Catching Conical Intersections in the Act: Monitoring Transient Electronic Coherences by Attosecond Stimulated X-Ray Raman Signals

Conical intersections (CIs) dominate the pathways and outcomes of virtually all photophysical and photochemical molecular processes. Despite extensive experimental and theoretical effort, CIs have not been directly observed yet and the experimental evidence is being inferred from fast reaction rates...

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Veröffentlicht in:	Physical review letters 2015-11, Vol.115 (19), p.193003-193003, Article 193003
Hauptverfasser:	Kowalewski, Markus, Bennett, Kochise, Dorfman, Konstantin E, Mukamel, Shaul
Format:	Artikel
Sprache:	eng
Schlagworte:	Coherence Computer Simulation Electronics Femtosecond Intersections Models, Theoretical Monitoring Photochemical Photochemical Processes Photochemistry - methods Spectral sensitivity Spectrum Analysis, Raman - methods X-rays
Online-Zugang:	Volltext
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