Determination of Oxygen Diffusion and Surface Exchange Coefficients of Mixed Ionic-Electronic Conductors by Oxygen Semi-Permeation Methods

Determination of Oxygen Diffusion and Surface Exchange Coefficients of Mixed Ionic-Electronic Conductors by Oxygen Semi-Permeation Methods

The understanding of oxygen transport mechanisms through mixed ionic-electronic conductors is of great interest for the development of electrochemical devices at high temperature for energy conversion applications. This study is focused on the determination of two coefficients-the oxygen diffusion c...

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Veröffentlicht in:Journal of the Electrochemical Society 2020-03, Vol.167 (6), p.64503
Hauptverfasser: Geffroy, Pierre-Marie, Deronzier, Eva, Gillibert, Jean, Munch, Pascal, Chartier, Thierry, Fouletier, Jacques
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Engineering Sciences
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Mechanics of materials
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container_issue 6
container_start_page 64503
container_title Journal of the Electrochemical Society
container_volume 167
creator Geffroy, Pierre-Marie
Deronzier, Eva
Gillibert, Jean
Munch, Pascal
Chartier, Thierry
Fouletier, Jacques
description The understanding of oxygen transport mechanisms through mixed ionic-electronic conductors is of great interest for the development of electrochemical devices at high temperature for energy conversion applications. This study is focused on the determination of two coefficients-the oxygen diffusion coefficient and the surface exchange coefficient which are key parameters for the electrochemical performance of a material. These coefficients can be largely impacted by the measurement conditions. The oxygen semi-permeation method is an adequate method to determine these two fundamental coefficients close to the working conditions of the material, i.e., under small or large oxygen partial pressure gradients.
doi_str_mv 10.1149/1945-7111/ab7b84
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Mechanics
Mechanics of materials
title Determination of Oxygen Diffusion and Surface Exchange Coefficients of Mixed Ionic-Electronic Conductors by Oxygen Semi-Permeation Methods
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