Building superlattices from individual nanoparticles via template-confined DNA-mediated assembly
DNA programmable assembly has been combined with top-down lithography to construct superlattices of discrete, reconfigurable nanoparticle architectures on a gold surface over large areas. Specifically, the assembly of individual colloidal plasmonic nanoparticles with different shapes and sizes is co...
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| Veröffentlicht in: | Science (American Association for the Advancement of Science) 2018-02, Vol.359 (6376), p.669-672 |
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| creator | Lin, Qing-Yuan Mason, Jarad A Li, Zhongyang Zhou, Wenjie O'Brien, Matthew N Brown, Keith A Jones, Matthew R Butun, Serkan Lee, Byeongdu Dravid, Vinayak P Aydin, Koray Mirkin, Chad A |
| description | DNA programmable assembly has been combined with top-down lithography to construct superlattices of discrete, reconfigurable nanoparticle architectures on a gold surface over large areas. Specifically, the assembly of individual colloidal plasmonic nanoparticles with different shapes and sizes is controlled by oligonucleotides containing "locked" nucleic acids and confined environments provided by polymer pores to yield oriented architectures that feature tunable arrangements and independently controllable distances at both nanometer- and micrometer-length scales. These structures, which would be difficult to construct by other common assembly methods, provide a platform to systematically study and control light-matter interactions in nanoparticle-based optical materials. The generality and potential of this approach are explored by identifying a broadband absorber with a solvent polarity response that allows dynamic tuning of visible light absorption. |
| doi_str_mv | 10.1126/science.aaq0591 |
| format | Article |
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Center for Bio-Inspired Energy Science (CBES)</creatorcontrib><creatorcontrib>Argonne National Lab. (ANL), Argonne, IL (United States)</creatorcontrib><title>Building superlattices from individual nanoparticles via template-confined DNA-mediated assembly</title><title>Science (American Association for the Advancement of Science)</title><addtitle>Science</addtitle><description>DNA programmable assembly has been combined with top-down lithography to construct superlattices of discrete, reconfigurable nanoparticle architectures on a gold surface over large areas. Specifically, the assembly of individual colloidal plasmonic nanoparticles with different shapes and sizes is controlled by oligonucleotides containing "locked" nucleic acids and confined environments provided by polymer pores to yield oriented architectures that feature tunable arrangements and independently controllable distances at both nanometer- and micrometer-length scales. These structures, which would be difficult to construct by other common assembly methods, provide a platform to systematically study and control light-matter interactions in nanoparticle-based optical materials. The generality and potential of this approach are explored by identifying a broadband absorber with a solvent polarity response that allows dynamic tuning of visible light absorption.</description><subject>Adenine</subject><subject>Assembly</subject><subject>Base pairs</subject><subject>Broadband</subject><subject>Confined spaces</subject><subject>Deoxyribonucleic acid</subject><subject>DNA</subject><subject>Electromagnetic absorption</subject><subject>Gold</subject><subject>MATERIALS SCIENCE</subject><subject>Nanoparticles</subject><subject>NANOSCIENCE AND NANOTECHNOLOGY</subject><subject>Nucleic acids</subject><subject>Oligonucleotides</subject><subject>Optical materials</subject><subject>Optics</subject><subject>Polarity</subject><subject>Polymers</subject><subject>Ribose</subject><subject>Stability</subject><subject>Stacks</subject><subject>Strands</subject><subject>Superlattices</subject><issn>0036-8075</issn><issn>1095-9203</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2018</creationdate><recordtype>article</recordtype><recordid>eNpdkbtPwzAQhy0EouUxs6EIFpaAH3Ecj1CeEoKlu3HsCxglTrCTSv3vMWphYLJ033cn3_0QOiH4khBaXkXjwBu41PoLc0l20JxgyXNJMdtFc4xZmVdY8Bk6iPET48Qk20czKllRsbKYo7ebybXW-fcsTgOEVo-jMxCzJvRd5rx1K2cn3WZe-37QIcE20ZXT2QjdkHTITe8b58Fmty_XeQfWpaLNdIzQ1e36CO01uo1wvH0P0fL-brl4zJ9fH54W18-5Kbgcc2FZY4WtrRVgKl3YEhpCa17XpjRUa2MkcJFYo2sjMAhDeVFJXkOBE2eH6Gwzto-jU-ksI5iP9DMPZlSkoCWpRJIuNtIQ-q8J4qg6Fw20rfbQT1ERWckSC8FpUs__qZ_9FHzaIFlSioJWjCTramOZ0McYoFFDcJ0Oa0Ww-glIbQNS24BSx-l27lSnW_35v4mwbwoJkN4</recordid><startdate>20180209</startdate><enddate>20180209</enddate><creator>Lin, Qing-Yuan</creator><creator>Mason, Jarad A</creator><creator>Li, Zhongyang</creator><creator>Zhou, Wenjie</creator><creator>O'Brien, Matthew N</creator><creator>Brown, Keith A</creator><creator>Jones, Matthew R</creator><creator>Butun, Serkan</creator><creator>Lee, Byeongdu</creator><creator>Dravid, Vinayak P</creator><creator>Aydin, Koray</creator><creator>Mirkin, Chad A</creator><general>The American Association for the Advancement of Science</general><general>AAAS</general><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7QF</scope><scope>7QG</scope><scope>7QL</scope><scope>7QP</scope><scope>7QQ</scope><scope>7QR</scope><scope>7SC</scope><scope>7SE</scope><scope>7SN</scope><scope>7SP</scope><scope>7SR</scope><scope>7SS</scope><scope>7T7</scope><scope>7TA</scope><scope>7TB</scope><scope>7TK</scope><scope>7TM</scope><scope>7U5</scope><scope>7U9</scope><scope>8BQ</scope><scope>8FD</scope><scope>C1K</scope><scope>F28</scope><scope>FR3</scope><scope>H8D</scope><scope>H8G</scope><scope>H94</scope><scope>JG9</scope><scope>JQ2</scope><scope>K9.</scope><scope>KR7</scope><scope>L7M</scope><scope>L~C</scope><scope>L~D</scope><scope>M7N</scope><scope>P64</scope><scope>RC3</scope><scope>7X8</scope><scope>OIOZB</scope><scope>OTOTI</scope><orcidid>https://orcid.org/0000-0003-0592-5339</orcidid><orcidid>https://orcid.org/0000-0002-1721-0464</orcidid><orcidid>https://orcid.org/0000-0002-6007-3063</orcidid><orcidid>https://orcid.org/0000-0002-7626-4032</orcidid><orcidid>https://orcid.org/0000-0001-9306-9311</orcidid><orcidid>https://orcid.org/0000-0001-6349-9185</orcidid><orcidid>https://orcid.org/0000-0002-2379-2018</orcidid><orcidid>https://orcid.org/0000-0002-6634-7627</orcidid><orcidid>https://orcid.org/0000-0002-9289-291X</orcidid><orcidid>https://orcid.org/0000-0003-2514-8805</orcidid><orcidid>https://orcid.org/0000-0002-3268-2216</orcidid><orcidid>https://orcid.org/0000-0003-0328-7775</orcidid><orcidid>https://orcid.org/0000000260073063</orcidid><orcidid>https://orcid.org/0000000232682216</orcidid><orcidid>https://orcid.org/0000000193069311</orcidid><orcidid>https://orcid.org/0000000223792018</orcidid><orcidid>https://orcid.org/0000000305925339</orcidid><orcidid>https://orcid.org/0000000303287775</orcidid><orcidid>https://orcid.org/0000000217210464</orcidid><orcidid>https://orcid.org/0000000266347627</orcidid><orcidid>https://orcid.org/0000000325148805</orcidid><orcidid>https://orcid.org/000000029289291X</orcidid><orcidid>https://orcid.org/0000000163499185</orcidid><orcidid>https://orcid.org/0000000276264032</orcidid></search><sort><creationdate>20180209</creationdate><title>Building superlattices from individual nanoparticles via template-confined DNA-mediated assembly</title><author>Lin, Qing-Yuan ; 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| identifier | ISSN: 0036-8075 |
| ispartof | Science (American Association for the Advancement of Science), 2018-02, Vol.359 (6376), p.669-672 |
| issn | 0036-8075 1095-9203 |
| language | eng |
| recordid | cdi_osti_scitechconnect_1426187 |
| source | American Association for the Advancement of Science; Jstor Complete Legacy |
| subjects | Adenine Assembly Base pairs Broadband Confined spaces Deoxyribonucleic acid DNA Electromagnetic absorption Gold MATERIALS SCIENCE Nanoparticles NANOSCIENCE AND NANOTECHNOLOGY Nucleic acids Oligonucleotides Optical materials Optics Polarity Polymers Ribose Stability Stacks Strands Superlattices |
| title | Building superlattices from individual nanoparticles via template-confined DNA-mediated assembly |
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