Noble gas migration experiment to support the detection of underground nuclear explosions
A Noble Gas Migration Experiment injected 127 Xe, 37 Ar, and sulfur hexafluoride into a former underground nuclear explosion shot cavity. These tracer gases were allowed to migrate from the cavity to near-surface and surface sampling locations and were detected in soil gas samples collected using va...
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| Veröffentlicht in: | Journal of radioanalytical and nuclear chemistry 2016-03, Vol.307 (3), p.2603-2610 |
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| creator | Olsen, K. B. Kirkham, R. R. Woods, V. T. Haas, D. H. Hayes, J. C. Bowyer, T. W. Mendoza, D. P. Lowrey, J. D. Lukins, C. D. Suarez, R. D. Humble, P. H. Ellefson, M. D. Ripplinger, M. D. Zhong, L. Mitroshkov, A. V. Aalseth, C. E. Prinke, A. M. Mace, E. K. McIntyre, J. I. Stewart, T. L. Mackley, R. D. Milbrath, B. D. Emer, D. F. Biegalski, S. R. |
| description | A Noble Gas Migration Experiment injected
127
Xe,
37
Ar, and sulfur hexafluoride into a former underground nuclear explosion shot cavity. These tracer gases were allowed to migrate from the cavity to near-surface and surface sampling locations and were detected in soil gas samples collected using various on-site inspection sampling approaches. Based on this experiment we came to the following conclusions: (1) SF
6
was enriched in all of the samples relative to both
37
Ar and
127
Xe. (2) There were no significant differences in the
127
Xe to
37
Ar ratio in the samples relative to the ratio injected into the cavity. (3) The migratory behavior of the chemical and radiotracers did not fit typical diffusion modeling scenarios. |
| doi_str_mv | 10.1007/s10967-015-4639-7 |
| format | Article |
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127
Xe,
37
Ar, and sulfur hexafluoride into a former underground nuclear explosion shot cavity. These tracer gases were allowed to migrate from the cavity to near-surface and surface sampling locations and were detected in soil gas samples collected using various on-site inspection sampling approaches. Based on this experiment we came to the following conclusions: (1) SF
6
was enriched in all of the samples relative to both
37
Ar and
127
Xe. (2) There were no significant differences in the
127
Xe to
37
Ar ratio in the samples relative to the ratio injected into the cavity. (3) The migratory behavior of the chemical and radiotracers did not fit typical diffusion modeling scenarios.</description><identifier>ISSN: 0236-5731</identifier><identifier>EISSN: 1588-2780</identifier><identifier>DOI: 10.1007/s10967-015-4639-7</identifier><language>eng</language><publisher>Dordrecht: Springer Netherlands</publisher><subject>Chemistry ; Chemistry and Materials Science ; Diagnostic Radiology ; Explosions ; Hadrons ; Heavy Ions ; Inorganic Chemistry ; Nuclear Chemistry ; Nuclear Physics ; Physical Chemistry ; Sulfur hexafluoride ; Tracers (Biology) ; Underground nuclear explosion, Explosion cavity, On-site inspection, Comprehensive Test-Ban Treaty, Noble gas signatures</subject><ispartof>Journal of radioanalytical and nuclear chemistry, 2016-03, Vol.307 (3), p.2603-2610</ispartof><rights>Akadémiai Kiadó, Budapest, Hungary 2015</rights><rights>COPYRIGHT 2016 Springer</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c354t-6955b2e45edccc316e83a423dbb350a03f9c1768eb9e1db7e3a6cd68bfe5abd43</citedby><cites>FETCH-LOGICAL-c354t-6955b2e45edccc316e83a423dbb350a03f9c1768eb9e1db7e3a6cd68bfe5abd43</cites><orcidid>0000-0002-9992-3045</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s10967-015-4639-7$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s10967-015-4639-7$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>230,314,776,780,881,27901,27902,41464,42533,51294</link.rule.ids><backlink>$$Uhttps://www.osti.gov/biblio/1243200$$D View this record in Osti.gov$$Hfree_for_read</backlink></links><search><creatorcontrib>Olsen, K. B.</creatorcontrib><creatorcontrib>Kirkham, R. R.</creatorcontrib><creatorcontrib>Woods, V. T.</creatorcontrib><creatorcontrib>Haas, D. H.</creatorcontrib><creatorcontrib>Hayes, J. C.</creatorcontrib><creatorcontrib>Bowyer, T. W.</creatorcontrib><creatorcontrib>Mendoza, D. P.</creatorcontrib><creatorcontrib>Lowrey, J. D.</creatorcontrib><creatorcontrib>Lukins, C. D.</creatorcontrib><creatorcontrib>Suarez, R. D.</creatorcontrib><creatorcontrib>Humble, P. H.</creatorcontrib><creatorcontrib>Ellefson, M. D.</creatorcontrib><creatorcontrib>Ripplinger, M. D.</creatorcontrib><creatorcontrib>Zhong, L.</creatorcontrib><creatorcontrib>Mitroshkov, A. V.</creatorcontrib><creatorcontrib>Aalseth, C. E.</creatorcontrib><creatorcontrib>Prinke, A. M.</creatorcontrib><creatorcontrib>Mace, E. K.</creatorcontrib><creatorcontrib>McIntyre, J. I.</creatorcontrib><creatorcontrib>Stewart, T. L.</creatorcontrib><creatorcontrib>Mackley, R. D.</creatorcontrib><creatorcontrib>Milbrath, B. D.</creatorcontrib><creatorcontrib>Emer, D. F.</creatorcontrib><creatorcontrib>Biegalski, S. R.</creatorcontrib><creatorcontrib>Pacific Northwest National Lab. (PNNL), Richland, WA (United States)</creatorcontrib><title>Noble gas migration experiment to support the detection of underground nuclear explosions</title><title>Journal of radioanalytical and nuclear chemistry</title><addtitle>J Radioanal Nucl Chem</addtitle><description>A Noble Gas Migration Experiment injected
127
Xe,
37
Ar, and sulfur hexafluoride into a former underground nuclear explosion shot cavity. These tracer gases were allowed to migrate from the cavity to near-surface and surface sampling locations and were detected in soil gas samples collected using various on-site inspection sampling approaches. Based on this experiment we came to the following conclusions: (1) SF
6
was enriched in all of the samples relative to both
37
Ar and
127
Xe. (2) There were no significant differences in the
127
Xe to
37
Ar ratio in the samples relative to the ratio injected into the cavity. (3) The migratory behavior of the chemical and radiotracers did not fit typical diffusion modeling scenarios.</description><subject>Chemistry</subject><subject>Chemistry and Materials Science</subject><subject>Diagnostic Radiology</subject><subject>Explosions</subject><subject>Hadrons</subject><subject>Heavy Ions</subject><subject>Inorganic Chemistry</subject><subject>Nuclear Chemistry</subject><subject>Nuclear Physics</subject><subject>Physical Chemistry</subject><subject>Sulfur hexafluoride</subject><subject>Tracers (Biology)</subject><subject>Underground nuclear explosion, Explosion cavity, On-site inspection, Comprehensive Test-Ban Treaty, Noble gas signatures</subject><issn>0236-5731</issn><issn>1588-2780</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2016</creationdate><recordtype>article</recordtype><recordid>eNp9kD1PwzAQhi0EEqXwA9gidhc7_krGquJLqmCBgcmynUuaKrUrO5Hg3-MSZuThrNPznO5ehG4pWVFC1H2ipJYKEyowl6zG6gwtqKgqXKqKnKMFKZnEQjF6ia5S2hNC6qpiC_T5GuwARWdScei7aMY--AK-jhD7A_ixGEORpuMxxPzdQdHACO6XCW0x-QZiF0OuhZ_cACae1CGkDKRrdNGaIcHNX12ij8eH980z3r49vWzWW-yY4COWtRC2BC6gcc4xKqFihpessZYJYghra0eVrMDWQBurgBnpGlnZFoSxDWdLdDfPDWnsdXJ93nDngvd5UU1LzkpCMrSaoc4MoHvfhjEal18Dhz7D0Pa5v-ZclLVkVGSBzoKLIaUIrT7mREz81pToU-J6TlznxPUpca2yU85OyqzvIOp9mKLPx_8j_QDvMIXG</recordid><startdate>20160301</startdate><enddate>20160301</enddate><creator>Olsen, K. B.</creator><creator>Kirkham, R. R.</creator><creator>Woods, V. T.</creator><creator>Haas, D. H.</creator><creator>Hayes, J. C.</creator><creator>Bowyer, T. W.</creator><creator>Mendoza, D. P.</creator><creator>Lowrey, J. D.</creator><creator>Lukins, C. D.</creator><creator>Suarez, R. D.</creator><creator>Humble, P. H.</creator><creator>Ellefson, M. D.</creator><creator>Ripplinger, M. D.</creator><creator>Zhong, L.</creator><creator>Mitroshkov, A. V.</creator><creator>Aalseth, C. E.</creator><creator>Prinke, A. M.</creator><creator>Mace, E. K.</creator><creator>McIntyre, J. I.</creator><creator>Stewart, T. L.</creator><creator>Mackley, R. D.</creator><creator>Milbrath, B. D.</creator><creator>Emer, D. F.</creator><creator>Biegalski, S. R.</creator><general>Springer Netherlands</general><general>Springer</general><scope>AAYXX</scope><scope>CITATION</scope><scope>OTOTI</scope><orcidid>https://orcid.org/0000-0002-9992-3045</orcidid></search><sort><creationdate>20160301</creationdate><title>Noble gas migration experiment to support the detection of underground nuclear explosions</title><author>Olsen, K. B. ; Kirkham, R. R. ; Woods, V. T. ; Haas, D. H. ; Hayes, J. C. ; Bowyer, T. W. ; Mendoza, D. P. ; Lowrey, J. D. ; Lukins, C. D. ; Suarez, R. D. ; Humble, P. H. ; Ellefson, M. D. ; Ripplinger, M. D. ; Zhong, L. ; Mitroshkov, A. V. ; Aalseth, C. E. ; Prinke, A. M. ; Mace, E. K. ; McIntyre, J. I. ; Stewart, T. L. ; Mackley, R. D. ; Milbrath, B. D. ; Emer, D. F. ; Biegalski, S. 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R.</creatorcontrib><creatorcontrib>Pacific Northwest National Lab. (PNNL), Richland, WA (United States)</creatorcontrib><collection>CrossRef</collection><collection>OSTI.GOV</collection><jtitle>Journal of radioanalytical and nuclear chemistry</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Olsen, K. B.</au><au>Kirkham, R. R.</au><au>Woods, V. T.</au><au>Haas, D. H.</au><au>Hayes, J. C.</au><au>Bowyer, T. W.</au><au>Mendoza, D. P.</au><au>Lowrey, J. D.</au><au>Lukins, C. D.</au><au>Suarez, R. D.</au><au>Humble, P. H.</au><au>Ellefson, M. D.</au><au>Ripplinger, M. D.</au><au>Zhong, L.</au><au>Mitroshkov, A. V.</au><au>Aalseth, C. E.</au><au>Prinke, A. M.</au><au>Mace, E. K.</au><au>McIntyre, J. I.</au><au>Stewart, T. L.</au><au>Mackley, R. D.</au><au>Milbrath, B. D.</au><au>Emer, D. F.</au><au>Biegalski, S. R.</au><aucorp>Pacific Northwest National Lab. (PNNL), Richland, WA (United States)</aucorp><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Noble gas migration experiment to support the detection of underground nuclear explosions</atitle><jtitle>Journal of radioanalytical and nuclear chemistry</jtitle><stitle>J Radioanal Nucl Chem</stitle><date>2016-03-01</date><risdate>2016</risdate><volume>307</volume><issue>3</issue><spage>2603</spage><epage>2610</epage><pages>2603-2610</pages><issn>0236-5731</issn><eissn>1588-2780</eissn><abstract>A Noble Gas Migration Experiment injected
127
Xe,
37
Ar, and sulfur hexafluoride into a former underground nuclear explosion shot cavity. These tracer gases were allowed to migrate from the cavity to near-surface and surface sampling locations and were detected in soil gas samples collected using various on-site inspection sampling approaches. Based on this experiment we came to the following conclusions: (1) SF
6
was enriched in all of the samples relative to both
37
Ar and
127
Xe. (2) There were no significant differences in the
127
Xe to
37
Ar ratio in the samples relative to the ratio injected into the cavity. (3) The migratory behavior of the chemical and radiotracers did not fit typical diffusion modeling scenarios.</abstract><cop>Dordrecht</cop><pub>Springer Netherlands</pub><doi>10.1007/s10967-015-4639-7</doi><tpages>8</tpages><orcidid>https://orcid.org/0000-0002-9992-3045</orcidid></addata></record> |
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| ispartof | Journal of radioanalytical and nuclear chemistry, 2016-03, Vol.307 (3), p.2603-2610 |
| issn | 0236-5731 1588-2780 |
| language | eng |
| recordid | cdi_osti_scitechconnect_1243200 |
| source | SpringerLink Journals |
| subjects | Chemistry Chemistry and Materials Science Diagnostic Radiology Explosions Hadrons Heavy Ions Inorganic Chemistry Nuclear Chemistry Nuclear Physics Physical Chemistry Sulfur hexafluoride Tracers (Biology) Underground nuclear explosion, Explosion cavity, On-site inspection, Comprehensive Test-Ban Treaty, Noble gas signatures |
| title | Noble gas migration experiment to support the detection of underground nuclear explosions |
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