A study of the vertical scale of halogen chemistry in the Arctic troposphere during Polar Sunrise at Barrow, Alaska
The vertical extent and impact of halogen chemistry in the Arctic springtime was investigated through balloon‐based measurement of several atmospheric chemical components. Various chemical species, including volatile organic compounds (VOCs), ozone, and elemental mercury, that are modified by haloge...
Gespeichert in:
| Veröffentlicht in: | Journal of Geophysical Research. D. Atmospheres 2007-04, Vol.112 (D7), p.n/a |
|---|---|
| Hauptverfasser: | , , , , , , , , |
| Format: | Artikel |
| Sprache: | eng |
| Schlagworte: | |
| Online-Zugang: | Volltext |
| Tags: |
Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
|
| container_end_page | n/a |
|---|---|
| container_issue | D7 |
| container_start_page | |
| container_title | Journal of Geophysical Research. D. Atmospheres |
| container_volume | 112 |
| creator | Tackett, Philip J. Cavender, Aubrey E. Keil, Adam D. Shepson, Paul B. Bottenheim, Jan W. Morin, Samuel Deary, John Steffen, Alexandra Doerge, Chris |
| description | The vertical extent and impact of halogen chemistry in the Arctic springtime was investigated through balloon‐based measurement of several atmospheric chemical components. Various chemical species, including volatile organic compounds (VOCs), ozone, and elemental mercury, that are modified by halogen chemistry were measured from the surface to ∼300 m during late March through mid‐April 2005 in Barrow, Alaska. It is observed that the halogen chemistry appears to be most active in the lowest 100–200 m of the atmosphere. The Hg vertical concentration profiles are consistent with destruction by chemistry that evolves from a species emitted from the snowpack, most likely Br2 and BrCl, and the VOC profiles also demonstrate the limited vertical scale of halogen‐initiated chemistry taking place above the Arctic snowpack. |
| doi_str_mv | 10.1029/2006JD007785 |
| format | Article |
| fullrecord | <record><control><sourceid>proquest_hal_p</sourceid><recordid>TN_cdi_hal_primary_oai_HAL_insu_00377484v1</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>19775448</sourcerecordid><originalsourceid>FETCH-LOGICAL-c4512-350fd5f5947f9d504d4b0c0d3a30a5a10a62d191452961b9a5c144b6e7dde39d3</originalsourceid><addsrcrecordid>eNp9kU9v1DAQxSMEEqu2Nz6AL3BADR3_i5Nj2MK21aotpcDRmo2drmkaL3bSdr89XlIVTsxhRhr93pNmXpa9ofCBAquOGEBxdgygVClfZDNGZZEzBuxlNgMqyhwYU6-zgxh_QiohCwF0lsWaxGE0W-JbMqwtubdhcA12JKZmd9s1dv7G9qRZ2zsXh7Alrv-D1qFJKBmC3_i4WdtgiRmD62_Ipe8wkK9jH1y0BAfyEUPwD4ek7jDe4n72qsUu2oOnuZd9-_zpen6SLy8Wp_N6mTdCUpZzCa2RrayEaisjQRixggYMRw4okQIWzNCKCsmqgq4qlA0VYlVYZYzlleF72fvJN52gN8HdYdhqj06f1Evt-jhqAK6UKMU9TfC7Cd4E_2u0cdDp2sZ2HfbWj1HTSikpRJnAwwlsgo8x2PbZmoLeJaH_TSLhb598cffSNmDfuPhXU6pCcgGJ4xP34Dq7_a-nPltcHVPOS5ZU-aRKydjHZxWGW10orqT-cb7QV_y8WF7Pv-jv_Dc80aTu</addsrcrecordid><sourcetype>Open Access Repository</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>19775448</pqid></control><display><type>article</type><title>A study of the vertical scale of halogen chemistry in the Arctic troposphere during Polar Sunrise at Barrow, Alaska</title><source>Wiley Online Library AGU Free Content</source><source>Access via Wiley Online Library</source><source>Wiley Online Library (Open Access Collection)</source><source>Alma/SFX Local Collection</source><creator>Tackett, Philip J. ; Cavender, Aubrey E. ; Keil, Adam D. ; Shepson, Paul B. ; Bottenheim, Jan W. ; Morin, Samuel ; Deary, John ; Steffen, Alexandra ; Doerge, Chris</creator><creatorcontrib>Tackett, Philip J. ; Cavender, Aubrey E. ; Keil, Adam D. ; Shepson, Paul B. ; Bottenheim, Jan W. ; Morin, Samuel ; Deary, John ; Steffen, Alexandra ; Doerge, Chris</creatorcontrib><description>The vertical extent and impact of halogen chemistry in the Arctic springtime was investigated through balloon‐based measurement of several atmospheric chemical components. Various chemical species, including volatile organic compounds (VOCs), ozone, and elemental mercury, that are modified by halogen chemistry were measured from the surface to ∼300 m during late March through mid‐April 2005 in Barrow, Alaska. It is observed that the halogen chemistry appears to be most active in the lowest 100–200 m of the atmosphere. The Hg vertical concentration profiles are consistent with destruction by chemistry that evolves from a species emitted from the snowpack, most likely Br2 and BrCl, and the VOC profiles also demonstrate the limited vertical scale of halogen‐initiated chemistry taking place above the Arctic snowpack.</description><identifier>ISSN: 0148-0227</identifier><identifier>ISSN: 2169-897X</identifier><identifier>EISSN: 2156-2202</identifier><identifier>EISSN: 2169-8996</identifier><identifier>DOI: 10.1029/2006JD007785</identifier><language>eng</language><publisher>Washington, DC: Blackwell Publishing Ltd</publisher><subject>Arctic ; Earth Sciences ; Earth, ocean, space ; Exact sciences and technology ; Glaciology ; halogen chemistry ; Sciences of the Universe ; vertical profiles</subject><ispartof>Journal of Geophysical Research. D. Atmospheres, 2007-04, Vol.112 (D7), p.n/a</ispartof><rights>Copyright 2007 by the American Geophysical Union.</rights><rights>2007 INIST-CNRS</rights><rights>Distributed under a Creative Commons Attribution 4.0 International License</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c4512-350fd5f5947f9d504d4b0c0d3a30a5a10a62d191452961b9a5c144b6e7dde39d3</citedby><cites>FETCH-LOGICAL-c4512-350fd5f5947f9d504d4b0c0d3a30a5a10a62d191452961b9a5c144b6e7dde39d3</cites><orcidid>0000-0002-1781-687X</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://onlinelibrary.wiley.com/doi/pdf/10.1029%2F2006JD007785$$EPDF$$P50$$Gwiley$$H</linktopdf><linktohtml>$$Uhttps://onlinelibrary.wiley.com/doi/full/10.1029%2F2006JD007785$$EHTML$$P50$$Gwiley$$H</linktohtml><link.rule.ids>230,314,780,784,885,1417,1433,11514,27924,27925,45574,45575,46409,46468,46833,46892</link.rule.ids><backlink>$$Uhttp://pascal-francis.inist.fr/vibad/index.php?action=getRecordDetail&idt=18765340$$DView record in Pascal Francis$$Hfree_for_read</backlink><backlink>$$Uhttps://insu.hal.science/insu-00377484$$DView record in HAL$$Hfree_for_read</backlink></links><search><creatorcontrib>Tackett, Philip J.</creatorcontrib><creatorcontrib>Cavender, Aubrey E.</creatorcontrib><creatorcontrib>Keil, Adam D.</creatorcontrib><creatorcontrib>Shepson, Paul B.</creatorcontrib><creatorcontrib>Bottenheim, Jan W.</creatorcontrib><creatorcontrib>Morin, Samuel</creatorcontrib><creatorcontrib>Deary, John</creatorcontrib><creatorcontrib>Steffen, Alexandra</creatorcontrib><creatorcontrib>Doerge, Chris</creatorcontrib><title>A study of the vertical scale of halogen chemistry in the Arctic troposphere during Polar Sunrise at Barrow, Alaska</title><title>Journal of Geophysical Research. D. Atmospheres</title><addtitle>J. Geophys. Res</addtitle><description>The vertical extent and impact of halogen chemistry in the Arctic springtime was investigated through balloon‐based measurement of several atmospheric chemical components. Various chemical species, including volatile organic compounds (VOCs), ozone, and elemental mercury, that are modified by halogen chemistry were measured from the surface to ∼300 m during late March through mid‐April 2005 in Barrow, Alaska. It is observed that the halogen chemistry appears to be most active in the lowest 100–200 m of the atmosphere. The Hg vertical concentration profiles are consistent with destruction by chemistry that evolves from a species emitted from the snowpack, most likely Br2 and BrCl, and the VOC profiles also demonstrate the limited vertical scale of halogen‐initiated chemistry taking place above the Arctic snowpack.</description><subject>Arctic</subject><subject>Earth Sciences</subject><subject>Earth, ocean, space</subject><subject>Exact sciences and technology</subject><subject>Glaciology</subject><subject>halogen chemistry</subject><subject>Sciences of the Universe</subject><subject>vertical profiles</subject><issn>0148-0227</issn><issn>2169-897X</issn><issn>2156-2202</issn><issn>2169-8996</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2007</creationdate><recordtype>article</recordtype><recordid>eNp9kU9v1DAQxSMEEqu2Nz6AL3BADR3_i5Nj2MK21aotpcDRmo2drmkaL3bSdr89XlIVTsxhRhr93pNmXpa9ofCBAquOGEBxdgygVClfZDNGZZEzBuxlNgMqyhwYU6-zgxh_QiohCwF0lsWaxGE0W-JbMqwtubdhcA12JKZmd9s1dv7G9qRZ2zsXh7Alrv-D1qFJKBmC3_i4WdtgiRmD62_Ipe8wkK9jH1y0BAfyEUPwD4ek7jDe4n72qsUu2oOnuZd9-_zpen6SLy8Wp_N6mTdCUpZzCa2RrayEaisjQRixggYMRw4okQIWzNCKCsmqgq4qlA0VYlVYZYzlleF72fvJN52gN8HdYdhqj06f1Evt-jhqAK6UKMU9TfC7Cd4E_2u0cdDp2sZ2HfbWj1HTSikpRJnAwwlsgo8x2PbZmoLeJaH_TSLhb598cffSNmDfuPhXU6pCcgGJ4xP34Dq7_a-nPltcHVPOS5ZU-aRKydjHZxWGW10orqT-cb7QV_y8WF7Pv-jv_Dc80aTu</recordid><startdate>20070416</startdate><enddate>20070416</enddate><creator>Tackett, Philip J.</creator><creator>Cavender, Aubrey E.</creator><creator>Keil, Adam D.</creator><creator>Shepson, Paul B.</creator><creator>Bottenheim, Jan W.</creator><creator>Morin, Samuel</creator><creator>Deary, John</creator><creator>Steffen, Alexandra</creator><creator>Doerge, Chris</creator><general>Blackwell Publishing Ltd</general><general>American Geophysical Union</general><scope>BSCLL</scope><scope>IQODW</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7TG</scope><scope>F1W</scope><scope>H96</scope><scope>KL.</scope><scope>L.G</scope><scope>1XC</scope><scope>VOOES</scope><orcidid>https://orcid.org/0000-0002-1781-687X</orcidid></search><sort><creationdate>20070416</creationdate><title>A study of the vertical scale of halogen chemistry in the Arctic troposphere during Polar Sunrise at Barrow, Alaska</title><author>Tackett, Philip J. ; Cavender, Aubrey E. ; Keil, Adam D. ; Shepson, Paul B. ; Bottenheim, Jan W. ; Morin, Samuel ; Deary, John ; Steffen, Alexandra ; Doerge, Chris</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c4512-350fd5f5947f9d504d4b0c0d3a30a5a10a62d191452961b9a5c144b6e7dde39d3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2007</creationdate><topic>Arctic</topic><topic>Earth Sciences</topic><topic>Earth, ocean, space</topic><topic>Exact sciences and technology</topic><topic>Glaciology</topic><topic>halogen chemistry</topic><topic>Sciences of the Universe</topic><topic>vertical profiles</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Tackett, Philip J.</creatorcontrib><creatorcontrib>Cavender, Aubrey E.</creatorcontrib><creatorcontrib>Keil, Adam D.</creatorcontrib><creatorcontrib>Shepson, Paul B.</creatorcontrib><creatorcontrib>Bottenheim, Jan W.</creatorcontrib><creatorcontrib>Morin, Samuel</creatorcontrib><creatorcontrib>Deary, John</creatorcontrib><creatorcontrib>Steffen, Alexandra</creatorcontrib><creatorcontrib>Doerge, Chris</creatorcontrib><collection>Istex</collection><collection>Pascal-Francis</collection><collection>CrossRef</collection><collection>Meteorological & Geoastrophysical Abstracts</collection><collection>ASFA: Aquatic Sciences and Fisheries Abstracts</collection><collection>Aquatic Science & Fisheries Abstracts (ASFA) 2: Ocean Technology, Policy & Non-Living Resources</collection><collection>Meteorological & Geoastrophysical Abstracts - Academic</collection><collection>Aquatic Science & Fisheries Abstracts (ASFA) Professional</collection><collection>Hyper Article en Ligne (HAL)</collection><collection>Hyper Article en Ligne (HAL) (Open Access)</collection><jtitle>Journal of Geophysical Research. D. Atmospheres</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Tackett, Philip J.</au><au>Cavender, Aubrey E.</au><au>Keil, Adam D.</au><au>Shepson, Paul B.</au><au>Bottenheim, Jan W.</au><au>Morin, Samuel</au><au>Deary, John</au><au>Steffen, Alexandra</au><au>Doerge, Chris</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>A study of the vertical scale of halogen chemistry in the Arctic troposphere during Polar Sunrise at Barrow, Alaska</atitle><jtitle>Journal of Geophysical Research. D. Atmospheres</jtitle><addtitle>J. Geophys. Res</addtitle><date>2007-04-16</date><risdate>2007</risdate><volume>112</volume><issue>D7</issue><epage>n/a</epage><issn>0148-0227</issn><issn>2169-897X</issn><eissn>2156-2202</eissn><eissn>2169-8996</eissn><abstract>The vertical extent and impact of halogen chemistry in the Arctic springtime was investigated through balloon‐based measurement of several atmospheric chemical components. Various chemical species, including volatile organic compounds (VOCs), ozone, and elemental mercury, that are modified by halogen chemistry were measured from the surface to ∼300 m during late March through mid‐April 2005 in Barrow, Alaska. It is observed that the halogen chemistry appears to be most active in the lowest 100–200 m of the atmosphere. The Hg vertical concentration profiles are consistent with destruction by chemistry that evolves from a species emitted from the snowpack, most likely Br2 and BrCl, and the VOC profiles also demonstrate the limited vertical scale of halogen‐initiated chemistry taking place above the Arctic snowpack.</abstract><cop>Washington, DC</cop><pub>Blackwell Publishing Ltd</pub><doi>10.1029/2006JD007785</doi><tpages>13</tpages><orcidid>https://orcid.org/0000-0002-1781-687X</orcidid><oa>free_for_read</oa></addata></record> |
| fulltext | fulltext |
| identifier | ISSN: 0148-0227 |
| ispartof | Journal of Geophysical Research. D. Atmospheres, 2007-04, Vol.112 (D7), p.n/a |
| issn | 0148-0227 2169-897X 2156-2202 2169-8996 |
| language | eng |
| recordid | cdi_hal_primary_oai_HAL_insu_00377484v1 |
| source | Wiley Online Library AGU Free Content; Access via Wiley Online Library; Wiley Online Library (Open Access Collection); Alma/SFX Local Collection |
| subjects | Arctic Earth Sciences Earth, ocean, space Exact sciences and technology Glaciology halogen chemistry Sciences of the Universe vertical profiles |
| title | A study of the vertical scale of halogen chemistry in the Arctic troposphere during Polar Sunrise at Barrow, Alaska |
| url | https://sfx.bib-bvb.de/sfx_tum?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2024-12-18T20%3A50%3A51IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-proquest_hal_p&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=A%20study%20of%20the%20vertical%20scale%20of%20halogen%20chemistry%20in%20the%20Arctic%20troposphere%20during%20Polar%20Sunrise%20at%20Barrow,%20Alaska&rft.jtitle=Journal%20of%20Geophysical%20Research.%20D.%20Atmospheres&rft.au=Tackett,%20Philip%20J.&rft.date=2007-04-16&rft.volume=112&rft.issue=D7&rft.epage=n/a&rft.issn=0148-0227&rft.eissn=2156-2202&rft_id=info:doi/10.1029/2006JD007785&rft_dat=%3Cproquest_hal_p%3E19775448%3C/proquest_hal_p%3E%3Curl%3E%3C/url%3E&disable_directlink=true&sfx.directlink=off&sfx.report_link=0&rft_id=info:oai/&rft_pqid=19775448&rft_id=info:pmid/&rfr_iscdi=true |