decades. In the last 10 years, the fastest‐growing branch in this area has been carbon‐based metal‐free ORR electrocatalysts. The most up‐to‐date results of this field are presented, along with remarks and perspectives for the future development of carbon‐based metal‐free ORR electrocatalysts. |
| doi_str_mv | 10.1002/adma.201804799 |
| format | Article |
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Replacing precious platinum with earth‐abundant materials in fuel cells for the oxygen reduction reaction (ORR) has been a worldwide objective for several decades. In the last 10 years, the fastest‐growing branch in this area has been carbon‐based metal‐free ORR electrocatalysts. The most up‐to‐date results of this field are presented, along with remarks and perspectives for the future development of carbon‐based metal‐free ORR electrocatalysts.</description><identifier>ISSN: 0935-9648</identifier><identifier>EISSN: 1521-4095</identifier><identifier>DOI: 10.1002/adma.201804799</identifier><identifier>PMID: 30637835</identifier><language>eng</language><publisher>Germany: Wiley Subscription Services, Inc</publisher><subject>Carbon ; carbon‐based metal‐free electrocatalysts ; Electrocatalysts ; Fuel cells ; Materials science ; multidoping ; nitrogen doping ; oxygen reduction reaction ; Oxygen reduction reactions ; Performance evaluation ; Platinum ; Predictive control</subject><ispartof>Advanced materials (Weinheim), 2019-03, Vol.31 (13), p.e1804799-n/a</ispartof><rights>2019 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim</rights><rights>2019 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c5439-6989e270ba2e5d414ceb94875fd47278abd9796a440bf910f2365fb2beec24ed3</citedby><cites>FETCH-LOGICAL-c5439-6989e270ba2e5d414ceb94875fd47278abd9796a440bf910f2365fb2beec24ed3</cites><orcidid>0000-0002-4847-899X ; 000000024847899X</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://onlinelibrary.wiley.com/doi/pdf/10.1002%2Fadma.201804799$$EPDF$$P50$$Gwiley$$H</linktopdf><linktohtml>$$Uhttps://onlinelibrary.wiley.com/doi/full/10.1002%2Fadma.201804799$$EHTML$$P50$$Gwiley$$H</linktohtml><link.rule.ids>230,314,776,780,881,1411,27901,27902,45550,45551</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/30637835$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink><backlink>$$Uhttps://www.osti.gov/biblio/1490764$$D View this record in Osti.gov$$Hfree_for_read</backlink></links><search><creatorcontrib>Yang, Lijun</creatorcontrib><creatorcontrib>Shui, Jianglan</creatorcontrib><creatorcontrib>Du, Lei</creatorcontrib><creatorcontrib>Shao, Yuyan</creatorcontrib><creatorcontrib>Liu, Jun</creatorcontrib><creatorcontrib>Dai, Liming</creatorcontrib><creatorcontrib>Hu, Zheng</creatorcontrib><title>Carbon‐Based Metal‐Free ORR Electrocatalysts for Fuel Cells: Past, Present, and Future</title><title>Advanced materials (Weinheim)</title><addtitle>Adv Mater</addtitle><description>Replacing precious platinum with earth‐abundant materials for the oxygen reduction reaction (ORR) in fuel cells has been the objective worldwide for several decades. In the last 10 years, the fastest‐growing branch in this area has been carbon‐based metal‐free ORR electrocatalysts. Great progress has been made in promoting the performance and understanding the underlying fundamentals. Here, a comprehensive review of this field is presented by emphasizing the emerging issues including the predictive design and controllable construction of porous structures and doping configurations, mechanistic understanding from the model catalysts, integrated experimental and theoretical studies, and performance evaluation in full cells. Centering on these topics, the most up‐to‐date results are presented, along with remarks and perspectives for the future development of carbon‐based metal‐free ORR electrocatalysts.
Replacing precious platinum with earth‐abundant materials in fuel cells for the oxygen reduction reaction (ORR) has been a worldwide objective for several decades. In the last 10 years, the fastest‐growing branch in this area has been carbon‐based metal‐free ORR electrocatalysts. The most up‐to‐date results of this field are presented, along with remarks and perspectives for the future development of carbon‐based metal‐free ORR electrocatalysts.</description><subject>Carbon</subject><subject>carbon‐based metal‐free electrocatalysts</subject><subject>Electrocatalysts</subject><subject>Fuel cells</subject><subject>Materials science</subject><subject>multidoping</subject><subject>nitrogen doping</subject><subject>oxygen reduction reaction</subject><subject>Oxygen reduction reactions</subject><subject>Performance evaluation</subject><subject>Platinum</subject><subject>Predictive control</subject><issn>0935-9648</issn><issn>1521-4095</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2019</creationdate><recordtype>article</recordtype><recordid>eNqFkc9u1DAQxi1ERZfClSOK4MKhWcaO_2S4LUu3RWrVqoILF8txJiJVNi52IrQ3HoFn5ElwtaVIXDh5PPObb2b0MfaCw5IDiLeu3bqlAF6DNIiP2IIrwUsJqB6zBWClStSyPmRPU7oBANSgn7DDCnRl6kot2Je1i00Yf_34-d4laosLmtyQf5tIVFxeXxcnA_kpBu9yfpemVHQhFpuZhmJNw5DeFVcuTcfFVaREYw7c2ObyNEd6xg46NyR6fv8esc-bk0_rs_L88vTjenVeeiUrLDXWSMJA4wSpVnLpqUFZG9W10ghTu6ZFg9pJCU2HHDpRadU1oiHyQlJbHbFXe92Qpt4m30_kv_owjnlxyyWC0TJDb_bQbQzfZkqT3fbJ5wvcSGFOVnCDlTZ5UkZf_4PehDmO-YRModZKAKhMLfeUjyGlSJ29jf3WxZ3lYO-ssXfW2AdrcsPLe9m52VL7gP_xIgO4B773A-3-I2dXHy5Wf8V_A_Hxmis</recordid><startdate>201903</startdate><enddate>201903</enddate><creator>Yang, Lijun</creator><creator>Shui, Jianglan</creator><creator>Du, Lei</creator><creator>Shao, Yuyan</creator><creator>Liu, Jun</creator><creator>Dai, Liming</creator><creator>Hu, Zheng</creator><general>Wiley Subscription Services, Inc</general><general>Wiley Blackwell (John Wiley & Sons)</general><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7SR</scope><scope>8BQ</scope><scope>8FD</scope><scope>JG9</scope><scope>7X8</scope><scope>OTOTI</scope><orcidid>https://orcid.org/0000-0002-4847-899X</orcidid><orcidid>https://orcid.org/000000024847899X</orcidid></search><sort><creationdate>201903</creationdate><title>Carbon‐Based Metal‐Free ORR Electrocatalysts for Fuel Cells: Past, Present, and Future</title><author>Yang, Lijun ; Shui, Jianglan ; Du, Lei ; Shao, Yuyan ; Liu, Jun ; Dai, Liming ; Hu, Zheng</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c5439-6989e270ba2e5d414ceb94875fd47278abd9796a440bf910f2365fb2beec24ed3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2019</creationdate><topic>Carbon</topic><topic>carbon‐based metal‐free electrocatalysts</topic><topic>Electrocatalysts</topic><topic>Fuel cells</topic><topic>Materials science</topic><topic>multidoping</topic><topic>nitrogen doping</topic><topic>oxygen reduction reaction</topic><topic>Oxygen reduction reactions</topic><topic>Performance evaluation</topic><topic>Platinum</topic><topic>Predictive control</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Yang, Lijun</creatorcontrib><creatorcontrib>Shui, Jianglan</creatorcontrib><creatorcontrib>Du, Lei</creatorcontrib><creatorcontrib>Shao, Yuyan</creatorcontrib><creatorcontrib>Liu, Jun</creatorcontrib><creatorcontrib>Dai, Liming</creatorcontrib><creatorcontrib>Hu, Zheng</creatorcontrib><collection>PubMed</collection><collection>CrossRef</collection><collection>Engineered Materials Abstracts</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>Materials Research Database</collection><collection>MEDLINE - Academic</collection><collection>OSTI.GOV</collection><jtitle>Advanced materials (Weinheim)</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Yang, Lijun</au><au>Shui, Jianglan</au><au>Du, Lei</au><au>Shao, Yuyan</au><au>Liu, Jun</au><au>Dai, Liming</au><au>Hu, Zheng</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Carbon‐Based Metal‐Free ORR Electrocatalysts for Fuel Cells: Past, Present, and Future</atitle><jtitle>Advanced materials (Weinheim)</jtitle><addtitle>Adv Mater</addtitle><date>2019-03</date><risdate>2019</risdate><volume>31</volume><issue>13</issue><spage>e1804799</spage><epage>n/a</epage><pages>e1804799-n/a</pages><issn>0935-9648</issn><eissn>1521-4095</eissn><abstract>Replacing precious platinum with earth‐abundant materials for the oxygen reduction reaction (ORR) in fuel cells has been the objective worldwide for several decades. 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Replacing precious platinum with earth‐abundant materials in fuel cells for the oxygen reduction reaction (ORR) has been a worldwide objective for several decades. In the last 10 years, the fastest‐growing branch in this area has been carbon‐based metal‐free ORR electrocatalysts. The most up‐to‐date results of this field are presented, along with remarks and perspectives for the future development of carbon‐based metal‐free ORR electrocatalysts.</abstract><cop>Germany</cop><pub>Wiley Subscription Services, Inc</pub><pmid>30637835</pmid><doi>10.1002/adma.201804799</doi><tpages>20</tpages><orcidid>https://orcid.org/0000-0002-4847-899X</orcidid><orcidid>https://orcid.org/000000024847899X</orcidid><oa>free_for_read</oa></addata></record> |
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| subjects | Carbon carbon‐based metal‐free electrocatalysts Electrocatalysts Fuel cells Materials science multidoping nitrogen doping oxygen reduction reaction Oxygen reduction reactions Performance evaluation Platinum Predictive control |
| title | Carbon‐Based Metal‐Free ORR Electrocatalysts for Fuel Cells: Past, Present, and Future |
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