High‐Resolution and Stable Ruddlesden–Popper Quasi‐2D Perovskite Flexible Photodetectors Arrays for Potential Applications as Optical Image Sensor
The development of an efficient fabrication route to achieve high‐resolution perovskite pixel array is key for large‐scale flexible image sensor devices. Herein, a high‐resolution and stable 10 × 10 flexible PDs array based on formamidinium(FA + ) and phenylmethylammonium (PMA + ) quasi‐2D (PMA) 2 F...
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| Veröffentlicht in: | Advanced functional materials 2023-10, Vol.33 (43) |
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| creator | Wang, Tao Zheng, Daming Vegso, Karol Mrkyvkova, Nada Siffalovic, Peter Pauporté, Thierry |
| description | The development of an efficient fabrication route to achieve high‐resolution perovskite pixel array is key for large‐scale flexible image sensor devices. Herein, a high‐resolution and stable 10 × 10 flexible PDs array based on formamidinium(FA
+
) and phenylmethylammonium (PMA
+
) quasi‐2D (PMA)
2
FAPb
2
I
7
(
n
= 2) perovskite is demonstrated by developing SiO
2
‐assisted hydrophobic and hydrophilic treatment process on polyethylene terephthalate substrate. By introducing Au nanoparticles (Au NPs), the perovskite film quality is improved and grain boundaries are reduced. The mechanism by which Au NPs upgrade the photoelectric quality of perovskite is mainly revealed by glow discharge‐optical emission spectroscopy (GD‐OES) and grazing‐incidence wide‐angle X‐ray scattering (GIWAXS). To further improve the photoelectric performance of the devices, a post‐treatment strategy with formamidinium chloride (FACl) is used . The optimized flexible PDs arrays show excellent optoelectronic properties with a high responsivity of 4.7 A W
−1
, a detectivity of 6.3 × 10
12
Jones, and a broad spectral sensitivity. The device also exhibits excellent electrical stability even under severe bending and excellent flexural strength, as well as excellent environmental stability. Finally, the integrated flexible PDs arrays are used as sensor pixels in an imaging system to obtain high‐resolution imaging patterns, demonstrating the imaging capability of the PDs arrays. |
| doi_str_mv | 10.1002/adfm.202304659 |
| format | Article |
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+
) and phenylmethylammonium (PMA
+
) quasi‐2D (PMA)
2
FAPb
2
I
7
(
n
= 2) perovskite is demonstrated by developing SiO
2
‐assisted hydrophobic and hydrophilic treatment process on polyethylene terephthalate substrate. By introducing Au nanoparticles (Au NPs), the perovskite film quality is improved and grain boundaries are reduced. The mechanism by which Au NPs upgrade the photoelectric quality of perovskite is mainly revealed by glow discharge‐optical emission spectroscopy (GD‐OES) and grazing‐incidence wide‐angle X‐ray scattering (GIWAXS). To further improve the photoelectric performance of the devices, a post‐treatment strategy with formamidinium chloride (FACl) is used . The optimized flexible PDs arrays show excellent optoelectronic properties with a high responsivity of 4.7 A W
−1
, a detectivity of 6.3 × 10
12
Jones, and a broad spectral sensitivity. The device also exhibits excellent electrical stability even under severe bending and excellent flexural strength, as well as excellent environmental stability. Finally, the integrated flexible PDs arrays are used as sensor pixels in an imaging system to obtain high‐resolution imaging patterns, demonstrating the imaging capability of the PDs arrays.</description><identifier>ISSN: 1616-301X</identifier><identifier>EISSN: 1616-3028</identifier><identifier>DOI: 10.1002/adfm.202304659</identifier><language>eng</language><publisher>Hoboken: Wiley Subscription Services, Inc</publisher><subject>Arrays ; Chemical Sciences ; Engineering Sciences ; Flexural strength ; Glow discharges ; Gold ; Grain boundaries ; Imaging ; Instrumentation and Detectors ; Material chemistry ; Materials science ; Micro and nanotechnologies ; Microelectronics ; Modulus of rupture in bending ; Nanoparticles ; Optical emission spectroscopy ; Optics ; Optoelectronics ; Perovskites ; Photoelectricity ; Photonic ; Physics ; Pixels ; Polyethylene terephthalate ; Sensors ; Silicon dioxide ; Spectral sensitivity ; Stability ; Substrates</subject><ispartof>Advanced functional materials, 2023-10, Vol.33 (43)</ispartof><rights>2023. This article is published under http://creativecommons.org/licenses/by-nc/4.0/ (the “License”). Notwithstanding the ProQuest Terms and Conditions, you may use this content in accordance with the terms of the License.</rights><rights>Distributed under a Creative Commons Attribution 4.0 International License</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c341t-9af0170801bb5ab0b8ed36ed1549f994d4b765cd4ad0bd76521c22926a69c8463</citedby><cites>FETCH-LOGICAL-c341t-9af0170801bb5ab0b8ed36ed1549f994d4b765cd4ad0bd76521c22926a69c8463</cites><orcidid>0000-0002-6939-5675 ; 0000-0001-5906-8075</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>230,315,781,785,886,27929,27930</link.rule.ids><backlink>$$Uhttps://cnrs.hal.science/hal-04149331$$DView record in HAL$$Hfree_for_read</backlink></links><search><creatorcontrib>Wang, Tao</creatorcontrib><creatorcontrib>Zheng, Daming</creatorcontrib><creatorcontrib>Vegso, Karol</creatorcontrib><creatorcontrib>Mrkyvkova, Nada</creatorcontrib><creatorcontrib>Siffalovic, Peter</creatorcontrib><creatorcontrib>Pauporté, Thierry</creatorcontrib><title>High‐Resolution and Stable Ruddlesden–Popper Quasi‐2D Perovskite Flexible Photodetectors Arrays for Potential Applications as Optical Image Sensor</title><title>Advanced functional materials</title><description>The development of an efficient fabrication route to achieve high‐resolution perovskite pixel array is key for large‐scale flexible image sensor devices. Herein, a high‐resolution and stable 10 × 10 flexible PDs array based on formamidinium(FA
+
) and phenylmethylammonium (PMA
+
) quasi‐2D (PMA)
2
FAPb
2
I
7
(
n
= 2) perovskite is demonstrated by developing SiO
2
‐assisted hydrophobic and hydrophilic treatment process on polyethylene terephthalate substrate. By introducing Au nanoparticles (Au NPs), the perovskite film quality is improved and grain boundaries are reduced. The mechanism by which Au NPs upgrade the photoelectric quality of perovskite is mainly revealed by glow discharge‐optical emission spectroscopy (GD‐OES) and grazing‐incidence wide‐angle X‐ray scattering (GIWAXS). To further improve the photoelectric performance of the devices, a post‐treatment strategy with formamidinium chloride (FACl) is used . The optimized flexible PDs arrays show excellent optoelectronic properties with a high responsivity of 4.7 A W
−1
, a detectivity of 6.3 × 10
12
Jones, and a broad spectral sensitivity. The device also exhibits excellent electrical stability even under severe bending and excellent flexural strength, as well as excellent environmental stability. Finally, the integrated flexible PDs arrays are used as sensor pixels in an imaging system to obtain high‐resolution imaging patterns, demonstrating the imaging capability of the PDs arrays.</description><subject>Arrays</subject><subject>Chemical Sciences</subject><subject>Engineering Sciences</subject><subject>Flexural strength</subject><subject>Glow discharges</subject><subject>Gold</subject><subject>Grain boundaries</subject><subject>Imaging</subject><subject>Instrumentation and Detectors</subject><subject>Material chemistry</subject><subject>Materials science</subject><subject>Micro and nanotechnologies</subject><subject>Microelectronics</subject><subject>Modulus of rupture in bending</subject><subject>Nanoparticles</subject><subject>Optical emission spectroscopy</subject><subject>Optics</subject><subject>Optoelectronics</subject><subject>Perovskites</subject><subject>Photoelectricity</subject><subject>Photonic</subject><subject>Physics</subject><subject>Pixels</subject><subject>Polyethylene terephthalate</subject><subject>Sensors</subject><subject>Silicon dioxide</subject><subject>Spectral sensitivity</subject><subject>Stability</subject><subject>Substrates</subject><issn>1616-301X</issn><issn>1616-3028</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2023</creationdate><recordtype>article</recordtype><recordid>eNo9UctOwzAQjBBIPK-cLXHi0OJX0-RY8SpSJcpL4mZt4g01uHGwHQQ3PgGJC9_Hl5CoqKedXc3M7mqS5JDRIaOUn4CulkNOuaAyHeUbyQ5LWToQlGeba8wet5PdEJ4pZeOxkDvJz9Q8LX4_v24xONtG42oCtSZ3EQqL5LbV2mLQWP9-fs9d06AnNy0E0yn4GZmjd2_hxUQkFxbfTS-ZL1x0GiOW0flAJt7DRyCV82TuItbRgCWTprGmhH5bIBDIdRO71pKrJTwhucM6OL-fbFVgAx78173k4eL8_nQ6mF1fXp1OZoNSSBYHOVTdKzSjrChGUNAiQy1S1Gwk8yrPpZbFOB2VWoKmhe4gZyXnOU8hzctMpmIvOV75LsCqxpsl-A_lwKjpZKb6GZVM5kKwN9Zxj1bcxrvXFkNUz671dXee4tk445xmgnes4YpVeheCx2pty6jqk1J9UmqdlPgDJYOLYg</recordid><startdate>20231018</startdate><enddate>20231018</enddate><creator>Wang, Tao</creator><creator>Zheng, Daming</creator><creator>Vegso, Karol</creator><creator>Mrkyvkova, Nada</creator><creator>Siffalovic, Peter</creator><creator>Pauporté, Thierry</creator><general>Wiley Subscription Services, Inc</general><general>Wiley</general><scope>AAYXX</scope><scope>CITATION</scope><scope>7SP</scope><scope>7SR</scope><scope>7U5</scope><scope>8BQ</scope><scope>8FD</scope><scope>JG9</scope><scope>L7M</scope><scope>1XC</scope><scope>VOOES</scope><orcidid>https://orcid.org/0000-0002-6939-5675</orcidid><orcidid>https://orcid.org/0000-0001-5906-8075</orcidid></search><sort><creationdate>20231018</creationdate><title>High‐Resolution and Stable Ruddlesden–Popper Quasi‐2D Perovskite Flexible Photodetectors Arrays for Potential Applications as Optical Image Sensor</title><author>Wang, Tao ; Zheng, Daming ; Vegso, Karol ; Mrkyvkova, Nada ; Siffalovic, Peter ; Pauporté, Thierry</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c341t-9af0170801bb5ab0b8ed36ed1549f994d4b765cd4ad0bd76521c22926a69c8463</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2023</creationdate><topic>Arrays</topic><topic>Chemical Sciences</topic><topic>Engineering Sciences</topic><topic>Flexural strength</topic><topic>Glow discharges</topic><topic>Gold</topic><topic>Grain boundaries</topic><topic>Imaging</topic><topic>Instrumentation and Detectors</topic><topic>Material chemistry</topic><topic>Materials science</topic><topic>Micro and nanotechnologies</topic><topic>Microelectronics</topic><topic>Modulus of rupture in bending</topic><topic>Nanoparticles</topic><topic>Optical emission spectroscopy</topic><topic>Optics</topic><topic>Optoelectronics</topic><topic>Perovskites</topic><topic>Photoelectricity</topic><topic>Photonic</topic><topic>Physics</topic><topic>Pixels</topic><topic>Polyethylene terephthalate</topic><topic>Sensors</topic><topic>Silicon dioxide</topic><topic>Spectral sensitivity</topic><topic>Stability</topic><topic>Substrates</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Wang, Tao</creatorcontrib><creatorcontrib>Zheng, Daming</creatorcontrib><creatorcontrib>Vegso, Karol</creatorcontrib><creatorcontrib>Mrkyvkova, Nada</creatorcontrib><creatorcontrib>Siffalovic, Peter</creatorcontrib><creatorcontrib>Pauporté, Thierry</creatorcontrib><collection>CrossRef</collection><collection>Electronics & Communications Abstracts</collection><collection>Engineered Materials Abstracts</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>Materials Research Database</collection><collection>Advanced Technologies Database with Aerospace</collection><collection>Hyper Article en Ligne (HAL)</collection><collection>Hyper Article en Ligne (HAL) (Open Access)</collection><jtitle>Advanced functional materials</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Wang, Tao</au><au>Zheng, Daming</au><au>Vegso, Karol</au><au>Mrkyvkova, Nada</au><au>Siffalovic, Peter</au><au>Pauporté, Thierry</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>High‐Resolution and Stable Ruddlesden–Popper Quasi‐2D Perovskite Flexible Photodetectors Arrays for Potential Applications as Optical Image Sensor</atitle><jtitle>Advanced functional materials</jtitle><date>2023-10-18</date><risdate>2023</risdate><volume>33</volume><issue>43</issue><issn>1616-301X</issn><eissn>1616-3028</eissn><abstract>The development of an efficient fabrication route to achieve high‐resolution perovskite pixel array is key for large‐scale flexible image sensor devices. Herein, a high‐resolution and stable 10 × 10 flexible PDs array based on formamidinium(FA
+
) and phenylmethylammonium (PMA
+
) quasi‐2D (PMA)
2
FAPb
2
I
7
(
n
= 2) perovskite is demonstrated by developing SiO
2
‐assisted hydrophobic and hydrophilic treatment process on polyethylene terephthalate substrate. By introducing Au nanoparticles (Au NPs), the perovskite film quality is improved and grain boundaries are reduced. The mechanism by which Au NPs upgrade the photoelectric quality of perovskite is mainly revealed by glow discharge‐optical emission spectroscopy (GD‐OES) and grazing‐incidence wide‐angle X‐ray scattering (GIWAXS). To further improve the photoelectric performance of the devices, a post‐treatment strategy with formamidinium chloride (FACl) is used . The optimized flexible PDs arrays show excellent optoelectronic properties with a high responsivity of 4.7 A W
−1
, a detectivity of 6.3 × 10
12
Jones, and a broad spectral sensitivity. The device also exhibits excellent electrical stability even under severe bending and excellent flexural strength, as well as excellent environmental stability. Finally, the integrated flexible PDs arrays are used as sensor pixels in an imaging system to obtain high‐resolution imaging patterns, demonstrating the imaging capability of the PDs arrays.</abstract><cop>Hoboken</cop><pub>Wiley Subscription Services, Inc</pub><doi>10.1002/adfm.202304659</doi><orcidid>https://orcid.org/0000-0002-6939-5675</orcidid><orcidid>https://orcid.org/0000-0001-5906-8075</orcidid><oa>free_for_read</oa></addata></record> |
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| subjects | Arrays Chemical Sciences Engineering Sciences Flexural strength Glow discharges Gold Grain boundaries Imaging Instrumentation and Detectors Material chemistry Materials science Micro and nanotechnologies Microelectronics Modulus of rupture in bending Nanoparticles Optical emission spectroscopy Optics Optoelectronics Perovskites Photoelectricity Photonic Physics Pixels Polyethylene terephthalate Sensors Silicon dioxide Spectral sensitivity Stability Substrates |
| title | High‐Resolution and Stable Ruddlesden–Popper Quasi‐2D Perovskite Flexible Photodetectors Arrays for Potential Applications as Optical Image Sensor |
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