Transition-Metal Single Atoms in a Graphene Shell as Active Centers for Highly Efficient Artificial Photosynthesis

Utilizing solar energy to fix CO2 with water into chemical fuels and oxygen, a mimic process of photosynthesis in nature, is becoming increasingly important but still challenged by low selectivity and activity, especially in CO2 electrocatalytic reduction. Here, we report transition-metal atoms coor...

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Veröffentlicht in:	Chem 2017-12, Vol.3 (6), p.950-960
Hauptverfasser:	Jiang, Kun, Siahrostami, Samira, Akey, Austin J., Li, Yanbin, Lu, Zhiyi, Lattimer, Judith, Hu, Yongfeng, Stokes, Chris, Gangishetty, Mahesh, Chen, Guangxu, Zhou, Yawei, Hill, Winfield, Cai, Wen-Bin, Bell, David, Chan, Karen, Nørskov, Jens K., Cui, Yi, Wang, Haotian
Format:	Artikel
Sprache:	eng
Schlagworte:	artificial photosynthesis carbon dioxide reduction graphene INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY nickel single atoms oxygen evolution reaction renewable energy single-atom catalysis SOLAR ENERGY solar-to-fuel conversion three-dimensional atom probe tomography transition metals
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