A High-Temperature Single-Photon Source from Nanowire Quantum Dots

We present a high-temperature single-photon source based on a quantum dot inside a nanowire. The nanowires were grown by molecular beam epitaxy in the vapor−liquid−solid growth mode. We utilize a two-step process that allows a thin, defect-free ZnSe nanowire to grow on top of a broader, cone-shaped...

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Veröffentlicht in:Nano letters 2008-12, Vol.8 (12), p.4326-4329
Hauptverfasser: Tribu, Adrien, Sallen, Gregory, Aichele, Thomas, André, Régis, Poizat, Jean-Philippe, Bougerol, Catherine, Tatarenko, Serge, Kheng, Kuntheak
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container_end_page 4329
container_issue 12
container_start_page 4326
container_title Nano letters
container_volume 8
creator Tribu, Adrien
Sallen, Gregory
Aichele, Thomas
André, Régis
Poizat, Jean-Philippe
Bougerol, Catherine
Tatarenko, Serge
Kheng, Kuntheak
description We present a high-temperature single-photon source based on a quantum dot inside a nanowire. The nanowires were grown by molecular beam epitaxy in the vapor−liquid−solid growth mode. We utilize a two-step process that allows a thin, defect-free ZnSe nanowire to grow on top of a broader, cone-shaped nanowire. Quantum dots are formed by incorporating a narrow zone of CdSe into the nanowire. We observe intense and highly polarized photoluminescence even from a single emitter. Efficient photon antibunching is observed up to 220 K, while conserving a normalized antibunching dip of at most 36%. This is the highest reported temperature for single-photon emission from a nonblinking quantum-dot source and principally allows compact and cheap operation by using Peltier cooling.
doi_str_mv 10.1021/nl802160z
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subjects Applied sciences
Cross-disciplinary physics: materials science
rheology
Electronics
Exact sciences and technology
Materials science
Molecular electronics, nanoelectronics
Nanocrystalline materials
Nanoscale materials and structures: fabrication and characterization
Physics
Quantum dots
Quantum wires
Semiconductor electronics. Microelectronics. Optoelectronics. Solid state devices
title A High-Temperature Single-Photon Source from Nanowire Quantum Dots
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