Temperature of photoanode for photoelectrochemical water oxidation
Solar-light-driven photoelectrochemical that can utilise water for high-performance artificial photosynthesis for low-cost green hydrogen fuel production. However, the interaction of photoanode with water is crucial to its heterogeneous water oxidation for sustainable fuel production for the replace...
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| Veröffentlicht in: | Renewable energy 2023-05, Vol.208, p.504-511 |
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| creator | Biswas, Neeraj Kumar Srivastav, Anupam Saxena, Sakshi Verma, Anuradha Dutta, Runjhun Srivastava, Manju Upadhyay, Sumant Satsangi, Vibha Rani Shrivastav, Rohit Dass, Sahab |
| description | Solar-light-driven photoelectrochemical that can utilise water for high-performance artificial photosynthesis for low-cost green hydrogen fuel production. However, the interaction of photoanode with water is crucial to its heterogeneous water oxidation for sustainable fuel production for the replacement of fossil fuels. Here, we report experiment investigations of photoelectrode with temperature for solar energy conversion. These measurements revealed that a rise in temperature affects the catalytic generation of hydrogen in three routes, viz., minimising the required energy for water splitting, reducing bandgap energy and mitigating the resistance at the interface.
[Display omitted]
•The bandgap of PCNDTO reduces with the increase in electrolytic temperature.•Resistance at semiconductor/electrolytes interface with rising temperature of electrolytes.•Faradaic efficiency of 92.49% for hydrogen production achieved at 45 °C in aqueous solution of NaOH + F6NaP. |
| doi_str_mv | 10.1016/j.renene.2023.02.129 |
| format | Article |
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[Display omitted]
•The bandgap of PCNDTO reduces with the increase in electrolytic temperature.•Resistance at semiconductor/electrolytes interface with rising temperature of electrolytes.•Faradaic efficiency of 92.49% for hydrogen production achieved at 45 °C in aqueous solution of NaOH + F6NaP.</description><identifier>ISSN: 0960-1481</identifier><identifier>EISSN: 1879-0682</identifier><identifier>DOI: 10.1016/j.renene.2023.02.129</identifier><language>eng</language><publisher>Elsevier Ltd</publisher><subject>Chemical Sciences ; Hydrogen ; Partially crystalline ; Photoelectrochemical ; Temperature ; TiO2</subject><ispartof>Renewable energy, 2023-05, Vol.208, p.504-511</ispartof><rights>2023 Elsevier Ltd</rights><rights>Distributed under a Creative Commons Attribution 4.0 International License</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c340t-89292d6559e14acd4c28455bcc336a0065b12bc6ca50c4c53a56c9adf1f8c3493</citedby><cites>FETCH-LOGICAL-c340t-89292d6559e14acd4c28455bcc336a0065b12bc6ca50c4c53a56c9adf1f8c3493</cites><orcidid>0000-0003-0798-2185 ; 0000-0003-1757-9744 ; 0000-0002-3992-7044</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktohtml>$$Uhttps://dx.doi.org/10.1016/j.renene.2023.02.129$$EHTML$$P50$$Gelsevier$$H</linktohtml><link.rule.ids>230,314,780,784,885,3550,27924,27925,45995</link.rule.ids><backlink>$$Uhttps://hal.science/hal-04124338$$DView record in HAL$$Hfree_for_read</backlink></links><search><creatorcontrib>Biswas, Neeraj Kumar</creatorcontrib><creatorcontrib>Srivastav, Anupam</creatorcontrib><creatorcontrib>Saxena, Sakshi</creatorcontrib><creatorcontrib>Verma, Anuradha</creatorcontrib><creatorcontrib>Dutta, Runjhun</creatorcontrib><creatorcontrib>Srivastava, Manju</creatorcontrib><creatorcontrib>Upadhyay, Sumant</creatorcontrib><creatorcontrib>Satsangi, Vibha Rani</creatorcontrib><creatorcontrib>Shrivastav, Rohit</creatorcontrib><creatorcontrib>Dass, Sahab</creatorcontrib><title>Temperature of photoanode for photoelectrochemical water oxidation</title><title>Renewable energy</title><description>Solar-light-driven photoelectrochemical that can utilise water for high-performance artificial photosynthesis for low-cost green hydrogen fuel production. However, the interaction of photoanode with water is crucial to its heterogeneous water oxidation for sustainable fuel production for the replacement of fossil fuels. Here, we report experiment investigations of photoelectrode with temperature for solar energy conversion. These measurements revealed that a rise in temperature affects the catalytic generation of hydrogen in three routes, viz., minimising the required energy for water splitting, reducing bandgap energy and mitigating the resistance at the interface.
[Display omitted]
•The bandgap of PCNDTO reduces with the increase in electrolytic temperature.•Resistance at semiconductor/electrolytes interface with rising temperature of electrolytes.•Faradaic efficiency of 92.49% for hydrogen production achieved at 45 °C in aqueous solution of NaOH + F6NaP.</description><subject>Chemical Sciences</subject><subject>Hydrogen</subject><subject>Partially crystalline</subject><subject>Photoelectrochemical</subject><subject>Temperature</subject><subject>TiO2</subject><issn>0960-1481</issn><issn>1879-0682</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2023</creationdate><recordtype>article</recordtype><recordid>eNp9kE9Lw0AQxRdRsFa_gYdcPSTO_u3mItSiVih4qedlO5nQLWm2bGLVb29KxKPMYZjhvQfvx9gth4IDN_e7IlE7TCFAyAJEwUV5xibczsocjBXnbAKlgZwryy_ZVdftALi2MzVhj2vaHyj5_iNRFuvssI199G2sKKtjGk9qCPsUcUv7gL7JPn1PKYtfofJ9iO01u6h909HN756y9-en9WKZr95eXhfzVY5SQZ_bUpSiMlqXxJXHSqGwSusNopTGAxi94WKDBr0GVKil1wZLX9W8tkNCKafsbszd-sYdUtj79O2iD245X7nTDxQXSkp75INWjVpMsesS1X8GDu7EzO3cyMydmDkQbmA22B5GGw09joGS6zBQi1SFNDBwVQz_B_wAY4t3Vw</recordid><startdate>202305</startdate><enddate>202305</enddate><creator>Biswas, Neeraj Kumar</creator><creator>Srivastav, Anupam</creator><creator>Saxena, Sakshi</creator><creator>Verma, Anuradha</creator><creator>Dutta, Runjhun</creator><creator>Srivastava, Manju</creator><creator>Upadhyay, Sumant</creator><creator>Satsangi, Vibha Rani</creator><creator>Shrivastav, Rohit</creator><creator>Dass, Sahab</creator><general>Elsevier Ltd</general><general>Elsevier</general><scope>AAYXX</scope><scope>CITATION</scope><scope>1XC</scope><orcidid>https://orcid.org/0000-0003-0798-2185</orcidid><orcidid>https://orcid.org/0000-0003-1757-9744</orcidid><orcidid>https://orcid.org/0000-0002-3992-7044</orcidid></search><sort><creationdate>202305</creationdate><title>Temperature of photoanode for photoelectrochemical water oxidation</title><author>Biswas, Neeraj Kumar ; Srivastav, Anupam ; Saxena, Sakshi ; Verma, Anuradha ; Dutta, Runjhun ; Srivastava, Manju ; Upadhyay, Sumant ; Satsangi, Vibha Rani ; Shrivastav, Rohit ; Dass, Sahab</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c340t-89292d6559e14acd4c28455bcc336a0065b12bc6ca50c4c53a56c9adf1f8c3493</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2023</creationdate><topic>Chemical Sciences</topic><topic>Hydrogen</topic><topic>Partially crystalline</topic><topic>Photoelectrochemical</topic><topic>Temperature</topic><topic>TiO2</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Biswas, Neeraj Kumar</creatorcontrib><creatorcontrib>Srivastav, Anupam</creatorcontrib><creatorcontrib>Saxena, Sakshi</creatorcontrib><creatorcontrib>Verma, Anuradha</creatorcontrib><creatorcontrib>Dutta, Runjhun</creatorcontrib><creatorcontrib>Srivastava, Manju</creatorcontrib><creatorcontrib>Upadhyay, Sumant</creatorcontrib><creatorcontrib>Satsangi, Vibha Rani</creatorcontrib><creatorcontrib>Shrivastav, Rohit</creatorcontrib><creatorcontrib>Dass, Sahab</creatorcontrib><collection>CrossRef</collection><collection>Hyper Article en Ligne (HAL)</collection><jtitle>Renewable energy</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Biswas, Neeraj Kumar</au><au>Srivastav, Anupam</au><au>Saxena, Sakshi</au><au>Verma, Anuradha</au><au>Dutta, Runjhun</au><au>Srivastava, Manju</au><au>Upadhyay, Sumant</au><au>Satsangi, Vibha Rani</au><au>Shrivastav, Rohit</au><au>Dass, Sahab</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Temperature of photoanode for photoelectrochemical water oxidation</atitle><jtitle>Renewable energy</jtitle><date>2023-05</date><risdate>2023</risdate><volume>208</volume><spage>504</spage><epage>511</epage><pages>504-511</pages><issn>0960-1481</issn><eissn>1879-0682</eissn><abstract>Solar-light-driven photoelectrochemical that can utilise water for high-performance artificial photosynthesis for low-cost green hydrogen fuel production. However, the interaction of photoanode with water is crucial to its heterogeneous water oxidation for sustainable fuel production for the replacement of fossil fuels. Here, we report experiment investigations of photoelectrode with temperature for solar energy conversion. These measurements revealed that a rise in temperature affects the catalytic generation of hydrogen in three routes, viz., minimising the required energy for water splitting, reducing bandgap energy and mitigating the resistance at the interface.
[Display omitted]
•The bandgap of PCNDTO reduces with the increase in electrolytic temperature.•Resistance at semiconductor/electrolytes interface with rising temperature of electrolytes.•Faradaic efficiency of 92.49% for hydrogen production achieved at 45 °C in aqueous solution of NaOH + F6NaP.</abstract><pub>Elsevier Ltd</pub><doi>10.1016/j.renene.2023.02.129</doi><tpages>8</tpages><orcidid>https://orcid.org/0000-0003-0798-2185</orcidid><orcidid>https://orcid.org/0000-0003-1757-9744</orcidid><orcidid>https://orcid.org/0000-0002-3992-7044</orcidid></addata></record> |
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| subjects | Chemical Sciences Hydrogen Partially crystalline Photoelectrochemical Temperature TiO2 |
| title | Temperature of photoanode for photoelectrochemical water oxidation |
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