Atmospheric Nitrous Oxide Variations on Centennial Time Scales During the Past Two Millennia

The continuous growth of atmospheric nitrous oxide (N2O) is of concern for its potential role in global warming and future stratospheric ozone destruction. Climate feedbacks that enhance N2O emissions in response to global warming are not well understood, and past records of N2O from ice cores are n...

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Veröffentlicht in:Global biogeochemical cycles 2020-09, Vol.34 (9), p.n/a
Hauptverfasser: Ryu, Y., Ahn, J., Yang, J.‐W., Brook, E. J., Timmermann, A., Blunier, T., Hur, S., Kim, S.‐J.
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container_issue 9
container_start_page
container_title Global biogeochemical cycles
container_volume 34
creator Ryu, Y.
Ahn, J.
Yang, J.‐W.
Brook, E. J.
Timmermann, A.
Blunier, T.
Hur, S.
Kim, S.‐J.
description The continuous growth of atmospheric nitrous oxide (N2O) is of concern for its potential role in global warming and future stratospheric ozone destruction. Climate feedbacks that enhance N2O emissions in response to global warming are not well understood, and past records of N2O from ice cores are not sufficiently well resolved to examine the underlying climate‐N2O feedbacks on societally relevant time scales. Here, we present a new high‐resolution and high‐precision N2O reconstruction obtained from the Greenland NEEM (North Greenland Eemian Ice Drilling) and the Antarctic Styx Glacier ice cores. Covering the N2O history of the past two millennia, our reconstruction shows a centennial‐scale variability of ~10 ppb. A pronounced minimum at ~600 CE coincides with the reorganizations of tropical hydroclimate and ocean productivity changes. Comparisons with proxy records suggest association of centennial‐ to millennial‐scale variations in N2O with changes in tropical and subtropical land hydrology and marine productivity. Plain Language Summary Nitrous oxide (N2O) is a greenhouse and ozone‐depleting gas. The growing level of N2O in the atmosphere is of global concern, and records of past N2O variations can provide an important context for understanding the links between N2O and climate change. In this study, we report new, high‐quality N2O records covering the last two millennia using ice cores obtained from Greenland and Antarctica. Our N2O records show rapid centennial‐scale changes in atmospheric N2O and confirm a pronounced minimum near 600 CE. Comparison with climate records suggests that hydroclimate change on land and changes in marine productivity contribute to centennial‐ to millennial‐scale N2O variations. Key Points We report records of N2O concentration for the last 2,000 yr from the Styx ice core in Antarctca and NEEM ice core in Greenland The data accurately reveal the timing and magnitude of N2O variations on centennial time scales Variations in N2O are associated with changes in tropical and subtropical land hydrology and marine productivity
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J. ; Timmermann, A. ; Blunier, T. ; Hur, S. ; Kim, S.‐J.</creator><creatorcontrib>Ryu, Y. ; Ahn, J. ; Yang, J.‐W. ; Brook, E. J. ; Timmermann, A. ; Blunier, T. ; Hur, S. ; Kim, S.‐J.</creatorcontrib><description>The continuous growth of atmospheric nitrous oxide (N2O) is of concern for its potential role in global warming and future stratospheric ozone destruction. Climate feedbacks that enhance N2O emissions in response to global warming are not well understood, and past records of N2O from ice cores are not sufficiently well resolved to examine the underlying climate‐N2O feedbacks on societally relevant time scales. Here, we present a new high‐resolution and high‐precision N2O reconstruction obtained from the Greenland NEEM (North Greenland Eemian Ice Drilling) and the Antarctic Styx Glacier ice cores. Covering the N2O history of the past two millennia, our reconstruction shows a centennial‐scale variability of ~10 ppb. A pronounced minimum at ~600 CE coincides with the reorganizations of tropical hydroclimate and ocean productivity changes. Comparisons with proxy records suggest association of centennial‐ to millennial‐scale variations in N2O with changes in tropical and subtropical land hydrology and marine productivity. Plain Language Summary Nitrous oxide (N2O) is a greenhouse and ozone‐depleting gas. The growing level of N2O in the atmosphere is of global concern, and records of past N2O variations can provide an important context for understanding the links between N2O and climate change. In this study, we report new, high‐quality N2O records covering the last two millennia using ice cores obtained from Greenland and Antarctica. Our N2O records show rapid centennial‐scale changes in atmospheric N2O and confirm a pronounced minimum near 600 CE. Comparison with climate records suggests that hydroclimate change on land and changes in marine productivity contribute to centennial‐ to millennial‐scale N2O variations. Key Points We report records of N2O concentration for the last 2,000 yr from the Styx ice core in Antarctca and NEEM ice core in Greenland The data accurately reveal the timing and magnitude of N2O variations on centennial time scales Variations in N2O are associated with changes in tropical and subtropical land hydrology and marine productivity</description><identifier>ISSN: 0886-6236</identifier><identifier>EISSN: 1944-9224</identifier><identifier>EISSN: 1944-8224</identifier><identifier>DOI: 10.1029/2020GB006568</identifier><language>eng</language><publisher>Washington: Blackwell Publishing Ltd</publisher><subject>Antarctic glaciers ; Climate change ; Cores ; Drilling ; Glacier ice ; Glaciers ; Global warming ; Hydroclimate ; Hydrology ; Ice ; ice core ; Ice cores ; Neem ; Nitrous oxide ; Ocean, Atmosphere ; Ozone ; Ozone depletion ; Ozone destruction ; paleoclimate ; Productivity ; Reconstruction ; Records ; Sciences of the Universe ; Stratospheric warming ; Time ; Tropical climate ; Variation</subject><ispartof>Global biogeochemical cycles, 2020-09, Vol.34 (9), p.n/a</ispartof><rights>2020. 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J.</creatorcontrib><creatorcontrib>Timmermann, A.</creatorcontrib><creatorcontrib>Blunier, T.</creatorcontrib><creatorcontrib>Hur, S.</creatorcontrib><creatorcontrib>Kim, S.‐J.</creatorcontrib><title>Atmospheric Nitrous Oxide Variations on Centennial Time Scales During the Past Two Millennia</title><title>Global biogeochemical cycles</title><description>The continuous growth of atmospheric nitrous oxide (N2O) is of concern for its potential role in global warming and future stratospheric ozone destruction. Climate feedbacks that enhance N2O emissions in response to global warming are not well understood, and past records of N2O from ice cores are not sufficiently well resolved to examine the underlying climate‐N2O feedbacks on societally relevant time scales. Here, we present a new high‐resolution and high‐precision N2O reconstruction obtained from the Greenland NEEM (North Greenland Eemian Ice Drilling) and the Antarctic Styx Glacier ice cores. 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J.</au><au>Timmermann, A.</au><au>Blunier, T.</au><au>Hur, S.</au><au>Kim, S.‐J.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Atmospheric Nitrous Oxide Variations on Centennial Time Scales During the Past Two Millennia</atitle><jtitle>Global biogeochemical cycles</jtitle><date>2020-09</date><risdate>2020</risdate><volume>34</volume><issue>9</issue><epage>n/a</epage><issn>0886-6236</issn><eissn>1944-9224</eissn><eissn>1944-8224</eissn><abstract>The continuous growth of atmospheric nitrous oxide (N2O) is of concern for its potential role in global warming and future stratospheric ozone destruction. Climate feedbacks that enhance N2O emissions in response to global warming are not well understood, and past records of N2O from ice cores are not sufficiently well resolved to examine the underlying climate‐N2O feedbacks on societally relevant time scales. Here, we present a new high‐resolution and high‐precision N2O reconstruction obtained from the Greenland NEEM (North Greenland Eemian Ice Drilling) and the Antarctic Styx Glacier ice cores. Covering the N2O history of the past two millennia, our reconstruction shows a centennial‐scale variability of ~10 ppb. A pronounced minimum at ~600 CE coincides with the reorganizations of tropical hydroclimate and ocean productivity changes. Comparisons with proxy records suggest association of centennial‐ to millennial‐scale variations in N2O with changes in tropical and subtropical land hydrology and marine productivity. Plain Language Summary Nitrous oxide (N2O) is a greenhouse and ozone‐depleting gas. The growing level of N2O in the atmosphere is of global concern, and records of past N2O variations can provide an important context for understanding the links between N2O and climate change. In this study, we report new, high‐quality N2O records covering the last two millennia using ice cores obtained from Greenland and Antarctica. Our N2O records show rapid centennial‐scale changes in atmospheric N2O and confirm a pronounced minimum near 600 CE. Comparison with climate records suggests that hydroclimate change on land and changes in marine productivity contribute to centennial‐ to millennial‐scale N2O variations. Key Points We report records of N2O concentration for the last 2,000 yr from the Styx ice core in Antarctca and NEEM ice core in Greenland The data accurately reveal the timing and magnitude of N2O variations on centennial time scales Variations in N2O are associated with changes in tropical and subtropical land hydrology and marine productivity</abstract><cop>Washington</cop><pub>Blackwell Publishing Ltd</pub><doi>10.1029/2020GB006568</doi><tpages>10</tpages><orcidid>https://orcid.org/0000-0002-6232-8082</orcidid><orcidid>https://orcid.org/0000-0003-2280-2832</orcidid><orcidid>https://orcid.org/0000-0001-8397-9274</orcidid><orcidid>https://orcid.org/0000-0001-5438-0115</orcidid><orcidid>https://orcid.org/0000-0002-6065-7747</orcidid><orcidid>https://orcid.org/0000-0002-3509-8082</orcidid><oa>free_for_read</oa></addata></record>
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subjects Antarctic glaciers
Climate change
Cores
Drilling
Glacier ice
Glaciers
Global warming
Hydroclimate
Hydrology
Ice
ice core
Ice cores
Neem
Nitrous oxide
Ocean, Atmosphere
Ozone
Ozone depletion
Ozone destruction
paleoclimate
Productivity
Reconstruction
Records
Sciences of the Universe
Stratospheric warming
Time
Tropical climate
Variation
title Atmospheric Nitrous Oxide Variations on Centennial Time Scales During the Past Two Millennia
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