Upcycling of Vine Shoots: Production of Fillers for PHBV-Based Biocomposite Applications
This paper aims at investigating the potential of vine shoots (ViSh) upcycling as fillers in novel poly(3-hydroxybutyrate-3-hydroxyvalerate) (PHBV) based biocomposites. ViSh particles of around 50 µm (apparent median diameter) were obtained combining dry grinding processes, and mixed with PHBV using...
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| Veröffentlicht in: | Journal of polymers and the environment 2021-02, Vol.29 (2), p.404-417 |
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| container_title | Journal of polymers and the environment |
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| creator | David, Grégoire Heux, Laurent Pradeau, Stéphanie Gontard, Nathalie Angellier-Coussy, Hélène |
| description | This paper aims at investigating the potential of vine shoots (ViSh) upcycling as fillers in novel poly(3-hydroxybutyrate-3-hydroxyvalerate) (PHBV) based biocomposites. ViSh particles of around 50 µm (apparent median diameter) were obtained combining dry grinding processes, and mixed with PHBV using melt extrusion. Thermal stability and elongation at break of biocomposites were reduced with increasing contents of ViSh particles (10, 20 and 30 wt%), while Young’s modulus and water vapor permeability were increased. It was shown that a surface gas-phase esterification allowed to significantly increase the hydrophobicity of ViSh particles (increase of water contact angles from 59° to 114°), leading to a reduction of 27% in the water vapor permeability of the biocomposite filled with 30 wt% of ViSh. The overall mechanical performance was not impacted by gas-phase esterification, demonstrating that the interfacial adhesion between the virgin ViSh particles and the PHBV matrix was already good and that such filler surface treatment was not required in that case. It was concluded that ViSh particles can be interestingly used as low cost fillers in PHBV-based biocomposites to decrease the overall cost of materials. |
| doi_str_mv | 10.1007/s10924-020-01884-8 |
| format | Article |
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ViSh particles of around 50 µm (apparent median diameter) were obtained combining dry grinding processes, and mixed with PHBV using melt extrusion. Thermal stability and elongation at break of biocomposites were reduced with increasing contents of ViSh particles (10, 20 and 30 wt%), while Young’s modulus and water vapor permeability were increased. It was shown that a surface gas-phase esterification allowed to significantly increase the hydrophobicity of ViSh particles (increase of water contact angles from 59° to 114°), leading to a reduction of 27% in the water vapor permeability of the biocomposite filled with 30 wt% of ViSh. The overall mechanical performance was not impacted by gas-phase esterification, demonstrating that the interfacial adhesion between the virgin ViSh particles and the PHBV matrix was already good and that such filler surface treatment was not required in that case. It was concluded that ViSh particles can be interestingly used as low cost fillers in PHBV-based biocomposites to decrease the overall cost of materials.</description><identifier>ISSN: 1566-2543</identifier><identifier>EISSN: 1572-8919</identifier><identifier>EISSN: 1572-8900</identifier><identifier>DOI: 10.1007/s10924-020-01884-8</identifier><language>eng</language><publisher>New York: Springer US</publisher><subject>Biomedical materials ; Chemistry ; Chemistry and Materials Science ; Composite materials ; Contact angle ; Dry grinding ; Elongation ; Environmental Chemistry ; Environmental Engineering/Biotechnology ; Esterification ; Extrusion ; Fillers ; Food engineering ; Hydrophobicity ; Industrial Chemistry/Chemical Engineering ; Life Sciences ; Materials Science ; Mechanical properties ; Modulus of elasticity ; Original Paper ; Permeability ; Polymer Sciences ; Surface treatment ; Thermal stability ; Water vapor</subject><ispartof>Journal of polymers and the environment, 2021-02, Vol.29 (2), p.404-417</ispartof><rights>The Author(s) 2020</rights><rights>The Author(s) 2020. 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ViSh particles of around 50 µm (apparent median diameter) were obtained combining dry grinding processes, and mixed with PHBV using melt extrusion. Thermal stability and elongation at break of biocomposites were reduced with increasing contents of ViSh particles (10, 20 and 30 wt%), while Young’s modulus and water vapor permeability were increased. It was shown that a surface gas-phase esterification allowed to significantly increase the hydrophobicity of ViSh particles (increase of water contact angles from 59° to 114°), leading to a reduction of 27% in the water vapor permeability of the biocomposite filled with 30 wt% of ViSh. The overall mechanical performance was not impacted by gas-phase esterification, demonstrating that the interfacial adhesion between the virgin ViSh particles and the PHBV matrix was already good and that such filler surface treatment was not required in that case. 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| subjects | Biomedical materials Chemistry Chemistry and Materials Science Composite materials Contact angle Dry grinding Elongation Environmental Chemistry Environmental Engineering/Biotechnology Esterification Extrusion Fillers Food engineering Hydrophobicity Industrial Chemistry/Chemical Engineering Life Sciences Materials Science Mechanical properties Modulus of elasticity Original Paper Permeability Polymer Sciences Surface treatment Thermal stability Water vapor |
| title | Upcycling of Vine Shoots: Production of Fillers for PHBV-Based Biocomposite Applications |
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