High-Efficiency Second-Harmonic Generation from Hybrid Light-Matter States
We report a novel approach to modify the second order nonlinear optical (NLO) susceptibility of organic nanofiber crystals by hybridization with the optical modes of microcavities in the strong coupling regime. The wavelength dependence of the SHG efficiency displays two intense peaks corresponding...
Gespeichert in:
| Veröffentlicht in: | Nano letters 2016-12, Vol.16 (12), p.7352-7356 |
|---|---|
| Hauptverfasser: | , , , , , , , , , , , , |
| Format: | Artikel |
| Sprache: | eng |
| Schlagworte: | |
| Online-Zugang: | Volltext |
| Tags: |
Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
|
| container_end_page | 7356 |
|---|---|
| container_issue | 12 |
| container_start_page | 7352 |
| container_title | Nano letters |
| container_volume | 16 |
| creator | Chervy, Thibault Xu, Jialiang Duan, Yulong Wang, Chunliang Mager, Loïc Frerejean, Maurice Münninghoff, Joris A. W Tinnemans, Paul Hutchison, James A Genet, Cyriaque Rowan, Alan E Rasing, Theo Ebbesen, Thomas W |
| description | We report a novel approach to modify the second order nonlinear optical (NLO) susceptibility of organic nanofiber crystals by hybridization with the optical modes of microcavities in the strong coupling regime. The wavelength dependence of the SHG efficiency displays two intense peaks corresponding to the so-formed light-matter hybrid states. Our results demonstrate an enhancement of the resonant SHG efficiency of the lower polariton by 2 orders of magnitude for the collectively coupled molecules as compared to that of the same material outside the microcavity. This study is a proof of principle that opens a new direction for NLO of organic materials in subwavelength resonators. |
| doi_str_mv | 10.1021/acs.nanolett.6b02567 |
| format | Article |
| fullrecord | <record><control><sourceid>proquest_hal_p</sourceid><recordid>TN_cdi_hal_primary_oai_HAL_hal_04680659v1</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>1852672016</sourcerecordid><originalsourceid>FETCH-LOGICAL-a448t-dbca07cc7f3bf4b926af382b0616ae537b0ca3248cd6418160662f641fb5942a3</originalsourceid><addsrcrecordid>eNp9kMtu2zAQRYmgReI8_qAotGwWcocURUlLI3CtFi66SLImhhTZMJDIlKQL-O8rw46XXc1gcO4d4BDyicKSAqNfUaelRx9Gk_NSKGC1aC7IgtYVlKLr2Ifz3vIrcp3SKwB0VQ2X5Io1nYCawoL86N3vl3JtrdPOeL0vHo0Ofih7jFPwThcb403E7IIvbAxT0e9VdEOxnWO5_Ik5m1g8Zswm3ZKPFsdk7k7zhjx_Wz899OX21-b7w2pbIudtLgelERqtG1spy1XHBNqqZQoEFWjqqlGgsWK81YPgtKUChGB2Xq2qO86wuiH3x94XHOVbdBPGvQzoZL_aysMNuGhB1N1fOrNfjuxbDH92JmU5uaTNOKI3YZckbWsmGgZUzCg_ojqGlKKx524K8mBczsblu3F5Mj7HPp8-7NRkhnPoXfEMwBE4xF_DLvpZzv87_wEUDY8I</addsrcrecordid><sourcetype>Open Access Repository</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>1852672016</pqid></control><display><type>article</type><title>High-Efficiency Second-Harmonic Generation from Hybrid Light-Matter States</title><source>American Chemical Society Journals</source><creator>Chervy, Thibault ; Xu, Jialiang ; Duan, Yulong ; Wang, Chunliang ; Mager, Loïc ; Frerejean, Maurice ; Münninghoff, Joris A. W ; Tinnemans, Paul ; Hutchison, James A ; Genet, Cyriaque ; Rowan, Alan E ; Rasing, Theo ; Ebbesen, Thomas W</creator><creatorcontrib>Chervy, Thibault ; Xu, Jialiang ; Duan, Yulong ; Wang, Chunliang ; Mager, Loïc ; Frerejean, Maurice ; Münninghoff, Joris A. W ; Tinnemans, Paul ; Hutchison, James A ; Genet, Cyriaque ; Rowan, Alan E ; Rasing, Theo ; Ebbesen, Thomas W</creatorcontrib><description>We report a novel approach to modify the second order nonlinear optical (NLO) susceptibility of organic nanofiber crystals by hybridization with the optical modes of microcavities in the strong coupling regime. The wavelength dependence of the SHG efficiency displays two intense peaks corresponding to the so-formed light-matter hybrid states. Our results demonstrate an enhancement of the resonant SHG efficiency of the lower polariton by 2 orders of magnitude for the collectively coupled molecules as compared to that of the same material outside the microcavity. This study is a proof of principle that opens a new direction for NLO of organic materials in subwavelength resonators.</description><identifier>ISSN: 1530-6984</identifier><identifier>EISSN: 1530-6992</identifier><identifier>DOI: 10.1021/acs.nanolett.6b02567</identifier><identifier>PMID: 27960510</identifier><language>eng</language><publisher>United States: American Chemical Society</publisher><subject>Chemical Sciences ; Material chemistry</subject><ispartof>Nano letters, 2016-12, Vol.16 (12), p.7352-7356</ispartof><rights>Copyright © 2016 American Chemical Society</rights><rights>Distributed under a Creative Commons Attribution 4.0 International License</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-a448t-dbca07cc7f3bf4b926af382b0616ae537b0ca3248cd6418160662f641fb5942a3</citedby><cites>FETCH-LOGICAL-a448t-dbca07cc7f3bf4b926af382b0616ae537b0ca3248cd6418160662f641fb5942a3</cites><orcidid>0000-0002-3999-1636 ; 0000-0001-9601-0024</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://pubs.acs.org/doi/pdf/10.1021/acs.nanolett.6b02567$$EPDF$$P50$$Gacs$$H</linktopdf><linktohtml>$$Uhttps://pubs.acs.org/doi/10.1021/acs.nanolett.6b02567$$EHTML$$P50$$Gacs$$H</linktohtml><link.rule.ids>230,314,776,780,881,2752,27053,27901,27902,56713,56763</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/27960510$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink><backlink>$$Uhttps://hal.science/hal-04680659$$DView record in HAL$$Hfree_for_read</backlink></links><search><creatorcontrib>Chervy, Thibault</creatorcontrib><creatorcontrib>Xu, Jialiang</creatorcontrib><creatorcontrib>Duan, Yulong</creatorcontrib><creatorcontrib>Wang, Chunliang</creatorcontrib><creatorcontrib>Mager, Loïc</creatorcontrib><creatorcontrib>Frerejean, Maurice</creatorcontrib><creatorcontrib>Münninghoff, Joris A. W</creatorcontrib><creatorcontrib>Tinnemans, Paul</creatorcontrib><creatorcontrib>Hutchison, James A</creatorcontrib><creatorcontrib>Genet, Cyriaque</creatorcontrib><creatorcontrib>Rowan, Alan E</creatorcontrib><creatorcontrib>Rasing, Theo</creatorcontrib><creatorcontrib>Ebbesen, Thomas W</creatorcontrib><title>High-Efficiency Second-Harmonic Generation from Hybrid Light-Matter States</title><title>Nano letters</title><addtitle>Nano Lett</addtitle><description>We report a novel approach to modify the second order nonlinear optical (NLO) susceptibility of organic nanofiber crystals by hybridization with the optical modes of microcavities in the strong coupling regime. The wavelength dependence of the SHG efficiency displays two intense peaks corresponding to the so-formed light-matter hybrid states. Our results demonstrate an enhancement of the resonant SHG efficiency of the lower polariton by 2 orders of magnitude for the collectively coupled molecules as compared to that of the same material outside the microcavity. This study is a proof of principle that opens a new direction for NLO of organic materials in subwavelength resonators.</description><subject>Chemical Sciences</subject><subject>Material chemistry</subject><issn>1530-6984</issn><issn>1530-6992</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2016</creationdate><recordtype>article</recordtype><recordid>eNp9kMtu2zAQRYmgReI8_qAotGwWcocURUlLI3CtFi66SLImhhTZMJDIlKQL-O8rw46XXc1gcO4d4BDyicKSAqNfUaelRx9Gk_NSKGC1aC7IgtYVlKLr2Ifz3vIrcp3SKwB0VQ2X5Io1nYCawoL86N3vl3JtrdPOeL0vHo0Ofih7jFPwThcb403E7IIvbAxT0e9VdEOxnWO5_Ik5m1g8Zswm3ZKPFsdk7k7zhjx_Wz899OX21-b7w2pbIudtLgelERqtG1spy1XHBNqqZQoEFWjqqlGgsWK81YPgtKUChGB2Xq2qO86wuiH3x94XHOVbdBPGvQzoZL_aysMNuGhB1N1fOrNfjuxbDH92JmU5uaTNOKI3YZckbWsmGgZUzCg_ojqGlKKx524K8mBczsblu3F5Mj7HPp8-7NRkhnPoXfEMwBE4xF_DLvpZzv87_wEUDY8I</recordid><startdate>20161214</startdate><enddate>20161214</enddate><creator>Chervy, Thibault</creator><creator>Xu, Jialiang</creator><creator>Duan, Yulong</creator><creator>Wang, Chunliang</creator><creator>Mager, Loïc</creator><creator>Frerejean, Maurice</creator><creator>Münninghoff, Joris A. W</creator><creator>Tinnemans, Paul</creator><creator>Hutchison, James A</creator><creator>Genet, Cyriaque</creator><creator>Rowan, Alan E</creator><creator>Rasing, Theo</creator><creator>Ebbesen, Thomas W</creator><general>American Chemical Society</general><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7X8</scope><scope>1XC</scope><orcidid>https://orcid.org/0000-0002-3999-1636</orcidid><orcidid>https://orcid.org/0000-0001-9601-0024</orcidid></search><sort><creationdate>20161214</creationdate><title>High-Efficiency Second-Harmonic Generation from Hybrid Light-Matter States</title><author>Chervy, Thibault ; Xu, Jialiang ; Duan, Yulong ; Wang, Chunliang ; Mager, Loïc ; Frerejean, Maurice ; Münninghoff, Joris A. W ; Tinnemans, Paul ; Hutchison, James A ; Genet, Cyriaque ; Rowan, Alan E ; Rasing, Theo ; Ebbesen, Thomas W</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-a448t-dbca07cc7f3bf4b926af382b0616ae537b0ca3248cd6418160662f641fb5942a3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2016</creationdate><topic>Chemical Sciences</topic><topic>Material chemistry</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Chervy, Thibault</creatorcontrib><creatorcontrib>Xu, Jialiang</creatorcontrib><creatorcontrib>Duan, Yulong</creatorcontrib><creatorcontrib>Wang, Chunliang</creatorcontrib><creatorcontrib>Mager, Loïc</creatorcontrib><creatorcontrib>Frerejean, Maurice</creatorcontrib><creatorcontrib>Münninghoff, Joris A. W</creatorcontrib><creatorcontrib>Tinnemans, Paul</creatorcontrib><creatorcontrib>Hutchison, James A</creatorcontrib><creatorcontrib>Genet, Cyriaque</creatorcontrib><creatorcontrib>Rowan, Alan E</creatorcontrib><creatorcontrib>Rasing, Theo</creatorcontrib><creatorcontrib>Ebbesen, Thomas W</creatorcontrib><collection>PubMed</collection><collection>CrossRef</collection><collection>MEDLINE - Academic</collection><collection>Hyper Article en Ligne (HAL)</collection><jtitle>Nano letters</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Chervy, Thibault</au><au>Xu, Jialiang</au><au>Duan, Yulong</au><au>Wang, Chunliang</au><au>Mager, Loïc</au><au>Frerejean, Maurice</au><au>Münninghoff, Joris A. W</au><au>Tinnemans, Paul</au><au>Hutchison, James A</au><au>Genet, Cyriaque</au><au>Rowan, Alan E</au><au>Rasing, Theo</au><au>Ebbesen, Thomas W</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>High-Efficiency Second-Harmonic Generation from Hybrid Light-Matter States</atitle><jtitle>Nano letters</jtitle><addtitle>Nano Lett</addtitle><date>2016-12-14</date><risdate>2016</risdate><volume>16</volume><issue>12</issue><spage>7352</spage><epage>7356</epage><pages>7352-7356</pages><issn>1530-6984</issn><eissn>1530-6992</eissn><abstract>We report a novel approach to modify the second order nonlinear optical (NLO) susceptibility of organic nanofiber crystals by hybridization with the optical modes of microcavities in the strong coupling regime. The wavelength dependence of the SHG efficiency displays two intense peaks corresponding to the so-formed light-matter hybrid states. Our results demonstrate an enhancement of the resonant SHG efficiency of the lower polariton by 2 orders of magnitude for the collectively coupled molecules as compared to that of the same material outside the microcavity. This study is a proof of principle that opens a new direction for NLO of organic materials in subwavelength resonators.</abstract><cop>United States</cop><pub>American Chemical Society</pub><pmid>27960510</pmid><doi>10.1021/acs.nanolett.6b02567</doi><tpages>5</tpages><orcidid>https://orcid.org/0000-0002-3999-1636</orcidid><orcidid>https://orcid.org/0000-0001-9601-0024</orcidid><oa>free_for_read</oa></addata></record> |
| fulltext | fulltext |
| identifier | ISSN: 1530-6984 |
| ispartof | Nano letters, 2016-12, Vol.16 (12), p.7352-7356 |
| issn | 1530-6984 1530-6992 |
| language | eng |
| recordid | cdi_hal_primary_oai_HAL_hal_04680659v1 |
| source | American Chemical Society Journals |
| subjects | Chemical Sciences Material chemistry |
| title | High-Efficiency Second-Harmonic Generation from Hybrid Light-Matter States |
| url | https://sfx.bib-bvb.de/sfx_tum?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2025-02-08T00%3A14%3A31IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-proquest_hal_p&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=High-Efficiency%20Second-Harmonic%20Generation%20from%20Hybrid%20Light-Matter%20States&rft.jtitle=Nano%20letters&rft.au=Chervy,%20Thibault&rft.date=2016-12-14&rft.volume=16&rft.issue=12&rft.spage=7352&rft.epage=7356&rft.pages=7352-7356&rft.issn=1530-6984&rft.eissn=1530-6992&rft_id=info:doi/10.1021/acs.nanolett.6b02567&rft_dat=%3Cproquest_hal_p%3E1852672016%3C/proquest_hal_p%3E%3Curl%3E%3C/url%3E&disable_directlink=true&sfx.directlink=off&sfx.report_link=0&rft_id=info:oai/&rft_pqid=1852672016&rft_id=info:pmid/27960510&rfr_iscdi=true |