A Novel Technology for Natural Gas Conversion by Means of Integrated Oxidative Coupling and Dry Reforming of Methane
A novel process concept for the oxidative coupling of methane followed by the oligomerization to liquids has been developed within the frame of the EU integrated project OCMOL. This technology is based on process intensification principles via cutting‐edge structured microreactor technology. It is a...
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| Veröffentlicht in: | Chemie ingenieur technik 2014-11, Vol.86 (11), p.1855-1870 |
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| creator | Thybaut, Joris W. Marin, Guy B. Mirodatos, Claude Schuurman, Yves van Veen, Andre C. Sadykov, Vladislav A. Pennemann, Helmut Bellinghausen, Rainer Mleczko, Leslaw |
| description | A novel process concept for the oxidative coupling of methane followed by the oligomerization to liquids has been developed within the frame of the EU integrated project OCMOL. This technology is based on process intensification principles via cutting‐edge structured microreactor technology. It is also a fully integrated industrial process through the re‐use and the recycling of by‐products, in particular CO2, at every process stage. The focus of this contribution is on the reaction engineering aspects of the core steps, i.e., catalysts, kinetics and reactor design for the methane coupling and reforming.
In the future, natural gas will replace crude oil in energy supply and feedstock generation because it is broadly available and has a lower price. Oxidative coupling of methane followed by oligomerization to liquids has been investigated as a means of converting the natural gas to higher hydrocarbons, including the catalyst concepts and reactor design. |
| doi_str_mv | 10.1002/cite.201400068 |
| format | Article |
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In the future, natural gas will replace crude oil in energy supply and feedstock generation because it is broadly available and has a lower price. Oxidative coupling of methane followed by oligomerization to liquids has been investigated as a means of converting the natural gas to higher hydrocarbons, including the catalyst concepts and reactor design.</description><identifier>ISSN: 0009-286X</identifier><identifier>EISSN: 1522-2640</identifier><identifier>DOI: 10.1002/cite.201400068</identifier><language>eng</language><publisher>Weinheim: WILEY-VCH Verlag</publisher><subject>Byproducts ; Catalysis ; Catalysts ; Chemical Sciences ; Environment and Society ; Environmental Sciences ; Joining ; Liquids ; Methane ; Natural gas ; Oxidative Coupling ; Process Intensification ; Reactor design ; Reforming</subject><ispartof>Chemie ingenieur technik, 2014-11, Vol.86 (11), p.1855-1870</ispartof><rights>Copyright © 2014 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim</rights><rights>Distributed under a Creative Commons Attribution 4.0 International License</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c4318-84babaafc5ad782c94a629f54961340e7e73429f2c06804d82bfce2fbb94c55b3</citedby><cites>FETCH-LOGICAL-c4318-84babaafc5ad782c94a629f54961340e7e73429f2c06804d82bfce2fbb94c55b3</cites><orcidid>0000-0002-2936-0910</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://onlinelibrary.wiley.com/doi/pdf/10.1002%2Fcite.201400068$$EPDF$$P50$$Gwiley$$H</linktopdf><linktohtml>$$Uhttps://onlinelibrary.wiley.com/doi/full/10.1002%2Fcite.201400068$$EHTML$$P50$$Gwiley$$H</linktohtml><link.rule.ids>230,314,778,782,883,1414,27907,27908,45557,45558</link.rule.ids><backlink>$$Uhttps://hal.science/hal-01277444$$DView record in HAL$$Hfree_for_read</backlink></links><search><creatorcontrib>Thybaut, Joris W.</creatorcontrib><creatorcontrib>Marin, Guy B.</creatorcontrib><creatorcontrib>Mirodatos, Claude</creatorcontrib><creatorcontrib>Schuurman, Yves</creatorcontrib><creatorcontrib>van Veen, Andre C.</creatorcontrib><creatorcontrib>Sadykov, Vladislav A.</creatorcontrib><creatorcontrib>Pennemann, Helmut</creatorcontrib><creatorcontrib>Bellinghausen, Rainer</creatorcontrib><creatorcontrib>Mleczko, Leslaw</creatorcontrib><title>A Novel Technology for Natural Gas Conversion by Means of Integrated Oxidative Coupling and Dry Reforming of Methane</title><title>Chemie ingenieur technik</title><addtitle>Chemie Ingenieur Technik</addtitle><description>A novel process concept for the oxidative coupling of methane followed by the oligomerization to liquids has been developed within the frame of the EU integrated project OCMOL. This technology is based on process intensification principles via cutting‐edge structured microreactor technology. It is also a fully integrated industrial process through the re‐use and the recycling of by‐products, in particular CO2, at every process stage. The focus of this contribution is on the reaction engineering aspects of the core steps, i.e., catalysts, kinetics and reactor design for the methane coupling and reforming.
In the future, natural gas will replace crude oil in energy supply and feedstock generation because it is broadly available and has a lower price. Oxidative coupling of methane followed by oligomerization to liquids has been investigated as a means of converting the natural gas to higher hydrocarbons, including the catalyst concepts and reactor design.</description><subject>Byproducts</subject><subject>Catalysis</subject><subject>Catalysts</subject><subject>Chemical Sciences</subject><subject>Environment and Society</subject><subject>Environmental Sciences</subject><subject>Joining</subject><subject>Liquids</subject><subject>Methane</subject><subject>Natural gas</subject><subject>Oxidative Coupling</subject><subject>Process Intensification</subject><subject>Reactor design</subject><subject>Reforming</subject><issn>0009-286X</issn><issn>1522-2640</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2014</creationdate><recordtype>article</recordtype><recordid>eNqFkc1v0zAYhy0EEmXsytlHOKTzV76OVRhtpbaTUKdxsxznTWtI42K7Zfnv5ypTtRsnyz8_z2tbP4S-UDKlhLA7bQJMGaGCEJIV79CEpowlLBPkPZrErExYkf36iD55_ztui3g8QWGGN_YMHd6C3ve2s7sBt9bhjQonpzo8Vx5Xtj-D88b2uB7wGlTvsW3xsg-wcypAgx-eTaOCOUNkT8fO9Dus-gZ_dwP-CXHc4ZJEZQ1hr3r4jD60qvNw-7reoMcf99tqkawe5stqtkq04LRIClGrWqlWp6rJC6ZLoTJWtqkoM8oFgRxyLmLAdPwvEU3B6lYDa-u6FDpNa36Dvo1z96qTR2cOyg3SKiMXs5W8ZISyPBdCnGlkv47s0dm_J_BBHozX0HXxvfbkJY1X8zQnKYvodES1s947aK-zKZGXKuSlCnmtIgrlKPwzHQz_oWW13N6_dZPRNT7A89VV7o_Mcp6n8mkzl2v-JOZ0wWXFXwCYppwm</recordid><startdate>201411</startdate><enddate>201411</enddate><creator>Thybaut, Joris W.</creator><creator>Marin, Guy B.</creator><creator>Mirodatos, Claude</creator><creator>Schuurman, Yves</creator><creator>van Veen, Andre C.</creator><creator>Sadykov, Vladislav A.</creator><creator>Pennemann, Helmut</creator><creator>Bellinghausen, Rainer</creator><creator>Mleczko, Leslaw</creator><general>WILEY-VCH Verlag</general><general>WILEY‐VCH Verlag</general><general>Wiley-VCH Verlag</general><scope>BSCLL</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7U5</scope><scope>8FD</scope><scope>L7M</scope><scope>1XC</scope><orcidid>https://orcid.org/0000-0002-2936-0910</orcidid></search><sort><creationdate>201411</creationdate><title>A Novel Technology for Natural Gas Conversion by Means of Integrated Oxidative Coupling and Dry Reforming of Methane</title><author>Thybaut, Joris W. ; Marin, Guy B. ; Mirodatos, Claude ; Schuurman, Yves ; van Veen, Andre C. ; Sadykov, Vladislav A. ; Pennemann, Helmut ; Bellinghausen, Rainer ; Mleczko, Leslaw</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c4318-84babaafc5ad782c94a629f54961340e7e73429f2c06804d82bfce2fbb94c55b3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2014</creationdate><topic>Byproducts</topic><topic>Catalysis</topic><topic>Catalysts</topic><topic>Chemical Sciences</topic><topic>Environment and Society</topic><topic>Environmental Sciences</topic><topic>Joining</topic><topic>Liquids</topic><topic>Methane</topic><topic>Natural gas</topic><topic>Oxidative Coupling</topic><topic>Process Intensification</topic><topic>Reactor design</topic><topic>Reforming</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Thybaut, Joris W.</creatorcontrib><creatorcontrib>Marin, Guy B.</creatorcontrib><creatorcontrib>Mirodatos, Claude</creatorcontrib><creatorcontrib>Schuurman, Yves</creatorcontrib><creatorcontrib>van Veen, Andre C.</creatorcontrib><creatorcontrib>Sadykov, Vladislav A.</creatorcontrib><creatorcontrib>Pennemann, Helmut</creatorcontrib><creatorcontrib>Bellinghausen, Rainer</creatorcontrib><creatorcontrib>Mleczko, Leslaw</creatorcontrib><collection>Istex</collection><collection>CrossRef</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>Technology Research Database</collection><collection>Advanced Technologies Database with Aerospace</collection><collection>Hyper Article en Ligne (HAL)</collection><jtitle>Chemie ingenieur technik</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Thybaut, Joris W.</au><au>Marin, Guy B.</au><au>Mirodatos, Claude</au><au>Schuurman, Yves</au><au>van Veen, Andre C.</au><au>Sadykov, Vladislav A.</au><au>Pennemann, Helmut</au><au>Bellinghausen, Rainer</au><au>Mleczko, Leslaw</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>A Novel Technology for Natural Gas Conversion by Means of Integrated Oxidative Coupling and Dry Reforming of Methane</atitle><jtitle>Chemie ingenieur technik</jtitle><addtitle>Chemie Ingenieur Technik</addtitle><date>2014-11</date><risdate>2014</risdate><volume>86</volume><issue>11</issue><spage>1855</spage><epage>1870</epage><pages>1855-1870</pages><issn>0009-286X</issn><eissn>1522-2640</eissn><abstract>A novel process concept for the oxidative coupling of methane followed by the oligomerization to liquids has been developed within the frame of the EU integrated project OCMOL. 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| source | Wiley Online Library Journals Frontfile Complete |
| subjects | Byproducts Catalysis Catalysts Chemical Sciences Environment and Society Environmental Sciences Joining Liquids Methane Natural gas Oxidative Coupling Process Intensification Reactor design Reforming |
| title | A Novel Technology for Natural Gas Conversion by Means of Integrated Oxidative Coupling and Dry Reforming of Methane |
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