Third harmonic generation at the charge transfer gap in Sr/sub 2/CuO/sub 2/Cl/sub 2

Summary form only given. Progress towards understanding high transition-temperature superconductivity in the copper oxides (cuprates) is hindered by the coexistence of complex spin, charge and lattice degrees of freedom. Even in the undoped parent compounds a detailed microscopic description of exci...

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Hauptverfasser: Carnahan, M.A., Schumacher, A.B., Dodge, J.S., Kaindl, R.A., Chemla, D.S.
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Schumacher, A.B.
Dodge, J.S.
Kaindl, R.A.
Chemla, D.S.
description Summary form only given. Progress towards understanding high transition-temperature superconductivity in the copper oxides (cuprates) is hindered by the coexistence of complex spin, charge and lattice degrees of freedom. Even in the undoped parent compounds a detailed microscopic description of excitations within the basic energy bandstructure as observed in electron and optical spectroscopies remains a formidable task. Nonlinear optical spectroscopy, however, allows precise control over excitation energies and symmetries, revealing important new information about such systems. Here, we employ third-harmonic generation (THG) spectroscopy to investigate the electronic structure around the charge-transfer gap in the strongly correlated cuprate Sr/sub 2/CuO/sub 2/Cl/sub 2/.
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source IEEE Electronic Library (IEL) Conference Proceedings
subjects Charge transfer
Copper
Electron optics
Frequency conversion
Nonlinear optics
Optical harmonic generation
Optical microscopy
Spectroscopy
Strontium
Superconductivity
title Third harmonic generation at the charge transfer gap in Sr/sub 2/CuO/sub 2/Cl/sub 2
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