Influence of Two-Photon Absorption Anisotropy on Terahertz Emission Through Optical Rectification in Zinc-Blende Crystals
We report for the first time on the observation of an angular anisotropy of the THz signal generated by optical rectification in a < 111 > ZnTe crystal. This cubic (zinc-blende) crystal in the orientation exhibits both transverse isotropy for optical effects involving the linear χ (1) and non...
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Veröffentlicht in: | Journal of infrared, millimeter and terahertz waves millimeter and terahertz waves, 2018-04, Vol.39 (4), p.378-386 |
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container_title | Journal of infrared, millimeter and terahertz waves |
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creator | Sanjuan, Federico Gaborit, Gwenaël Coutaz, Jean-Louis |
description | We report for the first time on the observation of an angular anisotropy of the THz signal generated by optical rectification in a < 111 > ZnTe crystal. This cubic (zinc-blende) crystal in the orientation exhibits both transverse isotropy for optical effects involving the linear
χ
(1)
and nonlinear
χ
(2)
susceptibilities. Thus, the observed anisotropy can only be related to
χ
(3)
effect, namely two-photon absorption, which leads to the photo-generation of free carriers that absorb the generated THz signal. Two-photon absorption in zinc-blende crystals is known to be due to a spin-orbit interaction between the valence and higher-conduction bands. We perform a couple of measurements that confirm our hypothesis, as well as we fit the recorded data with a simple model. This two-photon absorption effect makes difficult an efficient generation, through optical rectification in zinc-blende crystals, of THz beams of any given polarization state by only monitoring the laser pump polarization. |
doi_str_mv | 10.1007/s10762-018-0468-4 |
format | Article |
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χ
(1)
and nonlinear
χ
(2)
susceptibilities. Thus, the observed anisotropy can only be related to
χ
(3)
effect, namely two-photon absorption, which leads to the photo-generation of free carriers that absorb the generated THz signal. Two-photon absorption in zinc-blende crystals is known to be due to a spin-orbit interaction between the valence and higher-conduction bands. We perform a couple of measurements that confirm our hypothesis, as well as we fit the recorded data with a simple model. This two-photon absorption effect makes difficult an efficient generation, through optical rectification in < 111 > zinc-blende crystals, of THz beams of any given polarization state by only monitoring the laser pump polarization.</description><identifier>ISSN: 1866-6892</identifier><identifier>EISSN: 1866-6906</identifier><identifier>DOI: 10.1007/s10762-018-0468-4</identifier><language>eng</language><publisher>New York: Springer US</publisher><subject>Anisotropy ; Classical Electrodynamics ; Conduction bands ; Crystal structure ; Electrical Engineering ; Electromagnetism ; Electronics and Microelectronics ; Engineering ; Engineering Sciences ; Instrumentation ; Isotropy ; Laser beams ; Optical communication ; Optics ; Photon absorption ; Photonic ; Photons ; Physics ; Plasmas ; Polarization ; Spin-orbit interactions ; Zinc tellurides ; Zincblende</subject><ispartof>Journal of infrared, millimeter and terahertz waves, 2018-04, Vol.39 (4), p.378-386</ispartof><rights>Springer Science+Business Media, LLC, part of Springer Nature 2018</rights><rights>Copyright Springer Science & Business Media 2018</rights><rights>Journal of Infrared, Millimeter, and Terahertz Waves is a copyright of Springer, (2018). All Rights Reserved.</rights><rights>Distributed under a Creative Commons Attribution 4.0 International License</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c378t-52b26c4d5a3c5b266843e6a4075907ada471941a187a1aa8caaa782ddd0aabd53</citedby><cites>FETCH-LOGICAL-c378t-52b26c4d5a3c5b266843e6a4075907ada471941a187a1aa8caaa782ddd0aabd53</cites><orcidid>0000-0001-7688-6424 ; 0000-0001-9982-7910 ; 0000-0002-0810-3333</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s10762-018-0468-4$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s10762-018-0468-4$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>230,314,780,784,885,27923,27924,41487,42556,51318</link.rule.ids><backlink>$$Uhttps://hal.univ-grenoble-alpes.fr/hal-01996340$$DView record in HAL$$Hfree_for_read</backlink></links><search><creatorcontrib>Sanjuan, Federico</creatorcontrib><creatorcontrib>Gaborit, Gwenaël</creatorcontrib><creatorcontrib>Coutaz, Jean-Louis</creatorcontrib><title>Influence of Two-Photon Absorption Anisotropy on Terahertz Emission Through Optical Rectification in Zinc-Blende Crystals</title><title>Journal of infrared, millimeter and terahertz waves</title><addtitle>J Infrared Milli Terahz Waves</addtitle><description>We report for the first time on the observation of an angular anisotropy of the THz signal generated by optical rectification in a < 111 > ZnTe crystal. This cubic (zinc-blende) crystal in the < 111 > orientation exhibits both transverse isotropy for optical effects involving the linear
χ
(1)
and nonlinear
χ
(2)
susceptibilities. Thus, the observed anisotropy can only be related to
χ
(3)
effect, namely two-photon absorption, which leads to the photo-generation of free carriers that absorb the generated THz signal. Two-photon absorption in zinc-blende crystals is known to be due to a spin-orbit interaction between the valence and higher-conduction bands. We perform a couple of measurements that confirm our hypothesis, as well as we fit the recorded data with a simple model. This two-photon absorption effect makes difficult an efficient generation, through optical rectification in < 111 > zinc-blende crystals, of THz beams of any given polarization state by only monitoring the laser pump polarization.</description><subject>Anisotropy</subject><subject>Classical Electrodynamics</subject><subject>Conduction bands</subject><subject>Crystal structure</subject><subject>Electrical Engineering</subject><subject>Electromagnetism</subject><subject>Electronics and Microelectronics</subject><subject>Engineering</subject><subject>Engineering Sciences</subject><subject>Instrumentation</subject><subject>Isotropy</subject><subject>Laser beams</subject><subject>Optical communication</subject><subject>Optics</subject><subject>Photon absorption</subject><subject>Photonic</subject><subject>Photons</subject><subject>Physics</subject><subject>Plasmas</subject><subject>Polarization</subject><subject>Spin-orbit interactions</subject><subject>Zinc tellurides</subject><subject>Zincblende</subject><issn>1866-6892</issn><issn>1866-6906</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2018</creationdate><recordtype>article</recordtype><sourceid>AFKRA</sourceid><sourceid>BENPR</sourceid><sourceid>CCPQU</sourceid><sourceid>DWQXO</sourceid><recordid>eNp9kU1v1DAQhiNEJUrLD-BmiRMHl7Hj-OO4rFpaaaUitFy4WLOO06RK7cXOtlp-fR3CxwlO887oeWdGeqvqLYMLBqA-ZAZKcgpMUxBSU_GiOmVaSioNyJe_tTb8VfU653sAKYSRp9XxJnTjwQfnSezI9inSz32cYiCrXY5pPw2zDEOOU4r7Iynd1ifsfZp-kMuHIecZ2PYpHu56clt4hyP54t00dEX-tA-BfBuCox9HH1pP1umYJxzzeXXSleLf_Kpn1dery-36mm5uP92sVxvqaqUn2vAdl060DdauKVJqUXuJAlRjQGGLQjEjGDKtkCFqh4hK87ZtAXHXNvVZ9X7Z2-No92l4wHS0EQd7vdrYeQbMGFkLeGSFfbew-xS_H3ye7H08pFDes5w3RimQIP9LARgpuFKiUGyhXIo5J9_9Oc7AzpnZJbNyX9s5Mzt7-OLJhQ13Pv3d_G_TM-BmmYw</recordid><startdate>20180401</startdate><enddate>20180401</enddate><creator>Sanjuan, Federico</creator><creator>Gaborit, Gwenaël</creator><creator>Coutaz, Jean-Louis</creator><general>Springer US</general><general>Springer Nature B.V</general><general>Springer Verlag</general><scope>AAYXX</scope><scope>CITATION</scope><scope>8FE</scope><scope>8FG</scope><scope>AFKRA</scope><scope>ARAPS</scope><scope>BENPR</scope><scope>BGLVJ</scope><scope>CCPQU</scope><scope>DWQXO</scope><scope>HCIFZ</scope><scope>P5Z</scope><scope>P62</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>1XC</scope><orcidid>https://orcid.org/0000-0001-7688-6424</orcidid><orcidid>https://orcid.org/0000-0001-9982-7910</orcidid><orcidid>https://orcid.org/0000-0002-0810-3333</orcidid></search><sort><creationdate>20180401</creationdate><title>Influence of Two-Photon Absorption Anisotropy on Terahertz Emission Through Optical Rectification in Zinc-Blende Crystals</title><author>Sanjuan, Federico ; Gaborit, Gwenaël ; Coutaz, Jean-Louis</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c378t-52b26c4d5a3c5b266843e6a4075907ada471941a187a1aa8caaa782ddd0aabd53</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2018</creationdate><topic>Anisotropy</topic><topic>Classical Electrodynamics</topic><topic>Conduction bands</topic><topic>Crystal structure</topic><topic>Electrical Engineering</topic><topic>Electromagnetism</topic><topic>Electronics and Microelectronics</topic><topic>Engineering</topic><topic>Engineering Sciences</topic><topic>Instrumentation</topic><topic>Isotropy</topic><topic>Laser beams</topic><topic>Optical communication</topic><topic>Optics</topic><topic>Photon absorption</topic><topic>Photonic</topic><topic>Photons</topic><topic>Physics</topic><topic>Plasmas</topic><topic>Polarization</topic><topic>Spin-orbit interactions</topic><topic>Zinc tellurides</topic><topic>Zincblende</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Sanjuan, Federico</creatorcontrib><creatorcontrib>Gaborit, Gwenaël</creatorcontrib><creatorcontrib>Coutaz, Jean-Louis</creatorcontrib><collection>CrossRef</collection><collection>ProQuest SciTech Collection</collection><collection>ProQuest Technology Collection</collection><collection>ProQuest Central UK/Ireland</collection><collection>Advanced Technologies & Aerospace Collection</collection><collection>ProQuest Central</collection><collection>Technology Collection</collection><collection>ProQuest One Community College</collection><collection>ProQuest Central Korea</collection><collection>SciTech Premium Collection</collection><collection>Advanced Technologies & Aerospace Database</collection><collection>ProQuest Advanced Technologies & Aerospace Collection</collection><collection>ProQuest One Academic Eastern Edition (DO NOT USE)</collection><collection>ProQuest One Academic</collection><collection>ProQuest One Academic UKI Edition</collection><collection>Hyper Article en Ligne (HAL)</collection><jtitle>Journal of infrared, millimeter and terahertz waves</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Sanjuan, Federico</au><au>Gaborit, Gwenaël</au><au>Coutaz, Jean-Louis</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Influence of Two-Photon Absorption Anisotropy on Terahertz Emission Through Optical Rectification in Zinc-Blende Crystals</atitle><jtitle>Journal of infrared, millimeter and terahertz waves</jtitle><stitle>J Infrared Milli Terahz Waves</stitle><date>2018-04-01</date><risdate>2018</risdate><volume>39</volume><issue>4</issue><spage>378</spage><epage>386</epage><pages>378-386</pages><issn>1866-6892</issn><eissn>1866-6906</eissn><abstract>We report for the first time on the observation of an angular anisotropy of the THz signal generated by optical rectification in a < 111 > ZnTe crystal. This cubic (zinc-blende) crystal in the < 111 > orientation exhibits both transverse isotropy for optical effects involving the linear
χ
(1)
and nonlinear
χ
(2)
susceptibilities. Thus, the observed anisotropy can only be related to
χ
(3)
effect, namely two-photon absorption, which leads to the photo-generation of free carriers that absorb the generated THz signal. Two-photon absorption in zinc-blende crystals is known to be due to a spin-orbit interaction between the valence and higher-conduction bands. We perform a couple of measurements that confirm our hypothesis, as well as we fit the recorded data with a simple model. This two-photon absorption effect makes difficult an efficient generation, through optical rectification in < 111 > zinc-blende crystals, of THz beams of any given polarization state by only monitoring the laser pump polarization.</abstract><cop>New York</cop><pub>Springer US</pub><doi>10.1007/s10762-018-0468-4</doi><tpages>9</tpages><orcidid>https://orcid.org/0000-0001-7688-6424</orcidid><orcidid>https://orcid.org/0000-0001-9982-7910</orcidid><orcidid>https://orcid.org/0000-0002-0810-3333</orcidid></addata></record> |
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subjects | Anisotropy Classical Electrodynamics Conduction bands Crystal structure Electrical Engineering Electromagnetism Electronics and Microelectronics Engineering Engineering Sciences Instrumentation Isotropy Laser beams Optical communication Optics Photon absorption Photonic Photons Physics Plasmas Polarization Spin-orbit interactions Zinc tellurides Zincblende |
title | Influence of Two-Photon Absorption Anisotropy on Terahertz Emission Through Optical Rectification in Zinc-Blende Crystals |
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