Assessment of AlGaN/AlN superlattices on GaN nanowires as active region of electron-pumped ultraviolet sources
In this paper, we describe the design and characterization of 400 nm long (88 periods) Al Ga N/AlN (0 ≤ x ≤ 0.1) quantum dot superlattices deposited on self-assembled GaN nanowires for application in electron-pumped ultraviolet sources. The optical performance of GaN/AlN superlattices on nanowires i...
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Veröffentlicht in: | Nanotechnology 2020-05, Vol.31 (20), p.204001-204001 |
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creator | Dimkou, I Harikumar, A Donatini, F Lähnemann, J den Hertog, M I Bougerol, C Bellet-Amalric, E Mollard, N Ajay, A Ledoux, G Purcell, S T Monroy, E |
description | In this paper, we describe the design and characterization of 400 nm long (88 periods) Al
Ga
N/AlN (0 ≤ x ≤ 0.1) quantum dot superlattices deposited on self-assembled GaN nanowires for application in electron-pumped ultraviolet sources. The optical performance of GaN/AlN superlattices on nanowires is compared with the emission of planar GaN/AlN superlattices with the same periodicity and thickness grown on bulk GaN substrates along the N-polar and metal-polar crystallographic axes. The nanowire samples are less sensitive to nonradiative recombination than planar layers, attaining internal quantum efficiencies (IQE) in excess of 60% at room temperature even under low injection conditions. The IQE remains stable for higher excitation power densities, up to 50 kW cm
. We demonstrate that the nanowire superlattice is long enough to collect the electron-hole pairs generated by an electron beam with an acceleration voltage V
= 5 kV. At such V
, the light emitted from the nanowire ensemble does not show any sign of quenching under constant electron beam excitation (tested for an excitation power density around 8 kW cm
over the scale of minutes). Varying the dot/barrier thickness ratio and the Al content in the dots, the nanowire peak emission can be tuned in the range from 340 to 258 nm. |
doi_str_mv | 10.1088/1361-6528/ab704d |
format | Article |
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Ga
N/AlN (0 ≤ x ≤ 0.1) quantum dot superlattices deposited on self-assembled GaN nanowires for application in electron-pumped ultraviolet sources. The optical performance of GaN/AlN superlattices on nanowires is compared with the emission of planar GaN/AlN superlattices with the same periodicity and thickness grown on bulk GaN substrates along the N-polar and metal-polar crystallographic axes. The nanowire samples are less sensitive to nonradiative recombination than planar layers, attaining internal quantum efficiencies (IQE) in excess of 60% at room temperature even under low injection conditions. The IQE remains stable for higher excitation power densities, up to 50 kW cm
. We demonstrate that the nanowire superlattice is long enough to collect the electron-hole pairs generated by an electron beam with an acceleration voltage V
= 5 kV. At such V
, the light emitted from the nanowire ensemble does not show any sign of quenching under constant electron beam excitation (tested for an excitation power density around 8 kW cm
over the scale of minutes). Varying the dot/barrier thickness ratio and the Al content in the dots, the nanowire peak emission can be tuned in the range from 340 to 258 nm.</description><identifier>ISSN: 0957-4484</identifier><identifier>EISSN: 1361-6528</identifier><identifier>DOI: 10.1088/1361-6528/ab704d</identifier><identifier>PMID: 31986502</identifier><language>eng</language><publisher>England: Institute of Physics</publisher><subject>Chemical Sciences ; Engineering Sciences ; Physics</subject><ispartof>Nanotechnology, 2020-05, Vol.31 (20), p.204001-204001</ispartof><rights>Distributed under a Creative Commons Attribution 4.0 International License</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c333t-5f4d980daf6a77abc72ebfcb1b44b644cca2615b42a042ff66d2f7b010ad6ae83</citedby><cites>FETCH-LOGICAL-c333t-5f4d980daf6a77abc72ebfcb1b44b644cca2615b42a042ff66d2f7b010ad6ae83</cites><orcidid>0000-0001-5481-3267 ; 0000-0003-0781-9249 ; 0000-0002-6865-3820 ; 0000-0001-5738-5093 ; 0000-0003-4072-2369 ; 0000-0001-6556-1683 ; 0000-0002-4823-0919 ; 0000-0003-2977-1725 ; 0000-0002-0867-1285</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>230,314,776,780,881,27903,27904</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/31986502$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink><backlink>$$Uhttps://hal.science/hal-02869555$$DView record in HAL$$Hfree_for_read</backlink></links><search><creatorcontrib>Dimkou, I</creatorcontrib><creatorcontrib>Harikumar, A</creatorcontrib><creatorcontrib>Donatini, F</creatorcontrib><creatorcontrib>Lähnemann, J</creatorcontrib><creatorcontrib>den Hertog, M I</creatorcontrib><creatorcontrib>Bougerol, C</creatorcontrib><creatorcontrib>Bellet-Amalric, E</creatorcontrib><creatorcontrib>Mollard, N</creatorcontrib><creatorcontrib>Ajay, A</creatorcontrib><creatorcontrib>Ledoux, G</creatorcontrib><creatorcontrib>Purcell, S T</creatorcontrib><creatorcontrib>Monroy, E</creatorcontrib><title>Assessment of AlGaN/AlN superlattices on GaN nanowires as active region of electron-pumped ultraviolet sources</title><title>Nanotechnology</title><addtitle>Nanotechnology</addtitle><description>In this paper, we describe the design and characterization of 400 nm long (88 periods) Al
Ga
N/AlN (0 ≤ x ≤ 0.1) quantum dot superlattices deposited on self-assembled GaN nanowires for application in electron-pumped ultraviolet sources. The optical performance of GaN/AlN superlattices on nanowires is compared with the emission of planar GaN/AlN superlattices with the same periodicity and thickness grown on bulk GaN substrates along the N-polar and metal-polar crystallographic axes. The nanowire samples are less sensitive to nonradiative recombination than planar layers, attaining internal quantum efficiencies (IQE) in excess of 60% at room temperature even under low injection conditions. The IQE remains stable for higher excitation power densities, up to 50 kW cm
. We demonstrate that the nanowire superlattice is long enough to collect the electron-hole pairs generated by an electron beam with an acceleration voltage V
= 5 kV. At such V
, the light emitted from the nanowire ensemble does not show any sign of quenching under constant electron beam excitation (tested for an excitation power density around 8 kW cm
over the scale of minutes). Varying the dot/barrier thickness ratio and the Al content in the dots, the nanowire peak emission can be tuned in the range from 340 to 258 nm.</description><subject>Chemical Sciences</subject><subject>Engineering Sciences</subject><subject>Physics</subject><issn>0957-4484</issn><issn>1361-6528</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2020</creationdate><recordtype>article</recordtype><recordid>eNo9Uc-L1DAUDqK44-rdk_SohzpJmqSZY1l0VxjWi57DS_qilbSpSTrif2-GWQcePPh-Hb6PkLeMfmRU6z3rFGuV5HoPtqdifEZ2V-g52dGD7FshtLghr3L-RSljmrOX5KZjB60k5TuyDDljzjMupYm-GcI9PO6H8NjkbcUUoJTJYW7i0lSiWWCJf6ZUAajnynTCJuGPqdLVjAFdSXFp121ecWy2UBKcphiwNDluqQa9Ji88hIxvnv4t-f7507e7h_b49f7L3XBsXdd1pZVejAdNR_AK-h6s6zla7yyzQlglhHPAFZNWcKCCe6_UyH1vKaMwKkDd3ZIPl9yfEMyaphnSXxNhMg_D0ZwxyrU6SClPrGrfX7Rrir83zMXMU3YYAiwYt2x4J3rJqOxpldKL1KWYc0J_zWbUnBcx5_rNuX5zWaRa3j2lb3bG8Wr4P0H3D-C2iDo</recordid><startdate>20200515</startdate><enddate>20200515</enddate><creator>Dimkou, I</creator><creator>Harikumar, A</creator><creator>Donatini, F</creator><creator>Lähnemann, J</creator><creator>den Hertog, M I</creator><creator>Bougerol, C</creator><creator>Bellet-Amalric, E</creator><creator>Mollard, N</creator><creator>Ajay, A</creator><creator>Ledoux, G</creator><creator>Purcell, S T</creator><creator>Monroy, E</creator><general>Institute of Physics</general><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7X8</scope><scope>1XC</scope><scope>VOOES</scope><orcidid>https://orcid.org/0000-0001-5481-3267</orcidid><orcidid>https://orcid.org/0000-0003-0781-9249</orcidid><orcidid>https://orcid.org/0000-0002-6865-3820</orcidid><orcidid>https://orcid.org/0000-0001-5738-5093</orcidid><orcidid>https://orcid.org/0000-0003-4072-2369</orcidid><orcidid>https://orcid.org/0000-0001-6556-1683</orcidid><orcidid>https://orcid.org/0000-0002-4823-0919</orcidid><orcidid>https://orcid.org/0000-0003-2977-1725</orcidid><orcidid>https://orcid.org/0000-0002-0867-1285</orcidid></search><sort><creationdate>20200515</creationdate><title>Assessment of AlGaN/AlN superlattices on GaN nanowires as active region of electron-pumped ultraviolet sources</title><author>Dimkou, I ; Harikumar, A ; Donatini, F ; Lähnemann, J ; den Hertog, M I ; Bougerol, C ; Bellet-Amalric, E ; Mollard, N ; Ajay, A ; Ledoux, G ; Purcell, S T ; Monroy, E</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c333t-5f4d980daf6a77abc72ebfcb1b44b644cca2615b42a042ff66d2f7b010ad6ae83</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2020</creationdate><topic>Chemical Sciences</topic><topic>Engineering Sciences</topic><topic>Physics</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Dimkou, I</creatorcontrib><creatorcontrib>Harikumar, A</creatorcontrib><creatorcontrib>Donatini, F</creatorcontrib><creatorcontrib>Lähnemann, J</creatorcontrib><creatorcontrib>den Hertog, M I</creatorcontrib><creatorcontrib>Bougerol, C</creatorcontrib><creatorcontrib>Bellet-Amalric, E</creatorcontrib><creatorcontrib>Mollard, N</creatorcontrib><creatorcontrib>Ajay, A</creatorcontrib><creatorcontrib>Ledoux, G</creatorcontrib><creatorcontrib>Purcell, S T</creatorcontrib><creatorcontrib>Monroy, E</creatorcontrib><collection>PubMed</collection><collection>CrossRef</collection><collection>MEDLINE - Academic</collection><collection>Hyper Article en Ligne (HAL)</collection><collection>Hyper Article en Ligne (HAL) (Open Access)</collection><jtitle>Nanotechnology</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Dimkou, I</au><au>Harikumar, A</au><au>Donatini, F</au><au>Lähnemann, J</au><au>den Hertog, M I</au><au>Bougerol, C</au><au>Bellet-Amalric, E</au><au>Mollard, N</au><au>Ajay, A</au><au>Ledoux, G</au><au>Purcell, S T</au><au>Monroy, E</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Assessment of AlGaN/AlN superlattices on GaN nanowires as active region of electron-pumped ultraviolet sources</atitle><jtitle>Nanotechnology</jtitle><addtitle>Nanotechnology</addtitle><date>2020-05-15</date><risdate>2020</risdate><volume>31</volume><issue>20</issue><spage>204001</spage><epage>204001</epage><pages>204001-204001</pages><issn>0957-4484</issn><eissn>1361-6528</eissn><abstract>In this paper, we describe the design and characterization of 400 nm long (88 periods) Al
Ga
N/AlN (0 ≤ x ≤ 0.1) quantum dot superlattices deposited on self-assembled GaN nanowires for application in electron-pumped ultraviolet sources. The optical performance of GaN/AlN superlattices on nanowires is compared with the emission of planar GaN/AlN superlattices with the same periodicity and thickness grown on bulk GaN substrates along the N-polar and metal-polar crystallographic axes. The nanowire samples are less sensitive to nonradiative recombination than planar layers, attaining internal quantum efficiencies (IQE) in excess of 60% at room temperature even under low injection conditions. The IQE remains stable for higher excitation power densities, up to 50 kW cm
. We demonstrate that the nanowire superlattice is long enough to collect the electron-hole pairs generated by an electron beam with an acceleration voltage V
= 5 kV. At such V
, the light emitted from the nanowire ensemble does not show any sign of quenching under constant electron beam excitation (tested for an excitation power density around 8 kW cm
over the scale of minutes). Varying the dot/barrier thickness ratio and the Al content in the dots, the nanowire peak emission can be tuned in the range from 340 to 258 nm.</abstract><cop>England</cop><pub>Institute of Physics</pub><pmid>31986502</pmid><doi>10.1088/1361-6528/ab704d</doi><tpages>1</tpages><orcidid>https://orcid.org/0000-0001-5481-3267</orcidid><orcidid>https://orcid.org/0000-0003-0781-9249</orcidid><orcidid>https://orcid.org/0000-0002-6865-3820</orcidid><orcidid>https://orcid.org/0000-0001-5738-5093</orcidid><orcidid>https://orcid.org/0000-0003-4072-2369</orcidid><orcidid>https://orcid.org/0000-0001-6556-1683</orcidid><orcidid>https://orcid.org/0000-0002-4823-0919</orcidid><orcidid>https://orcid.org/0000-0003-2977-1725</orcidid><orcidid>https://orcid.org/0000-0002-0867-1285</orcidid><oa>free_for_read</oa></addata></record> |
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title | Assessment of AlGaN/AlN superlattices on GaN nanowires as active region of electron-pumped ultraviolet sources |
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