Carbon nanotubes as emerging quantum-light sources
Progress in quantum computing and quantum cryptography requires efficient, electrically triggered, single-photon sources at room temperature in the telecom wavelengths. It has been long known that semiconducting single-wall carbon nanotubes (SWCNTs) display strong excitonic binding and emit light ov...
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Veröffentlicht in: | Nature materials 2018-08, Vol.17 (8), p.663-670 |
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description | Progress in quantum computing and quantum cryptography requires efficient, electrically triggered, single-photon sources at room temperature in the telecom wavelengths. It has been long known that semiconducting single-wall carbon nanotubes (SWCNTs) display strong excitonic binding and emit light over a broad range of wavelengths, but their use has been hampered by a low quantum yield and a high sensitivity to spectral diffusion and blinking. In this Perspective, we discuss recent advances in the mastering of SWCNT optical properties by chemistry, electrical contacting and resonator coupling towards advancing their use as quantum light sources. We describe the latest results in terms of single-photon purity, generation efficiency and indistinguishability. Finally, we consider the main fundamental challenges stemming from the unique properties of SWCNTs and the most promising roads for SWCNT-based chip integrated quantum photonic sources.
This Perspective describes the recent advances in understanding and controlling the properties of single-wall carbon nanotubes as well as the progress towards the fabrication of new electrically driven single-photon sources. |
doi_str_mv | 10.1038/s41563-018-0109-2 |
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This Perspective describes the recent advances in understanding and controlling the properties of single-wall carbon nanotubes as well as the progress towards the fabrication of new electrically driven single-photon sources.</description><identifier>ISSN: 1476-1122</identifier><identifier>EISSN: 1476-4660</identifier><identifier>DOI: 10.1038/s41563-018-0109-2</identifier><identifier>PMID: 29915427</identifier><language>eng</language><publisher>London: Nature Publishing Group UK</publisher><subject>140/125 ; 639/624/399/1097 ; 639/638/541 ; 639/766/483/3925 ; 639/925/357/73 ; 639/925/927/1021 ; Biomaterials ; Blinking ; Chemistry and Materials Science ; Condensed Matter Physics ; Light sources ; Mastering ; Material Science ; Materials Science ; Nanotechnology ; Nanotubes ; Optical and Electronic Materials ; Optical properties ; Organic chemistry ; Perspective ; Photonics ; Quantum computing ; Quantum cryptography ; Single wall carbon nanotubes ; Spectral sensitivity ; Wavelengths</subject><ispartof>Nature materials, 2018-08, Vol.17 (8), p.663-670</ispartof><rights>Springer Nature Limited 2018</rights><rights>Copyright Nature Publishing Group Aug 2018</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c399t-fa17353a78e0a9b15c38a8295b82d8976db1cf999ecc3275a3d0c150ba4628153</citedby><cites>FETCH-LOGICAL-c399t-fa17353a78e0a9b15c38a8295b82d8976db1cf999ecc3275a3d0c150ba4628153</cites><orcidid>0000-0003-3696-2896 ; 0000-0003-4569-4213 ; 0000-0002-2232-2778 ; 0000-0002-4982-8250 ; 0000-0003-3175-9311 ; 0000-0002-0588-2458 ; 0000-0002-9535-2062 ; 0000000331759311 ; 0000000345694213 ; 0000000249828250 ; 0000000336962896 ; 0000000205882458 ; 0000000295352062 ; 0000000222322778</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>230,315,782,786,887,27933,27934</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/29915427$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink><backlink>$$Uhttps://www.osti.gov/biblio/1477723$$D View this record in Osti.gov$$Hfree_for_read</backlink></links><search><creatorcontrib>He, X.</creatorcontrib><creatorcontrib>Htoon, H.</creatorcontrib><creatorcontrib>Doorn, S. K.</creatorcontrib><creatorcontrib>Pernice, W. H. P.</creatorcontrib><creatorcontrib>Pyatkov, F.</creatorcontrib><creatorcontrib>Krupke, R.</creatorcontrib><creatorcontrib>Jeantet, A.</creatorcontrib><creatorcontrib>Chassagneux, Y.</creatorcontrib><creatorcontrib>Voisin, C.</creatorcontrib><creatorcontrib>Los Alamos National Lab. (LANL), Los Alamos, NM (United States)</creatorcontrib><title>Carbon nanotubes as emerging quantum-light sources</title><title>Nature materials</title><addtitle>Nature Mater</addtitle><addtitle>Nat Mater</addtitle><description>Progress in quantum computing and quantum cryptography requires efficient, electrically triggered, single-photon sources at room temperature in the telecom wavelengths. It has been long known that semiconducting single-wall carbon nanotubes (SWCNTs) display strong excitonic binding and emit light over a broad range of wavelengths, but their use has been hampered by a low quantum yield and a high sensitivity to spectral diffusion and blinking. In this Perspective, we discuss recent advances in the mastering of SWCNT optical properties by chemistry, electrical contacting and resonator coupling towards advancing their use as quantum light sources. We describe the latest results in terms of single-photon purity, generation efficiency and indistinguishability. Finally, we consider the main fundamental challenges stemming from the unique properties of SWCNTs and the most promising roads for SWCNT-based chip integrated quantum photonic sources.
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K.</au><au>Pernice, W. H. P.</au><au>Pyatkov, F.</au><au>Krupke, R.</au><au>Jeantet, A.</au><au>Chassagneux, Y.</au><au>Voisin, C.</au><aucorp>Los Alamos National Lab. (LANL), Los Alamos, NM (United States)</aucorp><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Carbon nanotubes as emerging quantum-light sources</atitle><jtitle>Nature materials</jtitle><stitle>Nature Mater</stitle><addtitle>Nat Mater</addtitle><date>2018-08-01</date><risdate>2018</risdate><volume>17</volume><issue>8</issue><spage>663</spage><epage>670</epage><pages>663-670</pages><issn>1476-1122</issn><eissn>1476-4660</eissn><abstract>Progress in quantum computing and quantum cryptography requires efficient, electrically triggered, single-photon sources at room temperature in the telecom wavelengths. It has been long known that semiconducting single-wall carbon nanotubes (SWCNTs) display strong excitonic binding and emit light over a broad range of wavelengths, but their use has been hampered by a low quantum yield and a high sensitivity to spectral diffusion and blinking. In this Perspective, we discuss recent advances in the mastering of SWCNT optical properties by chemistry, electrical contacting and resonator coupling towards advancing their use as quantum light sources. We describe the latest results in terms of single-photon purity, generation efficiency and indistinguishability. Finally, we consider the main fundamental challenges stemming from the unique properties of SWCNTs and the most promising roads for SWCNT-based chip integrated quantum photonic sources.
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subjects | 140/125 639/624/399/1097 639/638/541 639/766/483/3925 639/925/357/73 639/925/927/1021 Biomaterials Blinking Chemistry and Materials Science Condensed Matter Physics Light sources Mastering Material Science Materials Science Nanotechnology Nanotubes Optical and Electronic Materials Optical properties Organic chemistry Perspective Photonics Quantum computing Quantum cryptography Single wall carbon nanotubes Spectral sensitivity Wavelengths |
title | Carbon nanotubes as emerging quantum-light sources |
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