Direct conversion of syngas into aromatics over a bifunctional catalyst: inhibiting net CO2 release
Tandem catalysis via methanol intermediate is a promising route for the direct conversion of syngas into aromatics. However, the simultaneous formation of CO2 is a serious problem. Here, we demonstrate that CO2 was formed by the water-gas shift (WGS) reaction (CO + H2O → CO2 + H2) over a ZnO-ZrO2/H-...
Gespeichert in:
| Veröffentlicht in: | CHEMICAL COMMUNICATIONS 2020-05, Vol.56 (39), p.5239-5242 |
|---|---|
| Hauptverfasser: | , , , , , , , , , , , |
| Format: | Artikel |
| Sprache: | eng |
| Online-Zugang: | Volltext |
| Tags: |
Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
|
| container_end_page | 5242 |
|---|---|
| container_issue | 39 |
| container_start_page | 5239 |
| container_title | CHEMICAL COMMUNICATIONS |
| container_volume | 56 |
| creator | Zhou, Wei Zhou, Cheng Yin, Haoren Shi, Jiaqing Zhang, Guoquan Zheng, Xinlei Min, Xiaojian Zhang, Zhiqiang Cheng, Kang Kang, Jincan Zhang, Qinghong Wang, Ye |
| description | Tandem catalysis via methanol intermediate is a promising route for the direct conversion of syngas into aromatics. However, the simultaneous formation of CO2 is a serious problem. Here, we demonstrate that CO2 was formed by the water-gas shift (WGS) reaction (CO + H2O → CO2 + H2) over a ZnO-ZrO2/H-ZSM-5 catalyst, and the net CO2 formation could be inhibited without affecting the formation of aromatics by co-feeding CO2. |
| format | Article |
| fullrecord | <record><control><sourceid>kuleuven</sourceid><recordid>TN_cdi_kuleuven_dspace_20_500_12942_702723</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>20_500_12942_702723</sourcerecordid><originalsourceid>FETCH-kuleuven_dspace_20_500_12942_7027233</originalsourceid><addsrcrecordid>eNqVyrFOwzAQgGEPILUF3uHmSqkcu1Fo10DFxsJuXcyluLh2lbtE5O2bgQdo_-Vfvge1LG21K2q7rRZqxXzSc2X1ulT-LfTkBXxOI_UccoLcAU_piAwhSQbs8xkleIY8C0BoQzckLzPFCB4F48Syn_FPaIOEdIREAs2ngZ4iIdOzeuwwMr38_0mtD-9fzUfxO0QaRkrumy_oyRntKq1daXZb42ptamPtnXhzM3byJ_YKbplWsA</addsrcrecordid><sourcetype>Institutional Repository</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype></control><display><type>article</type><title>Direct conversion of syngas into aromatics over a bifunctional catalyst: inhibiting net CO2 release</title><source>Lirias (KU Leuven Association)</source><source>Royal Society Of Chemistry Journals 2008-</source><source>Alma/SFX Local Collection</source><creator>Zhou, Wei ; Zhou, Cheng ; Yin, Haoren ; Shi, Jiaqing ; Zhang, Guoquan ; Zheng, Xinlei ; Min, Xiaojian ; Zhang, Zhiqiang ; Cheng, Kang ; Kang, Jincan ; Zhang, Qinghong ; Wang, Ye</creator><creatorcontrib>Zhou, Wei ; Zhou, Cheng ; Yin, Haoren ; Shi, Jiaqing ; Zhang, Guoquan ; Zheng, Xinlei ; Min, Xiaojian ; Zhang, Zhiqiang ; Cheng, Kang ; Kang, Jincan ; Zhang, Qinghong ; Wang, Ye</creatorcontrib><description>Tandem catalysis via methanol intermediate is a promising route for the direct conversion of syngas into aromatics. However, the simultaneous formation of CO2 is a serious problem. Here, we demonstrate that CO2 was formed by the water-gas shift (WGS) reaction (CO + H2O → CO2 + H2) over a ZnO-ZrO2/H-ZSM-5 catalyst, and the net CO2 formation could be inhibited without affecting the formation of aromatics by co-feeding CO2.</description><identifier>ISSN: 1359-7345</identifier><language>eng</language><publisher>ROYAL SOC CHEMISTRY</publisher><ispartof>CHEMICAL COMMUNICATIONS, 2020-05, Vol.56 (39), p.5239-5242</ispartof><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,315,776,780,27839</link.rule.ids></links><search><creatorcontrib>Zhou, Wei</creatorcontrib><creatorcontrib>Zhou, Cheng</creatorcontrib><creatorcontrib>Yin, Haoren</creatorcontrib><creatorcontrib>Shi, Jiaqing</creatorcontrib><creatorcontrib>Zhang, Guoquan</creatorcontrib><creatorcontrib>Zheng, Xinlei</creatorcontrib><creatorcontrib>Min, Xiaojian</creatorcontrib><creatorcontrib>Zhang, Zhiqiang</creatorcontrib><creatorcontrib>Cheng, Kang</creatorcontrib><creatorcontrib>Kang, Jincan</creatorcontrib><creatorcontrib>Zhang, Qinghong</creatorcontrib><creatorcontrib>Wang, Ye</creatorcontrib><title>Direct conversion of syngas into aromatics over a bifunctional catalyst: inhibiting net CO2 release</title><title>CHEMICAL COMMUNICATIONS</title><description>Tandem catalysis via methanol intermediate is a promising route for the direct conversion of syngas into aromatics. However, the simultaneous formation of CO2 is a serious problem. Here, we demonstrate that CO2 was formed by the water-gas shift (WGS) reaction (CO + H2O → CO2 + H2) over a ZnO-ZrO2/H-ZSM-5 catalyst, and the net CO2 formation could be inhibited without affecting the formation of aromatics by co-feeding CO2.</description><issn>1359-7345</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2020</creationdate><recordtype>article</recordtype><sourceid>FZOIL</sourceid><recordid>eNqVyrFOwzAQgGEPILUF3uHmSqkcu1Fo10DFxsJuXcyluLh2lbtE5O2bgQdo_-Vfvge1LG21K2q7rRZqxXzSc2X1ulT-LfTkBXxOI_UccoLcAU_piAwhSQbs8xkleIY8C0BoQzckLzPFCB4F48Syn_FPaIOEdIREAs2ngZ4iIdOzeuwwMr38_0mtD-9fzUfxO0QaRkrumy_oyRntKq1daXZb42ptamPtnXhzM3byJ_YKbplWsA</recordid><startdate>20200514</startdate><enddate>20200514</enddate><creator>Zhou, Wei</creator><creator>Zhou, Cheng</creator><creator>Yin, Haoren</creator><creator>Shi, Jiaqing</creator><creator>Zhang, Guoquan</creator><creator>Zheng, Xinlei</creator><creator>Min, Xiaojian</creator><creator>Zhang, Zhiqiang</creator><creator>Cheng, Kang</creator><creator>Kang, Jincan</creator><creator>Zhang, Qinghong</creator><creator>Wang, Ye</creator><general>ROYAL SOC CHEMISTRY</general><scope>FZOIL</scope></search><sort><creationdate>20200514</creationdate><title>Direct conversion of syngas into aromatics over a bifunctional catalyst: inhibiting net CO2 release</title><author>Zhou, Wei ; Zhou, Cheng ; Yin, Haoren ; Shi, Jiaqing ; Zhang, Guoquan ; Zheng, Xinlei ; Min, Xiaojian ; Zhang, Zhiqiang ; Cheng, Kang ; Kang, Jincan ; Zhang, Qinghong ; Wang, Ye</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-kuleuven_dspace_20_500_12942_7027233</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2020</creationdate><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Zhou, Wei</creatorcontrib><creatorcontrib>Zhou, Cheng</creatorcontrib><creatorcontrib>Yin, Haoren</creatorcontrib><creatorcontrib>Shi, Jiaqing</creatorcontrib><creatorcontrib>Zhang, Guoquan</creatorcontrib><creatorcontrib>Zheng, Xinlei</creatorcontrib><creatorcontrib>Min, Xiaojian</creatorcontrib><creatorcontrib>Zhang, Zhiqiang</creatorcontrib><creatorcontrib>Cheng, Kang</creatorcontrib><creatorcontrib>Kang, Jincan</creatorcontrib><creatorcontrib>Zhang, Qinghong</creatorcontrib><creatorcontrib>Wang, Ye</creatorcontrib><collection>Lirias (KU Leuven Association)</collection><jtitle>CHEMICAL COMMUNICATIONS</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Zhou, Wei</au><au>Zhou, Cheng</au><au>Yin, Haoren</au><au>Shi, Jiaqing</au><au>Zhang, Guoquan</au><au>Zheng, Xinlei</au><au>Min, Xiaojian</au><au>Zhang, Zhiqiang</au><au>Cheng, Kang</au><au>Kang, Jincan</au><au>Zhang, Qinghong</au><au>Wang, Ye</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Direct conversion of syngas into aromatics over a bifunctional catalyst: inhibiting net CO2 release</atitle><jtitle>CHEMICAL COMMUNICATIONS</jtitle><date>2020-05-14</date><risdate>2020</risdate><volume>56</volume><issue>39</issue><spage>5239</spage><epage>5242</epage><pages>5239-5242</pages><issn>1359-7345</issn><abstract>Tandem catalysis via methanol intermediate is a promising route for the direct conversion of syngas into aromatics. However, the simultaneous formation of CO2 is a serious problem. Here, we demonstrate that CO2 was formed by the water-gas shift (WGS) reaction (CO + H2O → CO2 + H2) over a ZnO-ZrO2/H-ZSM-5 catalyst, and the net CO2 formation could be inhibited without affecting the formation of aromatics by co-feeding CO2.</abstract><pub>ROYAL SOC CHEMISTRY</pub></addata></record> |
| fulltext | fulltext |
| identifier | ISSN: 1359-7345 |
| ispartof | CHEMICAL COMMUNICATIONS, 2020-05, Vol.56 (39), p.5239-5242 |
| issn | 1359-7345 |
| language | eng |
| recordid | cdi_kuleuven_dspace_20_500_12942_702723 |
| source | Lirias (KU Leuven Association); Royal Society Of Chemistry Journals 2008-; Alma/SFX Local Collection |
| title | Direct conversion of syngas into aromatics over a bifunctional catalyst: inhibiting net CO2 release |
| url | https://sfx.bib-bvb.de/sfx_tum?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2025-01-27T02%3A55%3A54IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-kuleuven&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=Direct%20conversion%20of%20syngas%20into%20aromatics%20over%20a%20bifunctional%20catalyst:%20inhibiting%20net%20CO2%20release&rft.jtitle=CHEMICAL%20COMMUNICATIONS&rft.au=Zhou,%20Wei&rft.date=2020-05-14&rft.volume=56&rft.issue=39&rft.spage=5239&rft.epage=5242&rft.pages=5239-5242&rft.issn=1359-7345&rft_id=info:doi/&rft_dat=%3Ckuleuven%3E20_500_12942_702723%3C/kuleuven%3E%3Curl%3E%3C/url%3E&disable_directlink=true&sfx.directlink=off&sfx.report_link=0&rft_id=info:oai/&rft_id=info:pmid/&rfr_iscdi=true |