Experimental and modeling study of calcium carbonate precipitation and its effects on the degradation of oil well cement during carbonated brine exposure

Decalcification of cement in solutions of carbonated brine is important to a host of engineering applications, especially in subsurface service environments where cementitious materials are frequently utilized as engineered barriers for wellbore seals, as well as shaft and drift seals and waste form...

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Veröffentlicht in:Cement and concrete research 2018-11, Vol.113, p.1-12
Hauptverfasser: Matteo, Edward N., Huet, Bruno, Jové-Colón, Carlos F., Scherer, George W.
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container_end_page 12
container_issue
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container_title Cement and concrete research
container_volume 113
creator Matteo, Edward N.
Huet, Bruno
Jové-Colón, Carlos F.
Scherer, George W.
description Decalcification of cement in solutions of carbonated brine is important to a host of engineering applications, especially in subsurface service environments where cementitious materials are frequently utilized as engineered barriers for wellbore seals, as well as shaft and drift seals and waste forms for nuclear waste disposal. Analysis of leaching simulations and experiments shows that, depending on solution compositions (dissolved CO2 concentration, pH, Ca ion concentration), calcite precipitation occurring during leaching of cement in contact with carbonated brine can have a significant impact on cement reactivity, in some instances leading to complete arrest of reactivity via calcium carbonate “pore-clogging”. We present modeling and experimental results that examine the range of solution conditions that can lead to pore-clogging. Analysis of the results shows that distinct regimes of leaching behavior, based on pH and pCO2, can be used to form a framework to better understand the occurrence of pore-clogging.
doi_str_mv 10.1016/j.cemconres.2018.03.016
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Analysis of leaching simulations and experiments shows that, depending on solution compositions (dissolved CO2 concentration, pH, Ca ion concentration), calcite precipitation occurring during leaching of cement in contact with carbonated brine can have a significant impact on cement reactivity, in some instances leading to complete arrest of reactivity via calcium carbonate “pore-clogging”. We present modeling and experimental results that examine the range of solution conditions that can lead to pore-clogging. 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source Elsevier ScienceDirect Journals
subjects CaCO3
Calcite
Calcium
Calcium carbonate
Carbonation
Cement
Chemical compounds
Chemical precipitation
Computer simulation
Diffusion
Durability
Ion concentration
Leaching
Materials durability
MATERIALS SCIENCE
Modeling
Modelling
Oil well cement
Radioactive waste disposal
Radioactive wastes
Saline water
SEM
title Experimental and modeling study of calcium carbonate precipitation and its effects on the degradation of oil well cement during carbonated brine exposure
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