Quantum process tomography by 2D fluorescence spectroscopy

Reconstruction of the dynamics (quantum process tomography) of the single-exciton manifold in energy transfer systems is proposed here on the basis of two-dimensional fluorescence spectroscopy (2D-FS) with phase-modulation. The quantum-process-tomography protocol introduced here benefits from, e.g.,...

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Bibliographische Detailangaben

Veröffentlicht in:	The Journal of chemical physics 2015-06, Vol.142 (21), p.212442-212442
Hauptverfasser:	Pachón, Leonardo A, Marcus, Andrew H, Aspuru-Guzik, Alán
Format:	Artikel
Sprache:	eng
Schlagworte:	Energy transfer Excitons Fluorescence Parameters Reconstruction Sensitivity enhancement Spectroscopy Spectrum analysis Tomography
Online-Zugang:	Volltext
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