Single-size thermometric measurements on a size distribution of neutral fullerenes

Single-size thermometric measurements on a size distribution of neutral fullerenes

We present measurements of the velocity distribution of electrons emitted from mass-selected neutral fullerenes, performed at the intracavity free electron laser FELICE. We make use of mass-specific vibrational resonances in the infrared domain to selectively heat up one out of a distribution of sev...

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Veröffentlicht in:Physical review letters 2013-05, Vol.110 (19), p.193401-193401, Article 193401
Hauptverfasser: Cauchy, C, Bakker, J M, Huismans, Y, Rouzée, A, Redlich, B, van der Meer, A F G, Bordas, C, Vrakking, M J J, Lépine, F
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container_end_page 193401
container_issue 19
container_start_page 193401
container_title Physical review letters
container_volume 110
creator Cauchy, C
Bakker, J M
Huismans, Y
Rouzée, A
Redlich, B
van der Meer, A F G
Bordas, C
Vrakking, M J J
Lépine, F
description We present measurements of the velocity distribution of electrons emitted from mass-selected neutral fullerenes, performed at the intracavity free electron laser FELICE. We make use of mass-specific vibrational resonances in the infrared domain to selectively heat up one out of a distribution of several fullerene species. Efficient energy redistribution leads to decay via thermionic emission. Time-resolved electron kinetic energy distributions measured give information on the decay rate of the selected fullerene. This method is generally applicable to all neutral species that exhibit thermionic emission and provides a unique tool to study the stability of mass-selected neutral clusters and molecules that are only available as part of a size distribution.
doi_str_mv 10.1103/PhysRevLett.110.193401
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Engineering Sciences
Physics
title Single-size thermometric measurements on a size distribution of neutral fullerenes
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