Superconducting order from disorder in 2H-TaSe2−xSx
We report on the emergence of robust superconducting order in single crystal alloys of TaSe 2 − x S x (0 ≤ × ≤ 2). The critical temperature of the alloy is surprisingly higher than that of the two end compounds TaSe 2 and TaS 2 . The evolution of superconducting critical temperature T c ( x ) correl...
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creator | Li, Lijun Deng, Xiaoyu Wang, Zhen Liu, Yu Abeykoon, Milinda Dooryhee, Eric Tomic, Aleksandra Huang, Yanan Warren, John B. Bozin, Emil S. Billinge, Simon J. L. Sun, Yuping Zhu, Yimei Kotliar, Gabriel Petrovic, Cedomir |
description | We report on the emergence of robust superconducting order in single crystal alloys of TaSe
2
−
x
S
x
(0 ≤ × ≤ 2). The critical temperature of the alloy is surprisingly higher than that of the two end compounds TaSe
2
and TaS
2
. The evolution of superconducting critical temperature
T
c
(
x
) correlates with the full width at half maximum of the Bragg peaks and with the linear term of the high-temperature resistivity. The conductivity of the crystals near the middle of the alloy series is higher or similar than that of either one of the end members 2H-TaSe
2
and/or 2H-TaS
2
. It is known that in these materials superconductivity is in close competition with charge density wave order. We interpret our experimental findings in a picture where disorder tilts this balance in favor of superconductivity by destroying the charge density wave order.
Condensed matter physics: crystallographic disorder enhances superconductivity
Substituting sulfur into TaSe
2
induces disorder, which further helps to enhance superconductivity, with a higher transition temperature. It is higher than that of either TaSe
2
or TaS
2
. An international team of researchers led by Cedomir Petrovic at Brookhaven national laboratory of USA synthesized single crystal alloys of TaSe
2
−
x
S
x
and measured the electrical conductivity and superconducting transition temperature as a function of
x
. They found that the transition temperature optimally increased when a maximal disorder is introduced by substituting sulfur into TaSe
2
. The role of such a disorder was understood as to suppress other competing orders while keeping superconductivity intact. By breaking other orders, conducting carriers were released so that they contributed further to superconductivity. These results highlight a benefit role of disorder and provide a possible way to enhance superconductivity. |
doi_str_mv | 10.1038/s41535-017-0016-9 |
format | Article |
fullrecord | <record><control><sourceid>proquest_osti_</sourceid><recordid>TN_cdi_osti_scitechconnect_1351729</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>2389699619</sourcerecordid><originalsourceid>FETCH-LOGICAL-j249t-aa072459390e1f4649a1235be08254ae6660810dd7590ec10197a0edb8ad32c03</originalsourceid><addsrcrecordid>eNpNkM9KAzEQh4MoWLQP4G3Rc3Qm_zY5SlErFDy0nkOapLpFd2uyC30Ezz6iT2LKCnqaGfj48ZuPkAuEawSub7JAySUFrCkAKmqOyIRxU1OhhD7-t5-Sac5bAGCIWig1IXI57GLyXRsG3zftS9WlEFO1Sd17FZo8Xk1bsTlduWVk359f--X-nJxs3FuO0995Rp7v71azOV08PTzObhd0y4TpqXNQMyENNxBxUwoYh4zLdQTNpHBRKQUaIYRaFsIjoKkdxLDWLnDmgZ-RyzG3y31js2_66F9L2Tb63iKXWDNToKsR2qXuY4i5t9tuSG3pZRnXRhmj8ECxkcq7VP6M6Y9CsAeNdtRoi0Z70GgN_wFfLGMI</addsrcrecordid><sourcetype>Open Access Repository</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>2389699619</pqid></control><display><type>article</type><title>Superconducting order from disorder in 2H-TaSe2−xSx</title><source>DOAJ Directory of Open Access Journals</source><source>Springer Nature OA Free Journals</source><source>Nature Free</source><source>EZB-FREE-00999 freely available EZB journals</source><creator>Li, Lijun ; Deng, Xiaoyu ; Wang, Zhen ; Liu, Yu ; Abeykoon, Milinda ; Dooryhee, Eric ; Tomic, Aleksandra ; Huang, Yanan ; Warren, John B. ; Bozin, Emil S. ; Billinge, Simon J. L. ; Sun, Yuping ; Zhu, Yimei ; Kotliar, Gabriel ; Petrovic, Cedomir</creator><creatorcontrib>Li, Lijun ; Deng, Xiaoyu ; Wang, Zhen ; Liu, Yu ; Abeykoon, Milinda ; Dooryhee, Eric ; Tomic, Aleksandra ; Huang, Yanan ; Warren, John B. ; Bozin, Emil S. ; Billinge, Simon J. L. ; Sun, Yuping ; Zhu, Yimei ; Kotliar, Gabriel ; Petrovic, Cedomir ; Brookhaven National Lab. (BNL), Upton, NY (United States)</creatorcontrib><description>We report on the emergence of robust superconducting order in single crystal alloys of TaSe
2
−
x
S
x
(0 ≤ × ≤ 2). The critical temperature of the alloy is surprisingly higher than that of the two end compounds TaSe
2
and TaS
2
. The evolution of superconducting critical temperature
T
c
(
x
) correlates with the full width at half maximum of the Bragg peaks and with the linear term of the high-temperature resistivity. The conductivity of the crystals near the middle of the alloy series is higher or similar than that of either one of the end members 2H-TaSe
2
and/or 2H-TaS
2
. It is known that in these materials superconductivity is in close competition with charge density wave order. We interpret our experimental findings in a picture where disorder tilts this balance in favor of superconductivity by destroying the charge density wave order.
Condensed matter physics: crystallographic disorder enhances superconductivity
Substituting sulfur into TaSe
2
induces disorder, which further helps to enhance superconductivity, with a higher transition temperature. It is higher than that of either TaSe
2
or TaS
2
. An international team of researchers led by Cedomir Petrovic at Brookhaven national laboratory of USA synthesized single crystal alloys of TaSe
2
−
x
S
x
and measured the electrical conductivity and superconducting transition temperature as a function of
x
. They found that the transition temperature optimally increased when a maximal disorder is introduced by substituting sulfur into TaSe
2
. The role of such a disorder was understood as to suppress other competing orders while keeping superconductivity intact. By breaking other orders, conducting carriers were released so that they contributed further to superconductivity. These results highlight a benefit role of disorder and provide a possible way to enhance superconductivity.</description><identifier>ISSN: 2397-4648</identifier><identifier>EISSN: 2397-4648</identifier><identifier>DOI: 10.1038/s41535-017-0016-9</identifier><language>eng</language><publisher>London: Nature Publishing Group UK</publisher><subject>639/301/119/1003 ; 639/766/119/995 ; Alloys ; Charge density waves ; Condensed Matter Physics ; CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY ; Crystallography ; Electrical resistivity ; High temperature ; MATERIALS SCIENCE ; Physics ; Physics and Astronomy ; Quantum Physics ; Single crystals ; Structural Materials ; Sulfur ; Superconductivity ; Surfaces and Interfaces ; Thin Films ; Transition temperature</subject><ispartof>npj quantum materials, 2017-02, Vol.2 (1)</ispartof><rights>The Author(s) 2017</rights><rights>The Author(s) 2017. This work is published under http://creativecommons.org/licenses/by/4.0/ (the “License”). Notwithstanding the ProQuest Terms and Conditions, you may use this content in accordance with the terms of the License.</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><cites>FETCH-LOGICAL-j249t-aa072459390e1f4649a1235be08254ae6660810dd7590ec10197a0edb8ad32c03</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1038/s41535-017-0016-9$$EPDF$$P50$$Gspringer$$Hfree_for_read</linktopdf><linktohtml>$$Uhttps://doi.org/10.1038/s41535-017-0016-9$$EHTML$$P50$$Gspringer$$Hfree_for_read</linktohtml><link.rule.ids>230,315,782,786,866,887,27933,27934,41129,42198,51585</link.rule.ids><backlink>$$Uhttps://www.osti.gov/servlets/purl/1351729$$D View this record in Osti.gov$$Hfree_for_read</backlink></links><search><creatorcontrib>Li, Lijun</creatorcontrib><creatorcontrib>Deng, Xiaoyu</creatorcontrib><creatorcontrib>Wang, Zhen</creatorcontrib><creatorcontrib>Liu, Yu</creatorcontrib><creatorcontrib>Abeykoon, Milinda</creatorcontrib><creatorcontrib>Dooryhee, Eric</creatorcontrib><creatorcontrib>Tomic, Aleksandra</creatorcontrib><creatorcontrib>Huang, Yanan</creatorcontrib><creatorcontrib>Warren, John B.</creatorcontrib><creatorcontrib>Bozin, Emil S.</creatorcontrib><creatorcontrib>Billinge, Simon J. L.</creatorcontrib><creatorcontrib>Sun, Yuping</creatorcontrib><creatorcontrib>Zhu, Yimei</creatorcontrib><creatorcontrib>Kotliar, Gabriel</creatorcontrib><creatorcontrib>Petrovic, Cedomir</creatorcontrib><creatorcontrib>Brookhaven National Lab. (BNL), Upton, NY (United States)</creatorcontrib><title>Superconducting order from disorder in 2H-TaSe2−xSx</title><title>npj quantum materials</title><addtitle>npj Quant Mater</addtitle><description>We report on the emergence of robust superconducting order in single crystal alloys of TaSe
2
−
x
S
x
(0 ≤ × ≤ 2). The critical temperature of the alloy is surprisingly higher than that of the two end compounds TaSe
2
and TaS
2
. The evolution of superconducting critical temperature
T
c
(
x
) correlates with the full width at half maximum of the Bragg peaks and with the linear term of the high-temperature resistivity. The conductivity of the crystals near the middle of the alloy series is higher or similar than that of either one of the end members 2H-TaSe
2
and/or 2H-TaS
2
. It is known that in these materials superconductivity is in close competition with charge density wave order. We interpret our experimental findings in a picture where disorder tilts this balance in favor of superconductivity by destroying the charge density wave order.
Condensed matter physics: crystallographic disorder enhances superconductivity
Substituting sulfur into TaSe
2
induces disorder, which further helps to enhance superconductivity, with a higher transition temperature. It is higher than that of either TaSe
2
or TaS
2
. An international team of researchers led by Cedomir Petrovic at Brookhaven national laboratory of USA synthesized single crystal alloys of TaSe
2
−
x
S
x
and measured the electrical conductivity and superconducting transition temperature as a function of
x
. They found that the transition temperature optimally increased when a maximal disorder is introduced by substituting sulfur into TaSe
2
. The role of such a disorder was understood as to suppress other competing orders while keeping superconductivity intact. By breaking other orders, conducting carriers were released so that they contributed further to superconductivity. These results highlight a benefit role of disorder and provide a possible way to enhance superconductivity.</description><subject>639/301/119/1003</subject><subject>639/766/119/995</subject><subject>Alloys</subject><subject>Charge density waves</subject><subject>Condensed Matter Physics</subject><subject>CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY</subject><subject>Crystallography</subject><subject>Electrical resistivity</subject><subject>High temperature</subject><subject>MATERIALS SCIENCE</subject><subject>Physics</subject><subject>Physics and Astronomy</subject><subject>Quantum Physics</subject><subject>Single crystals</subject><subject>Structural Materials</subject><subject>Sulfur</subject><subject>Superconductivity</subject><subject>Surfaces and Interfaces</subject><subject>Thin Films</subject><subject>Transition temperature</subject><issn>2397-4648</issn><issn>2397-4648</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2017</creationdate><recordtype>article</recordtype><sourceid>C6C</sourceid><sourceid>ABUWG</sourceid><sourceid>AFKRA</sourceid><sourceid>AZQEC</sourceid><sourceid>BENPR</sourceid><sourceid>CCPQU</sourceid><sourceid>DWQXO</sourceid><recordid>eNpNkM9KAzEQh4MoWLQP4G3Rc3Qm_zY5SlErFDy0nkOapLpFd2uyC30Ezz6iT2LKCnqaGfj48ZuPkAuEawSub7JAySUFrCkAKmqOyIRxU1OhhD7-t5-Sac5bAGCIWig1IXI57GLyXRsG3zftS9WlEFO1Sd17FZo8Xk1bsTlduWVk359f--X-nJxs3FuO0995Rp7v71azOV08PTzObhd0y4TpqXNQMyENNxBxUwoYh4zLdQTNpHBRKQUaIYRaFsIjoKkdxLDWLnDmgZ-RyzG3y31js2_66F9L2Tb63iKXWDNToKsR2qXuY4i5t9tuSG3pZRnXRhmj8ECxkcq7VP6M6Y9CsAeNdtRoi0Z70GgN_wFfLGMI</recordid><startdate>20170224</startdate><enddate>20170224</enddate><creator>Li, Lijun</creator><creator>Deng, Xiaoyu</creator><creator>Wang, Zhen</creator><creator>Liu, Yu</creator><creator>Abeykoon, Milinda</creator><creator>Dooryhee, Eric</creator><creator>Tomic, Aleksandra</creator><creator>Huang, Yanan</creator><creator>Warren, John B.</creator><creator>Bozin, Emil S.</creator><creator>Billinge, Simon J. L.</creator><creator>Sun, Yuping</creator><creator>Zhu, Yimei</creator><creator>Kotliar, Gabriel</creator><creator>Petrovic, Cedomir</creator><general>Nature Publishing Group UK</general><general>Nature Publishing Group</general><scope>C6C</scope><scope>8FE</scope><scope>8FG</scope><scope>ABJCF</scope><scope>ABUWG</scope><scope>AFKRA</scope><scope>ARAPS</scope><scope>AZQEC</scope><scope>BENPR</scope><scope>BGLVJ</scope><scope>CCPQU</scope><scope>D1I</scope><scope>DWQXO</scope><scope>HCIFZ</scope><scope>KB.</scope><scope>P5Z</scope><scope>P62</scope><scope>PDBOC</scope><scope>PIMPY</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>PRINS</scope><scope>OIOZB</scope><scope>OTOTI</scope></search><sort><creationdate>20170224</creationdate><title>Superconducting order from disorder in 2H-TaSe2−xSx</title><author>Li, Lijun ; Deng, Xiaoyu ; Wang, Zhen ; Liu, Yu ; Abeykoon, Milinda ; Dooryhee, Eric ; Tomic, Aleksandra ; Huang, Yanan ; Warren, John B. ; Bozin, Emil S. ; Billinge, Simon J. L. ; Sun, Yuping ; Zhu, Yimei ; Kotliar, Gabriel ; Petrovic, Cedomir</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-j249t-aa072459390e1f4649a1235be08254ae6660810dd7590ec10197a0edb8ad32c03</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2017</creationdate><topic>639/301/119/1003</topic><topic>639/766/119/995</topic><topic>Alloys</topic><topic>Charge density waves</topic><topic>Condensed Matter Physics</topic><topic>CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY</topic><topic>Crystallography</topic><topic>Electrical resistivity</topic><topic>High temperature</topic><topic>MATERIALS SCIENCE</topic><topic>Physics</topic><topic>Physics and Astronomy</topic><topic>Quantum Physics</topic><topic>Single crystals</topic><topic>Structural Materials</topic><topic>Sulfur</topic><topic>Superconductivity</topic><topic>Surfaces and Interfaces</topic><topic>Thin Films</topic><topic>Transition temperature</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Li, Lijun</creatorcontrib><creatorcontrib>Deng, Xiaoyu</creatorcontrib><creatorcontrib>Wang, Zhen</creatorcontrib><creatorcontrib>Liu, Yu</creatorcontrib><creatorcontrib>Abeykoon, Milinda</creatorcontrib><creatorcontrib>Dooryhee, Eric</creatorcontrib><creatorcontrib>Tomic, Aleksandra</creatorcontrib><creatorcontrib>Huang, Yanan</creatorcontrib><creatorcontrib>Warren, John B.</creatorcontrib><creatorcontrib>Bozin, Emil S.</creatorcontrib><creatorcontrib>Billinge, Simon J. L.</creatorcontrib><creatorcontrib>Sun, Yuping</creatorcontrib><creatorcontrib>Zhu, Yimei</creatorcontrib><creatorcontrib>Kotliar, Gabriel</creatorcontrib><creatorcontrib>Petrovic, Cedomir</creatorcontrib><creatorcontrib>Brookhaven National Lab. (BNL), Upton, NY (United States)</creatorcontrib><collection>Springer Nature OA Free Journals</collection><collection>ProQuest SciTech Collection</collection><collection>ProQuest Technology Collection</collection><collection>Materials Science & Engineering Collection</collection><collection>ProQuest Central (Alumni Edition)</collection><collection>ProQuest Central UK/Ireland</collection><collection>Advanced Technologies & Aerospace Collection</collection><collection>ProQuest Central Essentials</collection><collection>ProQuest Central</collection><collection>Technology Collection</collection><collection>ProQuest One Community College</collection><collection>ProQuest Materials Science Collection</collection><collection>ProQuest Central Korea</collection><collection>SciTech Premium Collection</collection><collection>Materials Science Database</collection><collection>Advanced Technologies & Aerospace Database</collection><collection>ProQuest Advanced Technologies & Aerospace Collection</collection><collection>Materials Science Collection</collection><collection>Access via ProQuest (Open Access)</collection><collection>ProQuest One Academic Eastern Edition (DO NOT USE)</collection><collection>ProQuest One Academic</collection><collection>ProQuest One Academic UKI Edition</collection><collection>ProQuest Central China</collection><collection>OSTI.GOV - Hybrid</collection><collection>OSTI.GOV</collection><jtitle>npj quantum materials</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Li, Lijun</au><au>Deng, Xiaoyu</au><au>Wang, Zhen</au><au>Liu, Yu</au><au>Abeykoon, Milinda</au><au>Dooryhee, Eric</au><au>Tomic, Aleksandra</au><au>Huang, Yanan</au><au>Warren, John B.</au><au>Bozin, Emil S.</au><au>Billinge, Simon J. L.</au><au>Sun, Yuping</au><au>Zhu, Yimei</au><au>Kotliar, Gabriel</au><au>Petrovic, Cedomir</au><aucorp>Brookhaven National Lab. (BNL), Upton, NY (United States)</aucorp><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Superconducting order from disorder in 2H-TaSe2−xSx</atitle><jtitle>npj quantum materials</jtitle><stitle>npj Quant Mater</stitle><date>2017-02-24</date><risdate>2017</risdate><volume>2</volume><issue>1</issue><issn>2397-4648</issn><eissn>2397-4648</eissn><abstract>We report on the emergence of robust superconducting order in single crystal alloys of TaSe
2
−
x
S
x
(0 ≤ × ≤ 2). The critical temperature of the alloy is surprisingly higher than that of the two end compounds TaSe
2
and TaS
2
. The evolution of superconducting critical temperature
T
c
(
x
) correlates with the full width at half maximum of the Bragg peaks and with the linear term of the high-temperature resistivity. The conductivity of the crystals near the middle of the alloy series is higher or similar than that of either one of the end members 2H-TaSe
2
and/or 2H-TaS
2
. It is known that in these materials superconductivity is in close competition with charge density wave order. We interpret our experimental findings in a picture where disorder tilts this balance in favor of superconductivity by destroying the charge density wave order.
Condensed matter physics: crystallographic disorder enhances superconductivity
Substituting sulfur into TaSe
2
induces disorder, which further helps to enhance superconductivity, with a higher transition temperature. It is higher than that of either TaSe
2
or TaS
2
. An international team of researchers led by Cedomir Petrovic at Brookhaven national laboratory of USA synthesized single crystal alloys of TaSe
2
−
x
S
x
and measured the electrical conductivity and superconducting transition temperature as a function of
x
. They found that the transition temperature optimally increased when a maximal disorder is introduced by substituting sulfur into TaSe
2
. The role of such a disorder was understood as to suppress other competing orders while keeping superconductivity intact. By breaking other orders, conducting carriers were released so that they contributed further to superconductivity. These results highlight a benefit role of disorder and provide a possible way to enhance superconductivity.</abstract><cop>London</cop><pub>Nature Publishing Group UK</pub><doi>10.1038/s41535-017-0016-9</doi><oa>free_for_read</oa></addata></record> |
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subjects | 639/301/119/1003 639/766/119/995 Alloys Charge density waves Condensed Matter Physics CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY Crystallography Electrical resistivity High temperature MATERIALS SCIENCE Physics Physics and Astronomy Quantum Physics Single crystals Structural Materials Sulfur Superconductivity Surfaces and Interfaces Thin Films Transition temperature |
title | Superconducting order from disorder in 2H-TaSe2−xSx |
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