A study of xenon aggregates in uranium dioxide using X-ray absorption spectroscopy

X-ray absorption spectroscopy experiments were performed on a set of xenon implanted uranium dioxide samples. Results indicate that the gas forms highly pressurised inclusions as a result of temperature anneals or an external ion irradiation. Estimated bubble pressures were found to be in the region...

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Veröffentlicht in:Journal of nuclear materials 2006-06, Vol.352 (1-3), p.136-143
Hauptverfasser: Garcia, P., Martin, P., Carlot, G., Castelier, E., Ripert, M., Sabathier, C., Valot, C., D’Acapito, F., Hazemann, J-L., Proux, O., Nassif, V.
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container_end_page 143
container_issue 1-3
container_start_page 136
container_title Journal of nuclear materials
container_volume 352
creator Garcia, P.
Martin, P.
Carlot, G.
Castelier, E.
Ripert, M.
Sabathier, C.
Valot, C.
D’Acapito, F.
Hazemann, J-L.
Proux, O.
Nassif, V.
description X-ray absorption spectroscopy experiments were performed on a set of xenon implanted uranium dioxide samples. Results indicate that the gas forms highly pressurised inclusions as a result of temperature anneals or an external ion irradiation. Estimated bubble pressures were found to be in the region of 2–5GPa at low temperature. The consequences of such high pressures developing within intra-granular bubbles in irradiated fuels are discussed. A model is given enabling the computation of the sink strengths of bubbles as a function of the pressure of the rare-gas they contain. The model predicts that for pressure values found in the experiments, fission gas bubbles do not act as sinks for diffusing rare-gas atoms.
doi_str_mv 10.1016/j.jnucmat.2006.02.047
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subjects Applied sciences
Chemical Sciences
Condensed Matter
Cristallography
Energy
Energy. Thermal use of fuels
Exact sciences and technology
Fission nuclear power plants
Installations for energy generation and conversion: thermal and electrical energy
Material chemistry
Materials Science
Physics
title A study of xenon aggregates in uranium dioxide using X-ray absorption spectroscopy
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