Mercury Distribution in the Deûle River (Northern France) Measured by the Diffusive Gradients in Thin Films Technique and Conventional Methods
The distribution of mercury in surface water and in sediment from Deûle River in Northern France was studied by application of conventional sampling methods and by diffusive gradients in thin films technique (DGT). Concentration of total dissolved mercury in surface water was 20.8 ± 0.8 ng l⁻¹. The...
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| Veröffentlicht in: | Archives of environmental contamination and toxicology 2016-05, Vol.70 (4), p.700-709 |
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| creator | Diviš, Pavel Kadlecová, Milada Ouddane, Baghdad |
| description | The distribution of mercury in surface water and in sediment from Deûle River in Northern France was studied by application of conventional sampling methods and by diffusive gradients in thin films technique (DGT). Concentration of total dissolved mercury in surface water was 20.8 ± 0.8 ng l⁻¹. The particulate mercury concentration was 6.2 ± 0.6 µg g⁻¹. The particulate mercury was accumulated in sediment (9.9 ± 2.3 mg kg⁻¹), and it was transformed by methylating bacteria to methylmercury, mainly in the first 2-cm layer of the sediment. Total dissolved concentration of mercury in sediment pore water obtained by application of centrifugation extraction was 17.6 ± 4.1 ng l⁻¹, and it was comparable with total dissolved pore water mercury concentration measured by DGT probe containing Duolite GT-73 resin gel (18.2 ± 4.3 ng l⁻¹), taking the sediment heterogeneity and different principles of the applied methods into account. By application of two DGT probes with different resin gels specific for mercury, it was found that approximately 30 % of total dissolved mercury in sediment pore water was present in labile forms easy available for biota. The resolution of mercury DGT depth profiles was 0.5 cm, which allows, unlike conventional techniques, to study the connection of the geochemical cycle of mercury with geochemical cycles of iron and manganese. |
| doi_str_mv | 10.1007/s00244-015-0231-y |
| format | Article |
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Concentration of total dissolved mercury in surface water was 20.8 ± 0.8 ng l⁻¹. The particulate mercury concentration was 6.2 ± 0.6 µg g⁻¹. The particulate mercury was accumulated in sediment (9.9 ± 2.3 mg kg⁻¹), and it was transformed by methylating bacteria to methylmercury, mainly in the first 2-cm layer of the sediment. Total dissolved concentration of mercury in sediment pore water obtained by application of centrifugation extraction was 17.6 ± 4.1 ng l⁻¹, and it was comparable with total dissolved pore water mercury concentration measured by DGT probe containing Duolite GT-73 resin gel (18.2 ± 4.3 ng l⁻¹), taking the sediment heterogeneity and different principles of the applied methods into account. By application of two DGT probes with different resin gels specific for mercury, it was found that approximately 30 % of total dissolved mercury in sediment pore water was present in labile forms easy available for biota. The resolution of mercury DGT depth profiles was 0.5 cm, which allows, unlike conventional techniques, to study the connection of the geochemical cycle of mercury with geochemical cycles of iron and manganese.</description><identifier>ISSN: 0090-4341</identifier><identifier>EISSN: 1432-0703</identifier><identifier>DOI: 10.1007/s00244-015-0231-y</identifier><identifier>PMID: 26428003</identifier><language>eng</language><publisher>New York: Springer US</publisher><subject>Analysis ; Analytical chemistry ; Bacteria ; Biota ; Brackish ; Centrifugation ; Chemical Sciences ; Concentration (composition) ; Contaminated sediments ; Continental interfaces, environment ; Dissolution ; Earth and Environmental Science ; Earth Sciences ; Ecotoxicology ; Environment ; Environmental Chemistry ; Environmental Health ; Environmental Monitoring - methods ; Food chains ; France ; gels ; Geochemical cycles ; Geochemistry ; Heterogeneity ; iron ; Laboratories ; Lead ; Manganese ; Mercury ; Mercury (metal) ; Mercury - analysis ; Metals ; Methylmercury ; methylmercury compounds ; Monitoring/Environmental Analysis ; Planetary probes ; Pollution ; Pore water ; Porosity ; Production capacity ; Rivers ; Sampling methods ; Sciences of the Universe ; Sediments ; Soil Science & Conservation ; Studies ; Surface water ; Thin films ; Water Pollutants, Chemical - analysis ; Water pollution</subject><ispartof>Archives of environmental contamination and toxicology, 2016-05, Vol.70 (4), p.700-709</ispartof><rights>Springer Science+Business Media New York 2015</rights><rights>Springer Science+Business Media New York 2016</rights><rights>Distributed under a Creative Commons Attribution 4.0 International License</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-a519t-cf48245dfcce26c37c18de96313cc0308384e51a6e9af9cedba0bf6269ffcaeb3</citedby><cites>FETCH-LOGICAL-a519t-cf48245dfcce26c37c18de96313cc0308384e51a6e9af9cedba0bf6269ffcaeb3</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s00244-015-0231-y$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s00244-015-0231-y$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>230,314,777,781,882,27905,27906,41469,42538,51300</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/26428003$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink><backlink>$$Uhttps://hal.science/hal-01384560$$DView record in HAL$$Hfree_for_read</backlink></links><search><creatorcontrib>Diviš, Pavel</creatorcontrib><creatorcontrib>Kadlecová, Milada</creatorcontrib><creatorcontrib>Ouddane, Baghdad</creatorcontrib><title>Mercury Distribution in the Deûle River (Northern France) Measured by the Diffusive Gradients in Thin Films Technique and Conventional Methods</title><title>Archives of environmental contamination and toxicology</title><addtitle>Arch Environ Contam Toxicol</addtitle><addtitle>Arch Environ Contam Toxicol</addtitle><description>The distribution of mercury in surface water and in sediment from Deûle River in Northern France was studied by application of conventional sampling methods and by diffusive gradients in thin films technique (DGT). Concentration of total dissolved mercury in surface water was 20.8 ± 0.8 ng l⁻¹. The particulate mercury concentration was 6.2 ± 0.6 µg g⁻¹. The particulate mercury was accumulated in sediment (9.9 ± 2.3 mg kg⁻¹), and it was transformed by methylating bacteria to methylmercury, mainly in the first 2-cm layer of the sediment. Total dissolved concentration of mercury in sediment pore water obtained by application of centrifugation extraction was 17.6 ± 4.1 ng l⁻¹, and it was comparable with total dissolved pore water mercury concentration measured by DGT probe containing Duolite GT-73 resin gel (18.2 ± 4.3 ng l⁻¹), taking the sediment heterogeneity and different principles of the applied methods into account. By application of two DGT probes with different resin gels specific for mercury, it was found that approximately 30 % of total dissolved mercury in sediment pore water was present in labile forms easy available for biota. The resolution of mercury DGT depth profiles was 0.5 cm, which allows, unlike conventional techniques, to study the connection of the geochemical cycle of mercury with geochemical cycles of iron and manganese.</description><subject>Analysis</subject><subject>Analytical chemistry</subject><subject>Bacteria</subject><subject>Biota</subject><subject>Brackish</subject><subject>Centrifugation</subject><subject>Chemical Sciences</subject><subject>Concentration (composition)</subject><subject>Contaminated sediments</subject><subject>Continental interfaces, environment</subject><subject>Dissolution</subject><subject>Earth and Environmental Science</subject><subject>Earth Sciences</subject><subject>Ecotoxicology</subject><subject>Environment</subject><subject>Environmental Chemistry</subject><subject>Environmental Health</subject><subject>Environmental Monitoring - methods</subject><subject>Food chains</subject><subject>France</subject><subject>gels</subject><subject>Geochemical 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(HAL)</collection><jtitle>Archives of environmental contamination and toxicology</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Diviš, Pavel</au><au>Kadlecová, Milada</au><au>Ouddane, Baghdad</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Mercury Distribution in the Deûle River (Northern France) Measured by the Diffusive Gradients in Thin Films Technique and Conventional Methods</atitle><jtitle>Archives of environmental contamination and toxicology</jtitle><stitle>Arch Environ Contam Toxicol</stitle><addtitle>Arch Environ Contam Toxicol</addtitle><date>2016-05-01</date><risdate>2016</risdate><volume>70</volume><issue>4</issue><spage>700</spage><epage>709</epage><pages>700-709</pages><issn>0090-4341</issn><eissn>1432-0703</eissn><abstract>The distribution of mercury in surface water and in sediment from Deûle River in Northern France was studied by application of conventional sampling methods and by diffusive gradients in thin films technique (DGT). Concentration of total dissolved mercury in surface water was 20.8 ± 0.8 ng l⁻¹. The particulate mercury concentration was 6.2 ± 0.6 µg g⁻¹. The particulate mercury was accumulated in sediment (9.9 ± 2.3 mg kg⁻¹), and it was transformed by methylating bacteria to methylmercury, mainly in the first 2-cm layer of the sediment. Total dissolved concentration of mercury in sediment pore water obtained by application of centrifugation extraction was 17.6 ± 4.1 ng l⁻¹, and it was comparable with total dissolved pore water mercury concentration measured by DGT probe containing Duolite GT-73 resin gel (18.2 ± 4.3 ng l⁻¹), taking the sediment heterogeneity and different principles of the applied methods into account. By application of two DGT probes with different resin gels specific for mercury, it was found that approximately 30 % of total dissolved mercury in sediment pore water was present in labile forms easy available for biota. The resolution of mercury DGT depth profiles was 0.5 cm, which allows, unlike conventional techniques, to study the connection of the geochemical cycle of mercury with geochemical cycles of iron and manganese.</abstract><cop>New York</cop><pub>Springer US</pub><pmid>26428003</pmid><doi>10.1007/s00244-015-0231-y</doi><tpages>10</tpages></addata></record> |
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| subjects | Analysis Analytical chemistry Bacteria Biota Brackish Centrifugation Chemical Sciences Concentration (composition) Contaminated sediments Continental interfaces, environment Dissolution Earth and Environmental Science Earth Sciences Ecotoxicology Environment Environmental Chemistry Environmental Health Environmental Monitoring - methods Food chains France gels Geochemical cycles Geochemistry Heterogeneity iron Laboratories Lead Manganese Mercury Mercury (metal) Mercury - analysis Metals Methylmercury methylmercury compounds Monitoring/Environmental Analysis Planetary probes Pollution Pore water Porosity Production capacity Rivers Sampling methods Sciences of the Universe Sediments Soil Science & Conservation Studies Surface water Thin films Water Pollutants, Chemical - analysis Water pollution |
| title | Mercury Distribution in the Deûle River (Northern France) Measured by the Diffusive Gradients in Thin Films Technique and Conventional Methods |
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