Mechanical response of gasoline soot nanoparticles under compression: An in situ TEM study
Gasoline soot nanoparticles (SNPs) were studied by performing in situ compression tests on individual nanoparticles inside a transmission electron microscope. After consecutive compressions, the SNPs exhibited an elasto-plastic behavior, and an increasing trend in Young's modulus and hardness v...
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Veröffentlicht in: | Tribology international 2019-03, Vol.131, p.446-453 |
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description | Gasoline soot nanoparticles (SNPs) were studied by performing in situ compression tests on individual nanoparticles inside a transmission electron microscope. After consecutive compressions, the SNPs exhibited an elasto-plastic behavior, and an increasing trend in Young's modulus and hardness values. Molecular dynamics were used to simulate compression cycles, the results of which confirmed the observations made during the experiments. The simulations were used to investigate how the different structural components of the nanoparticles affect their elastic and plastic response. By comparing the behavior of gasoline and diesel SNPs under compression, differences were observed both experimentally and in the simulations: the former were found to be more elastic and less prone to become hard under compression compared to the latter.
•Gasoline soot nanoparticles (SNP) show elasto-plastic behavior upon compression.•During consecutive compression their hardness shows an increasing tendency.•Gasoline and diesel SNPs exhibit different hardness and elasticity.•Molecular dynamics simulations confirm the experimental findings.•Different structural components affect the SNPs elastic and plastic behavior. |
doi_str_mv | 10.1016/j.triboint.2018.11.001 |
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•Gasoline soot nanoparticles (SNP) show elasto-plastic behavior upon compression.•During consecutive compression their hardness shows an increasing tendency.•Gasoline and diesel SNPs exhibit different hardness and elasticity.•Molecular dynamics simulations confirm the experimental findings.•Different structural components affect the SNPs elastic and plastic behavior.</description><identifier>ISSN: 0301-679X</identifier><identifier>EISSN: 1879-2464</identifier><identifier>DOI: 10.1016/j.triboint.2018.11.001</identifier><language>eng</language><publisher>Kidlington: Elsevier Ltd</publisher><subject>Compression ; Compression tests ; Engineering Sciences ; Gasoline ; In situ TEM ; Materials ; Mechanical analysis ; Modulus of elasticity ; Molecular dynamics ; Nanoparticles ; Simulation ; Soot ; Soot nanoparticle</subject><ispartof>Tribology international, 2019-03, Vol.131, p.446-453</ispartof><rights>2018 Elsevier Ltd</rights><rights>Copyright Elsevier BV Mar 2019</rights><rights>Distributed under a Creative Commons Attribution 4.0 International License</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c374t-1ed10c0d5e4e5328e22d5ebf22df112be450737d664e42f7ec9e75f43a23fcdc3</citedby><cites>FETCH-LOGICAL-c374t-1ed10c0d5e4e5328e22d5ebf22df112be450737d664e42f7ec9e75f43a23fcdc3</cites><orcidid>0000-0002-1210-5745</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktohtml>$$Uhttps://dx.doi.org/10.1016/j.triboint.2018.11.001$$EHTML$$P50$$Gelsevier$$H</linktohtml><link.rule.ids>230,314,780,784,885,3550,27924,27925,45995</link.rule.ids><backlink>$$Uhttps://hal.science/hal-01991814$$DView record in HAL$$Hfree_for_read</backlink></links><search><creatorcontrib>Jenei, Istvan Zoltan</creatorcontrib><creatorcontrib>Dassenoy, Fabrice</creatorcontrib><creatorcontrib>Epicier, Thierry</creatorcontrib><creatorcontrib>Khajeh, Arash</creatorcontrib><creatorcontrib>Martini, Ashlie</creatorcontrib><creatorcontrib>Uy, Dairene</creatorcontrib><creatorcontrib>Ghaednia, Hamed</creatorcontrib><creatorcontrib>Gangopadhyay, Arup</creatorcontrib><title>Mechanical response of gasoline soot nanoparticles under compression: An in situ TEM study</title><title>Tribology international</title><description>Gasoline soot nanoparticles (SNPs) were studied by performing in situ compression tests on individual nanoparticles inside a transmission electron microscope. After consecutive compressions, the SNPs exhibited an elasto-plastic behavior, and an increasing trend in Young's modulus and hardness values. Molecular dynamics were used to simulate compression cycles, the results of which confirmed the observations made during the experiments. The simulations were used to investigate how the different structural components of the nanoparticles affect their elastic and plastic response. By comparing the behavior of gasoline and diesel SNPs under compression, differences were observed both experimentally and in the simulations: the former were found to be more elastic and less prone to become hard under compression compared to the latter.
•Gasoline soot nanoparticles (SNP) show elasto-plastic behavior upon compression.•During consecutive compression their hardness shows an increasing tendency.•Gasoline and diesel SNPs exhibit different hardness and elasticity.•Molecular dynamics simulations confirm the experimental findings.•Different structural components affect the SNPs elastic and plastic behavior.</description><subject>Compression</subject><subject>Compression tests</subject><subject>Engineering Sciences</subject><subject>Gasoline</subject><subject>In situ TEM</subject><subject>Materials</subject><subject>Mechanical analysis</subject><subject>Modulus of elasticity</subject><subject>Molecular dynamics</subject><subject>Nanoparticles</subject><subject>Simulation</subject><subject>Soot</subject><subject>Soot nanoparticle</subject><issn>0301-679X</issn><issn>1879-2464</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2019</creationdate><recordtype>article</recordtype><recordid>eNqFkM1LxDAQxYMouH78CxLw5KE1k6ZN68lF1g9Y8aIgXkI2nWqWmtQkFfzv7bLq1dMbht97zDxCToDlwKA6X-cp2JW3LuWcQZ0D5IzBDplBLZuMi0rskhkrGGSVbJ73yUGMa8aYFI2ckZd7NG_aWaN7GjAO3kWkvqOvOvreOqTR-0Sddn7QIVnTY6SjazFQ49-HyRGtdxd07qh1NNo00sfFPY1pbL-OyF6n-4jHP3pInq4Xj1e32fLh5u5qvsxMIUXKAFtghrUlCiwLXiPn07zqJukA-ApFyWQh26oSKHgn0TQoy04UmhedaU1xSM62uW-6V0Ow7zp8Ka-tup0v1WbHoGmgBvEJE3u6ZYfgP0aMSa39GNx0nuJQs7oqpdxQ1ZYywccYsPuLBaY2nau1-u1cbTpXAGrqfDJebo04_ftpMahoLDqDrQ1okmq9_S_iGw7Ijm4</recordid><startdate>201903</startdate><enddate>201903</enddate><creator>Jenei, Istvan Zoltan</creator><creator>Dassenoy, Fabrice</creator><creator>Epicier, Thierry</creator><creator>Khajeh, Arash</creator><creator>Martini, Ashlie</creator><creator>Uy, Dairene</creator><creator>Ghaednia, Hamed</creator><creator>Gangopadhyay, Arup</creator><general>Elsevier Ltd</general><general>Elsevier BV</general><general>Elsevier</general><scope>AAYXX</scope><scope>CITATION</scope><scope>7SR</scope><scope>7TB</scope><scope>7U5</scope><scope>8BQ</scope><scope>8FD</scope><scope>F28</scope><scope>FR3</scope><scope>JG9</scope><scope>L7M</scope><scope>1XC</scope><orcidid>https://orcid.org/0000-0002-1210-5745</orcidid></search><sort><creationdate>201903</creationdate><title>Mechanical response of gasoline soot nanoparticles under compression: An in situ TEM study</title><author>Jenei, Istvan Zoltan ; Dassenoy, Fabrice ; Epicier, Thierry ; Khajeh, Arash ; Martini, Ashlie ; Uy, Dairene ; Ghaednia, Hamed ; Gangopadhyay, Arup</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c374t-1ed10c0d5e4e5328e22d5ebf22df112be450737d664e42f7ec9e75f43a23fcdc3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2019</creationdate><topic>Compression</topic><topic>Compression tests</topic><topic>Engineering Sciences</topic><topic>Gasoline</topic><topic>In situ TEM</topic><topic>Materials</topic><topic>Mechanical analysis</topic><topic>Modulus of elasticity</topic><topic>Molecular dynamics</topic><topic>Nanoparticles</topic><topic>Simulation</topic><topic>Soot</topic><topic>Soot nanoparticle</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Jenei, Istvan Zoltan</creatorcontrib><creatorcontrib>Dassenoy, Fabrice</creatorcontrib><creatorcontrib>Epicier, Thierry</creatorcontrib><creatorcontrib>Khajeh, Arash</creatorcontrib><creatorcontrib>Martini, Ashlie</creatorcontrib><creatorcontrib>Uy, Dairene</creatorcontrib><creatorcontrib>Ghaednia, Hamed</creatorcontrib><creatorcontrib>Gangopadhyay, Arup</creatorcontrib><collection>CrossRef</collection><collection>Engineered Materials Abstracts</collection><collection>Mechanical & Transportation Engineering Abstracts</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>ANTE: Abstracts in New Technology & Engineering</collection><collection>Engineering Research Database</collection><collection>Materials Research Database</collection><collection>Advanced Technologies Database with Aerospace</collection><collection>Hyper Article en Ligne (HAL)</collection><jtitle>Tribology international</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Jenei, Istvan Zoltan</au><au>Dassenoy, Fabrice</au><au>Epicier, Thierry</au><au>Khajeh, Arash</au><au>Martini, Ashlie</au><au>Uy, Dairene</au><au>Ghaednia, Hamed</au><au>Gangopadhyay, Arup</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Mechanical response of gasoline soot nanoparticles under compression: An in situ TEM study</atitle><jtitle>Tribology international</jtitle><date>2019-03</date><risdate>2019</risdate><volume>131</volume><spage>446</spage><epage>453</epage><pages>446-453</pages><issn>0301-679X</issn><eissn>1879-2464</eissn><abstract>Gasoline soot nanoparticles (SNPs) were studied by performing in situ compression tests on individual nanoparticles inside a transmission electron microscope. After consecutive compressions, the SNPs exhibited an elasto-plastic behavior, and an increasing trend in Young's modulus and hardness values. Molecular dynamics were used to simulate compression cycles, the results of which confirmed the observations made during the experiments. The simulations were used to investigate how the different structural components of the nanoparticles affect their elastic and plastic response. By comparing the behavior of gasoline and diesel SNPs under compression, differences were observed both experimentally and in the simulations: the former were found to be more elastic and less prone to become hard under compression compared to the latter.
•Gasoline soot nanoparticles (SNP) show elasto-plastic behavior upon compression.•During consecutive compression their hardness shows an increasing tendency.•Gasoline and diesel SNPs exhibit different hardness and elasticity.•Molecular dynamics simulations confirm the experimental findings.•Different structural components affect the SNPs elastic and plastic behavior.</abstract><cop>Kidlington</cop><pub>Elsevier Ltd</pub><doi>10.1016/j.triboint.2018.11.001</doi><tpages>8</tpages><orcidid>https://orcid.org/0000-0002-1210-5745</orcidid></addata></record> |
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subjects | Compression Compression tests Engineering Sciences Gasoline In situ TEM Materials Mechanical analysis Modulus of elasticity Molecular dynamics Nanoparticles Simulation Soot Soot nanoparticle |
title | Mechanical response of gasoline soot nanoparticles under compression: An in situ TEM study |
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