Fast Lithium-Ion Conducting Thin-Film Electrolytes Integrated Directly on Flexible Substrates for High-Power Solid-State Batteries

By utilizing an equilibrium processing strategy that enables co‐firing of oxides and base metals, a means to integrate the lithium‐stable fast lithium‐ion conductor lanthanum lithium tantalate directly with a thin copper foil current collector appropriate for a solid‐state battery is presented. This...

Ausführliche Beschreibung

Gespeichert in:
Bibliographische Detailangaben
Veröffentlicht in:Advanced materials (Weinheim) 2011-12, Vol.23 (47), p.5663-5667
Hauptverfasser: Ihlefeld, Jon F., Clem, Paul G., Doyle, Barney L., Kotula, Paul G., Fenton, Kyle R., Apblett, Christopher A.
Format: Artikel
Sprache:eng
Schlagworte:
Online-Zugang:Volltext
Tags: Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
container_end_page 5667
container_issue 47
container_start_page 5663
container_title Advanced materials (Weinheim)
container_volume 23
creator Ihlefeld, Jon F.
Clem, Paul G.
Doyle, Barney L.
Kotula, Paul G.
Fenton, Kyle R.
Apblett, Christopher A.
description By utilizing an equilibrium processing strategy that enables co‐firing of oxides and base metals, a means to integrate the lithium‐stable fast lithium‐ion conductor lanthanum lithium tantalate directly with a thin copper foil current collector appropriate for a solid‐state battery is presented. This resulting thin‐film electrolyte possesses a room temperature lithium‐ion conductivity of 1.5 × 10−5 S cm−1, which has the potential to increase the power of a solid‐state battery over current state of the art.
doi_str_mv 10.1002/adma.201102980
format Article
fullrecord <record><control><sourceid>proquest_osti_</sourceid><recordid>TN_cdi_osti_scitechconnect_1108176</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>911930348</sourcerecordid><originalsourceid>FETCH-LOGICAL-c5160-5aef54071b854da7ae6c4799f878d69ae0765172b433e6d6eaa1502ca3bdbe883</originalsourceid><addsrcrecordid>eNqFkc9v0zAYhi0EYmVw5YgsLpxS7Di242PXLVul8kN0iKPlJF9bgxNvtqOtV_5yUmVU3Dj58D7vI31-EXpLyZwSkn80bWfmOaGU5Kokz9CM8pxmBVH8OZoRxXimRFGeoVcx_iSEKEHES3SW54TLgpEZ-l2ZmPDapr0dumzle7z0fTs0yfY7fLu3fVZZ1-ErB00K3h0SRLzqE-yCSdDiSxvGwB3wWKwcPNraAd4MdUzHPOKtD_jG7vbZV_8AAW-8s222SWOGL0xKECzE1-jF1rgIb57ec_S9urpd3mTrL9er5WKdNZwKknEDW14QSeuSF62RBkRTSKW2pSxboQwQKTiVeV0wBqIVYAzlJG8Mq9saypKdo_eT18dkdWxsgmbf-L4fL9DjB5ZUihH6MEF3wd8PEJPubGzAOdODH6JWlCpGWHHUzSeyCT7GAFt9F2xnwkFToo_b6OM2-rTNWHj3pB7qDtoT_neMEVAT8GAdHP6j04vLT4t_5dnUtTHB46lrwi8tJJNc__h8rWlRKaEuvuk1-wO71Krd</addsrcrecordid><sourcetype>Open Access Repository</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>911930348</pqid></control><display><type>article</type><title>Fast Lithium-Ion Conducting Thin-Film Electrolytes Integrated Directly on Flexible Substrates for High-Power Solid-State Batteries</title><source>MEDLINE</source><source>Wiley Online Library Journals Frontfile Complete</source><creator>Ihlefeld, Jon F. ; Clem, Paul G. ; Doyle, Barney L. ; Kotula, Paul G. ; Fenton, Kyle R. ; Apblett, Christopher A.</creator><creatorcontrib>Ihlefeld, Jon F. ; Clem, Paul G. ; Doyle, Barney L. ; Kotula, Paul G. ; Fenton, Kyle R. ; Apblett, Christopher A. ; Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)</creatorcontrib><description>By utilizing an equilibrium processing strategy that enables co‐firing of oxides and base metals, a means to integrate the lithium‐stable fast lithium‐ion conductor lanthanum lithium tantalate directly with a thin copper foil current collector appropriate for a solid‐state battery is presented. This resulting thin‐film electrolyte possesses a room temperature lithium‐ion conductivity of 1.5 × 10−5 S cm−1, which has the potential to increase the power of a solid‐state battery over current state of the art.</description><identifier>ISSN: 0935-9648</identifier><identifier>EISSN: 1521-4095</identifier><identifier>DOI: 10.1002/adma.201102980</identifier><identifier>PMID: 22057430</identifier><language>eng</language><publisher>Weinheim: WILEY-VCH Verlag</publisher><subject>base metals ; Cations - chemistry ; Electric Conductivity ; Electric Power Supplies ; Electrochemistry ; electrolytes ; Electrolytes - chemistry ; Lithium - chemistry ; lithium-ion batteries ; Nanotechnology - methods ; Oxides - chemistry ; Tantalum - chemistry ; thin films ; X-Ray Diffraction</subject><ispartof>Advanced materials (Weinheim), 2011-12, Vol.23 (47), p.5663-5667</ispartof><rights>Copyright © 2011 WILEY‐VCH Verlag GmbH &amp; Co. KGaA, Weinheim</rights><rights>Copyright © 2011 WILEY-VCH Verlag GmbH &amp; Co. KGaA, Weinheim.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c5160-5aef54071b854da7ae6c4799f878d69ae0765172b433e6d6eaa1502ca3bdbe883</citedby><cites>FETCH-LOGICAL-c5160-5aef54071b854da7ae6c4799f878d69ae0765172b433e6d6eaa1502ca3bdbe883</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://onlinelibrary.wiley.com/doi/pdf/10.1002%2Fadma.201102980$$EPDF$$P50$$Gwiley$$H</linktopdf><linktohtml>$$Uhttps://onlinelibrary.wiley.com/doi/full/10.1002%2Fadma.201102980$$EHTML$$P50$$Gwiley$$H</linktohtml><link.rule.ids>230,314,776,780,881,1411,27903,27904,45553,45554</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/22057430$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink><backlink>$$Uhttps://www.osti.gov/biblio/1108176$$D View this record in Osti.gov$$Hfree_for_read</backlink></links><search><creatorcontrib>Ihlefeld, Jon F.</creatorcontrib><creatorcontrib>Clem, Paul G.</creatorcontrib><creatorcontrib>Doyle, Barney L.</creatorcontrib><creatorcontrib>Kotula, Paul G.</creatorcontrib><creatorcontrib>Fenton, Kyle R.</creatorcontrib><creatorcontrib>Apblett, Christopher A.</creatorcontrib><creatorcontrib>Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)</creatorcontrib><title>Fast Lithium-Ion Conducting Thin-Film Electrolytes Integrated Directly on Flexible Substrates for High-Power Solid-State Batteries</title><title>Advanced materials (Weinheim)</title><addtitle>Adv. Mater</addtitle><description>By utilizing an equilibrium processing strategy that enables co‐firing of oxides and base metals, a means to integrate the lithium‐stable fast lithium‐ion conductor lanthanum lithium tantalate directly with a thin copper foil current collector appropriate for a solid‐state battery is presented. This resulting thin‐film electrolyte possesses a room temperature lithium‐ion conductivity of 1.5 × 10−5 S cm−1, which has the potential to increase the power of a solid‐state battery over current state of the art.</description><subject>base metals</subject><subject>Cations - chemistry</subject><subject>Electric Conductivity</subject><subject>Electric Power Supplies</subject><subject>Electrochemistry</subject><subject>electrolytes</subject><subject>Electrolytes - chemistry</subject><subject>Lithium - chemistry</subject><subject>lithium-ion batteries</subject><subject>Nanotechnology - methods</subject><subject>Oxides - chemistry</subject><subject>Tantalum - chemistry</subject><subject>thin films</subject><subject>X-Ray Diffraction</subject><issn>0935-9648</issn><issn>1521-4095</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2011</creationdate><recordtype>article</recordtype><sourceid>EIF</sourceid><recordid>eNqFkc9v0zAYhi0EYmVw5YgsLpxS7Di242PXLVul8kN0iKPlJF9bgxNvtqOtV_5yUmVU3Dj58D7vI31-EXpLyZwSkn80bWfmOaGU5Kokz9CM8pxmBVH8OZoRxXimRFGeoVcx_iSEKEHES3SW54TLgpEZ-l2ZmPDapr0dumzle7z0fTs0yfY7fLu3fVZZ1-ErB00K3h0SRLzqE-yCSdDiSxvGwB3wWKwcPNraAd4MdUzHPOKtD_jG7vbZV_8AAW-8s222SWOGL0xKECzE1-jF1rgIb57ec_S9urpd3mTrL9er5WKdNZwKknEDW14QSeuSF62RBkRTSKW2pSxboQwQKTiVeV0wBqIVYAzlJG8Mq9saypKdo_eT18dkdWxsgmbf-L4fL9DjB5ZUihH6MEF3wd8PEJPubGzAOdODH6JWlCpGWHHUzSeyCT7GAFt9F2xnwkFToo_b6OM2-rTNWHj3pB7qDtoT_neMEVAT8GAdHP6j04vLT4t_5dnUtTHB46lrwi8tJJNc__h8rWlRKaEuvuk1-wO71Krd</recordid><startdate>20111215</startdate><enddate>20111215</enddate><creator>Ihlefeld, Jon F.</creator><creator>Clem, Paul G.</creator><creator>Doyle, Barney L.</creator><creator>Kotula, Paul G.</creator><creator>Fenton, Kyle R.</creator><creator>Apblett, Christopher A.</creator><general>WILEY-VCH Verlag</general><general>WILEY‐VCH Verlag</general><scope>BSCLL</scope><scope>CGR</scope><scope>CUY</scope><scope>CVF</scope><scope>ECM</scope><scope>EIF</scope><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7X8</scope><scope>OTOTI</scope></search><sort><creationdate>20111215</creationdate><title>Fast Lithium-Ion Conducting Thin-Film Electrolytes Integrated Directly on Flexible Substrates for High-Power Solid-State Batteries</title><author>Ihlefeld, Jon F. ; Clem, Paul G. ; Doyle, Barney L. ; Kotula, Paul G. ; Fenton, Kyle R. ; Apblett, Christopher A.</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c5160-5aef54071b854da7ae6c4799f878d69ae0765172b433e6d6eaa1502ca3bdbe883</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2011</creationdate><topic>base metals</topic><topic>Cations - chemistry</topic><topic>Electric Conductivity</topic><topic>Electric Power Supplies</topic><topic>Electrochemistry</topic><topic>electrolytes</topic><topic>Electrolytes - chemistry</topic><topic>Lithium - chemistry</topic><topic>lithium-ion batteries</topic><topic>Nanotechnology - methods</topic><topic>Oxides - chemistry</topic><topic>Tantalum - chemistry</topic><topic>thin films</topic><topic>X-Ray Diffraction</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Ihlefeld, Jon F.</creatorcontrib><creatorcontrib>Clem, Paul G.</creatorcontrib><creatorcontrib>Doyle, Barney L.</creatorcontrib><creatorcontrib>Kotula, Paul G.</creatorcontrib><creatorcontrib>Fenton, Kyle R.</creatorcontrib><creatorcontrib>Apblett, Christopher A.</creatorcontrib><creatorcontrib>Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)</creatorcontrib><collection>Istex</collection><collection>Medline</collection><collection>MEDLINE</collection><collection>MEDLINE (Ovid)</collection><collection>MEDLINE</collection><collection>MEDLINE</collection><collection>PubMed</collection><collection>CrossRef</collection><collection>MEDLINE - Academic</collection><collection>OSTI.GOV</collection><jtitle>Advanced materials (Weinheim)</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Ihlefeld, Jon F.</au><au>Clem, Paul G.</au><au>Doyle, Barney L.</au><au>Kotula, Paul G.</au><au>Fenton, Kyle R.</au><au>Apblett, Christopher A.</au><aucorp>Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)</aucorp><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Fast Lithium-Ion Conducting Thin-Film Electrolytes Integrated Directly on Flexible Substrates for High-Power Solid-State Batteries</atitle><jtitle>Advanced materials (Weinheim)</jtitle><addtitle>Adv. Mater</addtitle><date>2011-12-15</date><risdate>2011</risdate><volume>23</volume><issue>47</issue><spage>5663</spage><epage>5667</epage><pages>5663-5667</pages><issn>0935-9648</issn><eissn>1521-4095</eissn><abstract>By utilizing an equilibrium processing strategy that enables co‐firing of oxides and base metals, a means to integrate the lithium‐stable fast lithium‐ion conductor lanthanum lithium tantalate directly with a thin copper foil current collector appropriate for a solid‐state battery is presented. This resulting thin‐film electrolyte possesses a room temperature lithium‐ion conductivity of 1.5 × 10−5 S cm−1, which has the potential to increase the power of a solid‐state battery over current state of the art.</abstract><cop>Weinheim</cop><pub>WILEY-VCH Verlag</pub><pmid>22057430</pmid><doi>10.1002/adma.201102980</doi><tpages>5</tpages></addata></record>
fulltext fulltext
identifier ISSN: 0935-9648
ispartof Advanced materials (Weinheim), 2011-12, Vol.23 (47), p.5663-5667
issn 0935-9648
1521-4095
language eng
recordid cdi_osti_scitechconnect_1108176
source MEDLINE; Wiley Online Library Journals Frontfile Complete
subjects base metals
Cations - chemistry
Electric Conductivity
Electric Power Supplies
Electrochemistry
electrolytes
Electrolytes - chemistry
Lithium - chemistry
lithium-ion batteries
Nanotechnology - methods
Oxides - chemistry
Tantalum - chemistry
thin films
X-Ray Diffraction
title Fast Lithium-Ion Conducting Thin-Film Electrolytes Integrated Directly on Flexible Substrates for High-Power Solid-State Batteries
url https://sfx.bib-bvb.de/sfx_tum?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2025-01-21T19%3A04%3A30IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-proquest_osti_&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=Fast%20Lithium-Ion%20Conducting%20Thin-Film%20Electrolytes%20Integrated%20Directly%20on%20Flexible%20Substrates%20for%20High-Power%20Solid-State%20Batteries&rft.jtitle=Advanced%20materials%20(Weinheim)&rft.au=Ihlefeld,%20Jon%20F.&rft.aucorp=Sandia%20National%20Lab.%20(SNL-NM),%20Albuquerque,%20NM%20(United%20States)&rft.date=2011-12-15&rft.volume=23&rft.issue=47&rft.spage=5663&rft.epage=5667&rft.pages=5663-5667&rft.issn=0935-9648&rft.eissn=1521-4095&rft_id=info:doi/10.1002/adma.201102980&rft_dat=%3Cproquest_osti_%3E911930348%3C/proquest_osti_%3E%3Curl%3E%3C/url%3E&disable_directlink=true&sfx.directlink=off&sfx.report_link=0&rft_id=info:oai/&rft_pqid=911930348&rft_id=info:pmid/22057430&rfr_iscdi=true