Collapse of superconductivity in cuprates via ultrafast quenching of phase coherence
The possibility of driving phase transitions in low-density condensates through the loss of phase coherence alone has far-reaching implications for the study of quantum phases of matter. This has inspired the development of tools to control and explore the collective properties of condensate phases...
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Veröffentlicht in: | Nature materials 2018-05, Vol.17 (5), p.416-420 |
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creator | Boschini, F. da Silva Neto, E. H. Razzoli, E. Zonno, M. Peli, S. Day, R. P. Michiardi, M. Schneider, M. Zwartsenberg, B. Nigge, P. Zhong, R. D. Schneeloch, J. Gu, G. D. Zhdanovich, S. Mills, A. K. Levy, G. Jones, D. J. Giannetti, C. Damascelli, A. |
description | The possibility of driving phase transitions in low-density condensates through the loss of phase coherence alone has far-reaching implications for the study of quantum phases of matter. This has inspired the development of tools to control and explore the collective properties of condensate phases via phase fluctuations. Electrically gated oxide interfaces
1
,
2
, ultracold Fermi atoms
3
,
4
and cuprate superconductors
5
,
6
, which are characterized by an intrinsically small phase stiffness, are paradigmatic examples where these tools are having a dramatic impact. Here we use light pulses shorter than the internal thermalization time to drive and probe the phase fragility of the Bi
2
Sr
2
CaCu
2
O
8+
δ
cuprate superconductor, completely melting the superconducting condensate without affecting the pairing strength. The resulting ultrafast dynamics of phase fluctuations and charge excitations are captured and disentangled by time-resolved photoemission spectroscopy. This work demonstrates the dominant role of phase coherence in the superconductor-to-normal state phase transition and offers a benchmark for non-equilibrium spectroscopic investigations of the cuprate phase diagram.
Pump–probe, time-resolved ARPES experiments with underdoped cuprates reveal the transient enhancement of the density of phase fluctuations, eventually leading to the collapse of superconductivity. |
doi_str_mv | 10.1038/s41563-018-0045-1 |
format | Article |
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1
,
2
, ultracold Fermi atoms
3
,
4
and cuprate superconductors
5
,
6
, which are characterized by an intrinsically small phase stiffness, are paradigmatic examples where these tools are having a dramatic impact. Here we use light pulses shorter than the internal thermalization time to drive and probe the phase fragility of the Bi
2
Sr
2
CaCu
2
O
8+
δ
cuprate superconductor, completely melting the superconducting condensate without affecting the pairing strength. The resulting ultrafast dynamics of phase fluctuations and charge excitations are captured and disentangled by time-resolved photoemission spectroscopy. This work demonstrates the dominant role of phase coherence in the superconductor-to-normal state phase transition and offers a benchmark for non-equilibrium spectroscopic investigations of the cuprate phase diagram.
Pump–probe, time-resolved ARPES experiments with underdoped cuprates reveal the transient enhancement of the density of phase fluctuations, eventually leading to the collapse of superconductivity.</description><identifier>ISSN: 1476-1122</identifier><identifier>EISSN: 1476-4660</identifier><identifier>DOI: 10.1038/s41563-018-0045-1</identifier><identifier>PMID: 29610487</identifier><language>eng</language><publisher>London: Nature Publishing Group UK</publisher><subject>140/125 ; 639/766/119 ; 639/766/119/1003 ; 639/766/119/2795 ; Biomaterials ; Chemistry and Materials Science ; Condensates ; Condensed Matter Physics ; CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY ; Cuprates ; Fluctuations ; Fragility ; Letter ; Materials Science ; Nanotechnology ; Optical and Electronic Materials ; Phase coherence ; Phase transitions ; Photoelectric emission ; Stiffness ; Superconductivity ; Thermalization (energy absorption) ; Variation</subject><ispartof>Nature materials, 2018-05, Vol.17 (5), p.416-420</ispartof><rights>The Author(s) 2018</rights><rights>Copyright Nature Publishing Group May 2018</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c508t-b3d59656c2ad7df36b270f82be84697be770fe883feb9c93acdd6f57119637f33</citedby><cites>FETCH-LOGICAL-c508t-b3d59656c2ad7df36b270f82be84697be770fe883feb9c93acdd6f57119637f33</cites><orcidid>0000-0003-1652-9454 ; 0000-0003-2664-9492 ; 0000000326649492 ; 0000000298863255 ; 0000000316529454</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1038/s41563-018-0045-1$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1038/s41563-018-0045-1$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>230,314,776,780,881,27901,27902,41464,42533,51294</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/29610487$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink><backlink>$$Uhttps://www.osti.gov/servlets/purl/1440896$$D View this record in Osti.gov$$Hfree_for_read</backlink></links><search><creatorcontrib>Boschini, F.</creatorcontrib><creatorcontrib>da Silva Neto, E. H.</creatorcontrib><creatorcontrib>Razzoli, E.</creatorcontrib><creatorcontrib>Zonno, M.</creatorcontrib><creatorcontrib>Peli, S.</creatorcontrib><creatorcontrib>Day, R. P.</creatorcontrib><creatorcontrib>Michiardi, M.</creatorcontrib><creatorcontrib>Schneider, M.</creatorcontrib><creatorcontrib>Zwartsenberg, B.</creatorcontrib><creatorcontrib>Nigge, P.</creatorcontrib><creatorcontrib>Zhong, R. D.</creatorcontrib><creatorcontrib>Schneeloch, J.</creatorcontrib><creatorcontrib>Gu, G. D.</creatorcontrib><creatorcontrib>Zhdanovich, S.</creatorcontrib><creatorcontrib>Mills, A. K.</creatorcontrib><creatorcontrib>Levy, G.</creatorcontrib><creatorcontrib>Jones, D. J.</creatorcontrib><creatorcontrib>Giannetti, C.</creatorcontrib><creatorcontrib>Damascelli, A.</creatorcontrib><creatorcontrib>Energy Frontier Research Centers (EFRC) (United States). Center for Emergent Superconductivity (CES)</creatorcontrib><creatorcontrib>Brookhaven National Laboratory (BNL), Upton, NY (United States)</creatorcontrib><title>Collapse of superconductivity in cuprates via ultrafast quenching of phase coherence</title><title>Nature materials</title><addtitle>Nature Mater</addtitle><addtitle>Nat Mater</addtitle><description>The possibility of driving phase transitions in low-density condensates through the loss of phase coherence alone has far-reaching implications for the study of quantum phases of matter. This has inspired the development of tools to control and explore the collective properties of condensate phases via phase fluctuations. Electrically gated oxide interfaces
1
,
2
, ultracold Fermi atoms
3
,
4
and cuprate superconductors
5
,
6
, which are characterized by an intrinsically small phase stiffness, are paradigmatic examples where these tools are having a dramatic impact. Here we use light pulses shorter than the internal thermalization time to drive and probe the phase fragility of the Bi
2
Sr
2
CaCu
2
O
8+
δ
cuprate superconductor, completely melting the superconducting condensate without affecting the pairing strength. The resulting ultrafast dynamics of phase fluctuations and charge excitations are captured and disentangled by time-resolved photoemission spectroscopy. This work demonstrates the dominant role of phase coherence in the superconductor-to-normal state phase transition and offers a benchmark for non-equilibrium spectroscopic investigations of the cuprate phase diagram.
Pump–probe, time-resolved ARPES experiments with underdoped cuprates reveal the transient enhancement of the density of phase fluctuations, eventually leading to the collapse of superconductivity.</description><subject>140/125</subject><subject>639/766/119</subject><subject>639/766/119/1003</subject><subject>639/766/119/2795</subject><subject>Biomaterials</subject><subject>Chemistry and Materials Science</subject><subject>Condensates</subject><subject>Condensed Matter Physics</subject><subject>CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY</subject><subject>Cuprates</subject><subject>Fluctuations</subject><subject>Fragility</subject><subject>Letter</subject><subject>Materials Science</subject><subject>Nanotechnology</subject><subject>Optical and Electronic Materials</subject><subject>Phase coherence</subject><subject>Phase transitions</subject><subject>Photoelectric emission</subject><subject>Stiffness</subject><subject>Superconductivity</subject><subject>Thermalization (energy absorption)</subject><subject>Variation</subject><issn>1476-1122</issn><issn>1476-4660</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2018</creationdate><recordtype>article</recordtype><sourceid>BENPR</sourceid><recordid>eNp1kUtP3DAUhS1UxMDAD2BTRe2GTcDvOMtqVGglpG5gbTnONWM0E6e2MxL_HkcZWqlSV3599_jecxC6JviWYKbuEidCshoTVWPMRU1O0Dnhjay5lPjTcU8IpSt0kdIrxpQIIc_QiraSYK6ac_S0CbudGRNUwVVpGiHaMPSTzf7g81vlh8pOYzQZUnXwppp2ORpnUq5-TzDYrR9e5sJxa4qCDVuI5RYu0akzuwRXx3WNnu-_P21-1I-_Hn5uvj3WVmCV6471opVCWmr6pndMdrTBTtEOFJdt00FTjqAUc9C1tmXG9r10oiGklaxxjK3Rl0U3pOx1sj6D3Zb-B7BZE86xKuAa3SzQGENpOmW998lCmXqAMCVNiyuMclocXaOv_6CvYYpDGWGmWtHi4lqhyELZGFKK4PQY_d7EN02wnnPRSy665KLnXDQpNZ-PylO3h_5PxUcQBaALkMrT8ALx79f_V30HK7iXxg</recordid><startdate>20180501</startdate><enddate>20180501</enddate><creator>Boschini, F.</creator><creator>da Silva Neto, E. 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H. ; Razzoli, E. ; Zonno, M. ; Peli, S. ; Day, R. P. ; Michiardi, M. ; Schneider, M. ; Zwartsenberg, B. ; Nigge, P. ; Zhong, R. D. ; Schneeloch, J. ; Gu, G. D. ; Zhdanovich, S. ; Mills, A. K. ; Levy, G. ; Jones, D. 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H.</au><au>Razzoli, E.</au><au>Zonno, M.</au><au>Peli, S.</au><au>Day, R. P.</au><au>Michiardi, M.</au><au>Schneider, M.</au><au>Zwartsenberg, B.</au><au>Nigge, P.</au><au>Zhong, R. D.</au><au>Schneeloch, J.</au><au>Gu, G. D.</au><au>Zhdanovich, S.</au><au>Mills, A. K.</au><au>Levy, G.</au><au>Jones, D. J.</au><au>Giannetti, C.</au><au>Damascelli, A.</au><aucorp>Energy Frontier Research Centers (EFRC) (United States). Center for Emergent Superconductivity (CES)</aucorp><aucorp>Brookhaven National Laboratory (BNL), Upton, NY (United States)</aucorp><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Collapse of superconductivity in cuprates via ultrafast quenching of phase coherence</atitle><jtitle>Nature materials</jtitle><stitle>Nature Mater</stitle><addtitle>Nat Mater</addtitle><date>2018-05-01</date><risdate>2018</risdate><volume>17</volume><issue>5</issue><spage>416</spage><epage>420</epage><pages>416-420</pages><issn>1476-1122</issn><eissn>1476-4660</eissn><abstract>The possibility of driving phase transitions in low-density condensates through the loss of phase coherence alone has far-reaching implications for the study of quantum phases of matter. This has inspired the development of tools to control and explore the collective properties of condensate phases via phase fluctuations. Electrically gated oxide interfaces
1
,
2
, ultracold Fermi atoms
3
,
4
and cuprate superconductors
5
,
6
, which are characterized by an intrinsically small phase stiffness, are paradigmatic examples where these tools are having a dramatic impact. Here we use light pulses shorter than the internal thermalization time to drive and probe the phase fragility of the Bi
2
Sr
2
CaCu
2
O
8+
δ
cuprate superconductor, completely melting the superconducting condensate without affecting the pairing strength. The resulting ultrafast dynamics of phase fluctuations and charge excitations are captured and disentangled by time-resolved photoemission spectroscopy. This work demonstrates the dominant role of phase coherence in the superconductor-to-normal state phase transition and offers a benchmark for non-equilibrium spectroscopic investigations of the cuprate phase diagram.
Pump–probe, time-resolved ARPES experiments with underdoped cuprates reveal the transient enhancement of the density of phase fluctuations, eventually leading to the collapse of superconductivity.</abstract><cop>London</cop><pub>Nature Publishing Group UK</pub><pmid>29610487</pmid><doi>10.1038/s41563-018-0045-1</doi><tpages>5</tpages><orcidid>https://orcid.org/0000-0003-1652-9454</orcidid><orcidid>https://orcid.org/0000-0003-2664-9492</orcidid><orcidid>https://orcid.org/0000000326649492</orcidid><orcidid>https://orcid.org/0000000298863255</orcidid><orcidid>https://orcid.org/0000000316529454</orcidid><oa>free_for_read</oa></addata></record> |
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subjects | 140/125 639/766/119 639/766/119/1003 639/766/119/2795 Biomaterials Chemistry and Materials Science Condensates Condensed Matter Physics CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY Cuprates Fluctuations Fragility Letter Materials Science Nanotechnology Optical and Electronic Materials Phase coherence Phase transitions Photoelectric emission Stiffness Superconductivity Thermalization (energy absorption) Variation |
title | Collapse of superconductivity in cuprates via ultrafast quenching of phase coherence |
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