Generation and propagation of high-order harmonics in crystals
The observation of nonperturbative high-order-harmonic generation in periodic solids has been interpreted in terms of a two step process comprising tunnel ionization and radiation from electrons undergoing frequency modulated Bloch oscillations in a strong laser field [Ghimire et al. Nat. Phys. 7 13...
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Veröffentlicht in: | Physical review. A, Atomic, molecular, and optical physics Atomic, molecular, and optical physics, 2012-04, Vol.85 (4), Article 043836 |
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creator | Ghimire, Shambhu DiChiara, Anthony D. Sistrunk, Emily Ndabashimiye, Georges Szafruga, Urszula B. Mohammad, Anis Agostini, Pierre DiMauro, Louis F. Reis, David A. |
description | The observation of nonperturbative high-order-harmonic generation in periodic solids has been interpreted in terms of a two step process comprising tunnel ionization and radiation from electrons undergoing frequency modulated Bloch oscillations in a strong laser field [Ghimire et al. Nat. Phys. 7 138 (2011)]. Here we extend the model to include propagation effects. We show that the predicted efficiency is limited by phase velocity mismatch for emission below the band gap and by absorption above the band gap. The efficiency of harmonics scales with the square of the carrier density, suggesting that direct seeding could lead to higher yield. The emitted harmonics should have a temporal profile consisting of a train of subcycle pulses with duration on the order of 650 as depending on the crystal thickness. |
doi_str_mv | 10.1103/PhysRevA.85.043836 |
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Nat. Phys. 7 138 (2011)]. Here we extend the model to include propagation effects. We show that the predicted efficiency is limited by phase velocity mismatch for emission below the band gap and by absorption above the band gap. The efficiency of harmonics scales with the square of the carrier density, suggesting that direct seeding could lead to higher yield. The emitted harmonics should have a temporal profile consisting of a train of subcycle pulses with duration on the order of 650 as depending on the crystal thickness.</description><identifier>ISSN: 1050-2947</identifier><identifier>EISSN: 1094-1622</identifier><identifier>DOI: 10.1103/PhysRevA.85.043836</identifier><language>eng</language><publisher>United States: American Physical Society</publisher><subject>Crystals ; Harmonics ; Lasers ; Mathematical models ; Nucleation ; Oscillations ; Phase velocity ; Trains</subject><ispartof>Physical review. 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The emitted harmonics should have a temporal profile consisting of a train of subcycle pulses with duration on the order of 650 as depending on the crystal thickness.</description><subject>Crystals</subject><subject>Harmonics</subject><subject>Lasers</subject><subject>Mathematical models</subject><subject>Nucleation</subject><subject>Oscillations</subject><subject>Phase velocity</subject><subject>Trains</subject><issn>1050-2947</issn><issn>1094-1622</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2012</creationdate><recordtype>article</recordtype><recordid>eNo1kEFLAzEQhYMoWKt_wNPiycvWZLObTS5CKVqFgiJ6DtnZ2W6kTWqyFfrvm7I6lzcPPoZ5j5BbRmeMUf7w3h_iB_7OZ7Ka0ZJLLs7IhFFV5kwUxflpr2heqLK-JFcxftM0pVQT8rhEh8EM1rvMuDbbBb8z69H7Luvtus99aDFkvQlb7yzEzLoMwiEOZhOvyUWXBG_-dEq-np8-Fy_56m35upivciiFGHKRnmgQuOEckbVCtFXTFNBJyqGpCtZSptqyBiYNbTpeK9XUCgCxNZUpG86n5G686-NgdQQ7IPTgnUMYdMopa1El6H6EUoifPcZBb20E3GyMQ7-PieOMUymVTGgxohB8jAE7vQt2a8IhQfrUqP5vVMtKj43yI9DFa4I</recordid><startdate>20120420</startdate><enddate>20120420</enddate><creator>Ghimire, Shambhu</creator><creator>DiChiara, Anthony D.</creator><creator>Sistrunk, Emily</creator><creator>Ndabashimiye, Georges</creator><creator>Szafruga, Urszula B.</creator><creator>Mohammad, Anis</creator><creator>Agostini, Pierre</creator><creator>DiMauro, Louis F.</creator><creator>Reis, David A.</creator><general>American Physical Society</general><scope>AAYXX</scope><scope>CITATION</scope><scope>7U5</scope><scope>8FD</scope><scope>H8D</scope><scope>L7M</scope><scope>OTOTI</scope></search><sort><creationdate>20120420</creationdate><title>Generation and propagation of high-order harmonics in crystals</title><author>Ghimire, Shambhu ; DiChiara, Anthony D. ; Sistrunk, Emily ; Ndabashimiye, Georges ; Szafruga, Urszula B. ; Mohammad, Anis ; Agostini, Pierre ; DiMauro, Louis F. ; Reis, David A.</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c466t-6622bec3a33ee1d66d5bb2cf803cb521d019d47c18a0bf3799b79cceeda5a4b33</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2012</creationdate><topic>Crystals</topic><topic>Harmonics</topic><topic>Lasers</topic><topic>Mathematical models</topic><topic>Nucleation</topic><topic>Oscillations</topic><topic>Phase velocity</topic><topic>Trains</topic><toplevel>online_resources</toplevel><creatorcontrib>Ghimire, Shambhu</creatorcontrib><creatorcontrib>DiChiara, Anthony D.</creatorcontrib><creatorcontrib>Sistrunk, Emily</creatorcontrib><creatorcontrib>Ndabashimiye, Georges</creatorcontrib><creatorcontrib>Szafruga, Urszula B.</creatorcontrib><creatorcontrib>Mohammad, Anis</creatorcontrib><creatorcontrib>Agostini, Pierre</creatorcontrib><creatorcontrib>DiMauro, Louis F.</creatorcontrib><creatorcontrib>Reis, David A.</creatorcontrib><collection>CrossRef</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>Technology Research Database</collection><collection>Aerospace Database</collection><collection>Advanced Technologies Database with Aerospace</collection><collection>OSTI.GOV</collection><jtitle>Physical review. 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subjects | Crystals Harmonics Lasers Mathematical models Nucleation Oscillations Phase velocity Trains |
title | Generation and propagation of high-order harmonics in crystals |
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