Interplay between multipolar spin interactions, Jahn-Teller effect, and electronic correlation in a J eff = 3 2 insulator
In this work we study the complex entanglement between spin interactions, electron correlation and Janh-Teller structural instabilities in the 5d 1 J ef f = 3 2 spin-orbit coupled double perovskite Ba2NaOsO6 using first principles approaches. By combining non-collinear magnetic calculations with mul...
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| Veröffentlicht in: | Physical review. B 2021-03, Vol.103 (10), Article 104401 |
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| container_title | Physical review. B |
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| creator | Fiore Mosca, Dario Pourovskii, Leonid V. Kim, Beom Hyun Liu, Peitao Sanna, Samuele Boscherini, Federico Khmelevskyi, Sergii Franchini, Cesare |
| description | In this work we study the complex entanglement between spin interactions, electron correlation and Janh-Teller structural instabilities in the 5d 1 J ef f = 3 2 spin-orbit coupled double perovskite Ba2NaOsO6 using first principles approaches. By combining non-collinear magnetic calculations with multipolar pseudospin Hamiltonian analysis and many-body techniques we elucidate the origin of the observed quadrupolar canted antifferomagnetic. We show that the non-collinear magnetic order originates from Jahn-Teller distortions due to the cooperation of Heisenberg exchange, quadrupolar spin-spin terms and both dipolar and multipolar Dzyaloshinskii-Moriya interactions. We find a strong competition between ferromagnetic and antiferromagnetic canted and collinear quadrupolar magnetic phases: the transition from one magnetic order to another can be controlled by the strength of the electronic correlation (U) and by the degree of Jahn-Teller distortions. |
| doi_str_mv | 10.1103/PhysRevB.103.104401 |
| format | Article |
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By combining non-collinear magnetic calculations with multipolar pseudospin Hamiltonian analysis and many-body techniques we elucidate the origin of the observed quadrupolar canted antifferomagnetic. We show that the non-collinear magnetic order originates from Jahn-Teller distortions due to the cooperation of Heisenberg exchange, quadrupolar spin-spin terms and both dipolar and multipolar Dzyaloshinskii-Moriya interactions. 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B</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Fiore Mosca, Dario</au><au>Pourovskii, Leonid V.</au><au>Kim, Beom Hyun</au><au>Liu, Peitao</au><au>Sanna, Samuele</au><au>Boscherini, Federico</au><au>Khmelevskyi, Sergii</au><au>Franchini, Cesare</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Interplay between multipolar spin interactions, Jahn-Teller effect, and electronic correlation in a J eff = 3 2 insulator</atitle><jtitle>Physical review. B</jtitle><date>2021-03</date><risdate>2021</risdate><volume>103</volume><issue>10</issue><artnum>104401</artnum><issn>2469-9950</issn><eissn>2469-9969</eissn><abstract>In this work we study the complex entanglement between spin interactions, electron correlation and Janh-Teller structural instabilities in the 5d 1 J ef f = 3 2 spin-orbit coupled double perovskite Ba2NaOsO6 using first principles approaches. By combining non-collinear magnetic calculations with multipolar pseudospin Hamiltonian analysis and many-body techniques we elucidate the origin of the observed quadrupolar canted antifferomagnetic. We show that the non-collinear magnetic order originates from Jahn-Teller distortions due to the cooperation of Heisenberg exchange, quadrupolar spin-spin terms and both dipolar and multipolar Dzyaloshinskii-Moriya interactions. 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| subjects | Condensed Matter Materials Science Physics Strongly Correlated Electrons |
| title | Interplay between multipolar spin interactions, Jahn-Teller effect, and electronic correlation in a J eff = 3 2 insulator |
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