Progress in the Development of Oxygen Reduction Reaction Catalysts for Low-Temperature Fuel Cells
We present a brief summary on the most recent progress in the design of catalysts for electrochemical reduction of oxygen. The main challenge in the wide spread of fuel cell technology is to lower the content of, or even eliminate, Pt and other precious metals in catalysts without sacrificing their...
Gespeichert in:
| Veröffentlicht in: | Annual review of chemical and biomolecular engineering 2016-06, Vol.7 (1), p.509-532 |
|---|---|
| Hauptverfasser: | , , , , |
| Format: | Artikel |
| Sprache: | eng |
| Schlagworte: | |
| Online-Zugang: | Volltext |
| Tags: |
Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
|
| container_end_page | 532 |
|---|---|
| container_issue | 1 |
| container_start_page | 509 |
| container_title | Annual review of chemical and biomolecular engineering |
| container_volume | 7 |
| creator | Li, Dongguo Lv, Haifeng Kang, Yijin Markovic, Nenad M Stamenkovic, Vojislav R |
| description | We present a brief summary on the most recent progress in the design of catalysts for electrochemical reduction of oxygen. The main challenge in the wide spread of fuel cell technology is to lower the content of, or even eliminate, Pt and other precious metals in catalysts without sacrificing their performance. Pt-based nanosized catalysts with novel and refined architectures continue to dominate in catalytic performance, and formation of Pt-skin-like surfaces is key to achieving the highest values in activity. Moreover, durability has also been improved in Pt-based systems with addition of Au, which plays an important role in stabilizing the Pt topmost layers against dissolution. However, various carbon-based materials without precious metal have shown improvement in activity and durability and have been explored to serve as catalyst supports. Understanding how the doped elements interact with each other and or carbon is challenging and necessary in the design of robust fuel cell catalysts. |
| doi_str_mv | 10.1146/annurev-chembioeng-080615-034526 |
| format | Article |
| fullrecord | <record><control><sourceid>proquest_osti_</sourceid><recordid>TN_cdi_osti_scitechconnect_1352589</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>1795878756</sourcerecordid><originalsourceid>FETCH-LOGICAL-a544t-e73dd580f9516bc22196f4f82c1c6f763f7d3b28f2925cce3c601a84a4a21e9a3</originalsourceid><addsrcrecordid>eNqVkU1v1DAURSMEoqXwF5DFqpuAv-3sQNMWkEYqQmVteZznmaDEHmynZf49HmUoS0Be-C6O7rvSaZpLgt8SwuU7G8Kc4L51O5g2Q4SwbbHGkogWMy6ofNKck46rVnAunz5mps-aFzl_x1gqLfnz5owqXJ-U5439kuI2Qc5oCKjsAF3BPYxxP0EoKHp0-_OwhYC-Qj-7MsRjsktY2WLHQy4Z-ZjQOj60dzDtIdlSJ6KbGUa0gnHML5tn3o4ZXp3-i-bbzfXd6lO7vv34efVh3dq6trSgWN8LjX0niNw4SkknPfeaOuKkV5J51bMN1Z52VDgHzElMrOaWW0qgs-yiebP0xlwGk91QwO1cDAFcMYQJKnRXocsF2qf4Y4ZczDRkV2faAHHOhmgmJJFYqH9ACdGad1L8HVWd0EorISv6fkFdijkn8GafhsmmgyHYHB2bk2Pzx7FZHJvFca14fbo2byboHwt-S63A9QIcq-xYywZ4yP9_6BcT_cCZ</addsrcrecordid><sourcetype>Open Access Repository</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>1795878756</pqid></control><display><type>article</type><title>Progress in the Development of Oxygen Reduction Reaction Catalysts for Low-Temperature Fuel Cells</title><source>Annual Reviews Complete A-Z List</source><source>MEDLINE</source><creator>Li, Dongguo ; Lv, Haifeng ; Kang, Yijin ; Markovic, Nenad M ; Stamenkovic, Vojislav R</creator><creatorcontrib>Li, Dongguo ; Lv, Haifeng ; Kang, Yijin ; Markovic, Nenad M ; Stamenkovic, Vojislav R ; Argonne National Laboratory (ANL), Argonne, IL (United States)</creatorcontrib><description>We present a brief summary on the most recent progress in the design of catalysts for electrochemical reduction of oxygen. The main challenge in the wide spread of fuel cell technology is to lower the content of, or even eliminate, Pt and other precious metals in catalysts without sacrificing their performance. Pt-based nanosized catalysts with novel and refined architectures continue to dominate in catalytic performance, and formation of Pt-skin-like surfaces is key to achieving the highest values in activity. Moreover, durability has also been improved in Pt-based systems with addition of Au, which plays an important role in stabilizing the Pt topmost layers against dissolution. However, various carbon-based materials without precious metal have shown improvement in activity and durability and have been explored to serve as catalyst supports. Understanding how the doped elements interact with each other and or carbon is challenging and necessary in the design of robust fuel cell catalysts.</description><identifier>ISSN: 1947-5438</identifier><identifier>EISSN: 1947-5446</identifier><identifier>DOI: 10.1146/annurev-chembioeng-080615-034526</identifier><identifier>PMID: 27070766</identifier><language>eng</language><publisher>United States: Annual Reviews</publisher><subject>Carbon ; Carbon - chemistry ; Catalysis ; Catalysts ; Core-shell ; Design engineering ; Durability ; Electrochemical Techniques ; Electrochemistry ; Fuel cells ; INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY ; MATERIALS SCIENCE ; Nanoparticle ; Nanoparticles - chemistry ; Oxidation-Reduction ; Oxygen ; Oxygen - chemistry ; Platinum ; Platinum - chemistry ; Precious metals ; Temperature ; Thin films</subject><ispartof>Annual review of chemical and biomolecular engineering, 2016-06, Vol.7 (1), p.509-532</ispartof><rights>2016</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-a544t-e73dd580f9516bc22196f4f82c1c6f763f7d3b28f2925cce3c601a84a4a21e9a3</citedby><cites>FETCH-LOGICAL-a544t-e73dd580f9516bc22196f4f82c1c6f763f7d3b28f2925cce3c601a84a4a21e9a3</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://www.annualreviews.org/content/journals/10.1146/annurev-chembioeng-080615-034526?crawler=true&mimetype=application/pdf$$EPDF$$P50$$Gannualreviews$$H</linktopdf><linktohtml>$$Uhttps://www.annualreviews.org/content/journals/10.1146/annurev-chembioeng-080615-034526$$EHTML$$P50$$Gannualreviews$$H</linktohtml><link.rule.ids>70,230,314,780,784,885,4182,27924,27925,78254,78255</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/27070766$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink><backlink>$$Uhttps://www.osti.gov/servlets/purl/1352589$$D View this record in Osti.gov$$Hfree_for_read</backlink></links><search><creatorcontrib>Li, Dongguo</creatorcontrib><creatorcontrib>Lv, Haifeng</creatorcontrib><creatorcontrib>Kang, Yijin</creatorcontrib><creatorcontrib>Markovic, Nenad M</creatorcontrib><creatorcontrib>Stamenkovic, Vojislav R</creatorcontrib><creatorcontrib>Argonne National Laboratory (ANL), Argonne, IL (United States)</creatorcontrib><title>Progress in the Development of Oxygen Reduction Reaction Catalysts for Low-Temperature Fuel Cells</title><title>Annual review of chemical and biomolecular engineering</title><addtitle>Annu Rev Chem Biomol Eng</addtitle><description>We present a brief summary on the most recent progress in the design of catalysts for electrochemical reduction of oxygen. The main challenge in the wide spread of fuel cell technology is to lower the content of, or even eliminate, Pt and other precious metals in catalysts without sacrificing their performance. Pt-based nanosized catalysts with novel and refined architectures continue to dominate in catalytic performance, and formation of Pt-skin-like surfaces is key to achieving the highest values in activity. Moreover, durability has also been improved in Pt-based systems with addition of Au, which plays an important role in stabilizing the Pt topmost layers against dissolution. However, various carbon-based materials without precious metal have shown improvement in activity and durability and have been explored to serve as catalyst supports. Understanding how the doped elements interact with each other and or carbon is challenging and necessary in the design of robust fuel cell catalysts.</description><subject>Carbon</subject><subject>Carbon - chemistry</subject><subject>Catalysis</subject><subject>Catalysts</subject><subject>Core-shell</subject><subject>Design engineering</subject><subject>Durability</subject><subject>Electrochemical Techniques</subject><subject>Electrochemistry</subject><subject>Fuel cells</subject><subject>INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY</subject><subject>MATERIALS SCIENCE</subject><subject>Nanoparticle</subject><subject>Nanoparticles - chemistry</subject><subject>Oxidation-Reduction</subject><subject>Oxygen</subject><subject>Oxygen - chemistry</subject><subject>Platinum</subject><subject>Platinum - chemistry</subject><subject>Precious metals</subject><subject>Temperature</subject><subject>Thin films</subject><issn>1947-5438</issn><issn>1947-5446</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2016</creationdate><recordtype>article</recordtype><sourceid>EIF</sourceid><recordid>eNqVkU1v1DAURSMEoqXwF5DFqpuAv-3sQNMWkEYqQmVteZznmaDEHmynZf49HmUoS0Be-C6O7rvSaZpLgt8SwuU7G8Kc4L51O5g2Q4SwbbHGkogWMy6ofNKck46rVnAunz5mps-aFzl_x1gqLfnz5owqXJ-U5439kuI2Qc5oCKjsAF3BPYxxP0EoKHp0-_OwhYC-Qj-7MsRjsktY2WLHQy4Z-ZjQOj60dzDtIdlSJ6KbGUa0gnHML5tn3o4ZXp3-i-bbzfXd6lO7vv34efVh3dq6trSgWN8LjX0niNw4SkknPfeaOuKkV5J51bMN1Z52VDgHzElMrOaWW0qgs-yiebP0xlwGk91QwO1cDAFcMYQJKnRXocsF2qf4Y4ZczDRkV2faAHHOhmgmJJFYqH9ACdGad1L8HVWd0EorISv6fkFdijkn8GafhsmmgyHYHB2bk2Pzx7FZHJvFca14fbo2byboHwt-S63A9QIcq-xYywZ4yP9_6BcT_cCZ</recordid><startdate>20160607</startdate><enddate>20160607</enddate><creator>Li, Dongguo</creator><creator>Lv, Haifeng</creator><creator>Kang, Yijin</creator><creator>Markovic, Nenad M</creator><creator>Stamenkovic, Vojislav R</creator><general>Annual Reviews</general><scope>CGR</scope><scope>CUY</scope><scope>CVF</scope><scope>ECM</scope><scope>EIF</scope><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7X8</scope><scope>7QO</scope><scope>8FD</scope><scope>FR3</scope><scope>P64</scope><scope>7SR</scope><scope>7U5</scope><scope>8BQ</scope><scope>JG9</scope><scope>L7M</scope><scope>OIOZB</scope><scope>OTOTI</scope></search><sort><creationdate>20160607</creationdate><title>Progress in the Development of Oxygen Reduction Reaction Catalysts for Low-Temperature Fuel Cells</title><author>Li, Dongguo ; Lv, Haifeng ; Kang, Yijin ; Markovic, Nenad M ; Stamenkovic, Vojislav R</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-a544t-e73dd580f9516bc22196f4f82c1c6f763f7d3b28f2925cce3c601a84a4a21e9a3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2016</creationdate><topic>Carbon</topic><topic>Carbon - chemistry</topic><topic>Catalysis</topic><topic>Catalysts</topic><topic>Core-shell</topic><topic>Design engineering</topic><topic>Durability</topic><topic>Electrochemical Techniques</topic><topic>Electrochemistry</topic><topic>Fuel cells</topic><topic>INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY</topic><topic>MATERIALS SCIENCE</topic><topic>Nanoparticle</topic><topic>Nanoparticles - chemistry</topic><topic>Oxidation-Reduction</topic><topic>Oxygen</topic><topic>Oxygen - chemistry</topic><topic>Platinum</topic><topic>Platinum - chemistry</topic><topic>Precious metals</topic><topic>Temperature</topic><topic>Thin films</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Li, Dongguo</creatorcontrib><creatorcontrib>Lv, Haifeng</creatorcontrib><creatorcontrib>Kang, Yijin</creatorcontrib><creatorcontrib>Markovic, Nenad M</creatorcontrib><creatorcontrib>Stamenkovic, Vojislav R</creatorcontrib><creatorcontrib>Argonne National Laboratory (ANL), Argonne, IL (United States)</creatorcontrib><collection>Medline</collection><collection>MEDLINE</collection><collection>MEDLINE (Ovid)</collection><collection>MEDLINE</collection><collection>MEDLINE</collection><collection>PubMed</collection><collection>CrossRef</collection><collection>MEDLINE - Academic</collection><collection>Biotechnology Research Abstracts</collection><collection>Technology Research Database</collection><collection>Engineering Research Database</collection><collection>Biotechnology and BioEngineering Abstracts</collection><collection>Engineered Materials Abstracts</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>METADEX</collection><collection>Materials Research Database</collection><collection>Advanced Technologies Database with Aerospace</collection><collection>OSTI.GOV - Hybrid</collection><collection>OSTI.GOV</collection><jtitle>Annual review of chemical and biomolecular engineering</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Li, Dongguo</au><au>Lv, Haifeng</au><au>Kang, Yijin</au><au>Markovic, Nenad M</au><au>Stamenkovic, Vojislav R</au><aucorp>Argonne National Laboratory (ANL), Argonne, IL (United States)</aucorp><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Progress in the Development of Oxygen Reduction Reaction Catalysts for Low-Temperature Fuel Cells</atitle><jtitle>Annual review of chemical and biomolecular engineering</jtitle><addtitle>Annu Rev Chem Biomol Eng</addtitle><date>2016-06-07</date><risdate>2016</risdate><volume>7</volume><issue>1</issue><spage>509</spage><epage>532</epage><pages>509-532</pages><issn>1947-5438</issn><eissn>1947-5446</eissn><abstract>We present a brief summary on the most recent progress in the design of catalysts for electrochemical reduction of oxygen. The main challenge in the wide spread of fuel cell technology is to lower the content of, or even eliminate, Pt and other precious metals in catalysts without sacrificing their performance. Pt-based nanosized catalysts with novel and refined architectures continue to dominate in catalytic performance, and formation of Pt-skin-like surfaces is key to achieving the highest values in activity. Moreover, durability has also been improved in Pt-based systems with addition of Au, which plays an important role in stabilizing the Pt topmost layers against dissolution. However, various carbon-based materials without precious metal have shown improvement in activity and durability and have been explored to serve as catalyst supports. Understanding how the doped elements interact with each other and or carbon is challenging and necessary in the design of robust fuel cell catalysts.</abstract><cop>United States</cop><pub>Annual Reviews</pub><pmid>27070766</pmid><doi>10.1146/annurev-chembioeng-080615-034526</doi><tpages>24</tpages><oa>free_for_read</oa></addata></record> |
| fulltext | fulltext |
| identifier | ISSN: 1947-5438 |
| ispartof | Annual review of chemical and biomolecular engineering, 2016-06, Vol.7 (1), p.509-532 |
| issn | 1947-5438 1947-5446 |
| language | eng |
| recordid | cdi_osti_scitechconnect_1352589 |
| source | Annual Reviews Complete A-Z List; MEDLINE |
| subjects | Carbon Carbon - chemistry Catalysis Catalysts Core-shell Design engineering Durability Electrochemical Techniques Electrochemistry Fuel cells INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY MATERIALS SCIENCE Nanoparticle Nanoparticles - chemistry Oxidation-Reduction Oxygen Oxygen - chemistry Platinum Platinum - chemistry Precious metals Temperature Thin films |
| title | Progress in the Development of Oxygen Reduction Reaction Catalysts for Low-Temperature Fuel Cells |
| url | https://sfx.bib-bvb.de/sfx_tum?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2025-01-04T22%3A43%3A11IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-proquest_osti_&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=Progress%20in%20the%20Development%20of%20Oxygen%20Reduction%20Reaction%20Catalysts%20for%20Low-Temperature%20Fuel%20Cells&rft.jtitle=Annual%20review%20of%20chemical%20and%20biomolecular%20engineering&rft.au=Li,%20Dongguo&rft.aucorp=Argonne%20National%20Laboratory%20(ANL),%20Argonne,%20IL%20(United%20States)&rft.date=2016-06-07&rft.volume=7&rft.issue=1&rft.spage=509&rft.epage=532&rft.pages=509-532&rft.issn=1947-5438&rft.eissn=1947-5446&rft_id=info:doi/10.1146/annurev-chembioeng-080615-034526&rft_dat=%3Cproquest_osti_%3E1795878756%3C/proquest_osti_%3E%3Curl%3E%3C/url%3E&disable_directlink=true&sfx.directlink=off&sfx.report_link=0&rft_id=info:oai/&rft_pqid=1795878756&rft_id=info:pmid/27070766&rfr_iscdi=true |