Impact of Carbon Co-Doping on the Optical and Scintillation Properties of a YAG:Ce Scintillator
This paper addresses the carbon co-doping of Ce-doped garnets, an efficient scintillation material and white light phosphor. The composition and the optical and scintillation properties of carbon-co-doped Y3Al5O12 (YAG) are studied at different cerium and carbon concentrations. YAG:Ce,C crystals wer...
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| Veröffentlicht in: | Crystal growth & design 2021-05, Vol.21 (5), p.3063-3070 |
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| creator | Sidletskiy, Oleg Gerasymov, Iaroslav Boyaryntseva, Yanina Arhipov, Pavlo Tkachenko, Serhii Zelenskaya, Olga Bryleva, Kateryna Belikov, Konstantin Lebbou, Kheirreddine Dujardin, Christophe Büchner, Bernd Grynyov, Borys |
| description | This paper addresses the carbon co-doping of Ce-doped garnets, an efficient scintillation material and white light phosphor. The composition and the optical and scintillation properties of carbon-co-doped Y3Al5O12 (YAG) are studied at different cerium and carbon concentrations. YAG:Ce,C crystals were grown in the Ar + CO atmosphere from W crucibles. The carbon concentration reaches 0.5 atom %, but it does not affect the Ce distribution coefficient. The appearance and elimination of color centers are discussed in comparison to Ce-free YAG:C crystals. The tuning of cerium and carbon concentrations provides a light yield enhancement of up to 29 600 phot/MeV. The achieved enhancement may extend the application range of garnet-type phosphors and scintillators. |
| doi_str_mv | 10.1021/acs.cgd.1c00259 |
| format | Article |
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The composition and the optical and scintillation properties of carbon-co-doped Y3Al5O12 (YAG) are studied at different cerium and carbon concentrations. YAG:Ce,C crystals were grown in the Ar + CO atmosphere from W crucibles. The carbon concentration reaches 0.5 atom %, but it does not affect the Ce distribution coefficient. The appearance and elimination of color centers are discussed in comparison to Ce-free YAG:C crystals. The tuning of cerium and carbon concentrations provides a light yield enhancement of up to 29 600 phot/MeV. 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Growth Des</addtitle><date>2021-05-05</date><risdate>2021</risdate><volume>21</volume><issue>5</issue><spage>3063</spage><epage>3070</epage><pages>3063-3070</pages><issn>1528-7483</issn><eissn>1528-7505</eissn><abstract>This paper addresses the carbon co-doping of Ce-doped garnets, an efficient scintillation material and white light phosphor. The composition and the optical and scintillation properties of carbon-co-doped Y3Al5O12 (YAG) are studied at different cerium and carbon concentrations. YAG:Ce,C crystals were grown in the Ar + CO atmosphere from W crucibles. The carbon concentration reaches 0.5 atom %, but it does not affect the Ce distribution coefficient. The appearance and elimination of color centers are discussed in comparison to Ce-free YAG:C crystals. The tuning of cerium and carbon concentrations provides a light yield enhancement of up to 29 600 phot/MeV. 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| title | Impact of Carbon Co-Doping on the Optical and Scintillation Properties of a YAG:Ce Scintillator |
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