Supported Au catalysts for propene total oxidation: Study of support morphology and gold particle size effects
In this work gold nanoparticles supported over three different metal oxides, TiO 2, ZnO and Al 2O 3 were characterized by BET surface area and pore size distribution, XRD, XPS and TEM techniques and their catalytic performances were evaluated in the total oxidation of propene, chosen as model VOC mo...
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| Veröffentlicht in: | Catalysis today 2011-11, Vol.176 (1), p.7-13 |
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| container_title | Catalysis today |
| container_volume | 176 |
| creator | Ousmane, M. Liotta, L.F. Pantaleo, G. Venezia, A.M. Di Carlo, G. Aouine, M. Retailleau, L. Giroir-Fendler, A. |
| description | In this work gold nanoparticles supported over three different metal oxides, TiO
2, ZnO and Al
2O
3 were characterized by BET surface area and pore size distribution, XRD, XPS and TEM techniques and their catalytic performances were evaluated in the total oxidation of propene, chosen as model VOC molecule. Attention was focused on the evaluation of the catalytic activity by performing three consecutive catalytic runs. Characterizations by XPS and TEM were carried out on the spent catalysts after propene oxidation tests.
The results were discussed in terms of relationship between morphological, structural, electronic and catalytic properties as a function of the nature of the support. |
| doi_str_mv | 10.1016/j.cattod.2011.07.009 |
| format | Article |
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2, ZnO and Al
2O
3 were characterized by BET surface area and pore size distribution, XRD, XPS and TEM techniques and their catalytic performances were evaluated in the total oxidation of propene, chosen as model VOC molecule. Attention was focused on the evaluation of the catalytic activity by performing three consecutive catalytic runs. Characterizations by XPS and TEM were carried out on the spent catalysts after propene oxidation tests.
The results were discussed in terms of relationship between morphological, structural, electronic and catalytic properties as a function of the nature of the support.</description><identifier>ISSN: 0920-5861</identifier><identifier>EISSN: 1873-4308</identifier><identifier>DOI: 10.1016/j.cattod.2011.07.009</identifier><identifier>CODEN: CATTEA</identifier><language>eng</language><publisher>Amsterdam: Elsevier B.V</publisher><subject>Al 2O 3 ; Au particle size ; Catalysis ; Chemical Sciences ; Chemistry ; Colloidal state and disperse state ; Environment and Society ; Environmental Sciences ; Exact sciences and technology ; General and physical chemistry ; Metal–support interaction ; Physical and chemical studies. Granulometry. Electrokinetic phenomena ; Porous materials ; Propene oxidation ; Support morphology ; Theory of reactions, general kinetics. Catalysis. Nomenclature, chemical documentation, computer chemistry ; TiO 2 ; ZnO</subject><ispartof>Catalysis today, 2011-11, Vol.176 (1), p.7-13</ispartof><rights>2011 Elsevier B.V.</rights><rights>2015 INIST-CNRS</rights><rights>Distributed under a Creative Commons Attribution 4.0 International License</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c436t-751679a70dbd9cdf26e8f736d5c091a4f781be7873827747472ca09969d3d953</citedby><cites>FETCH-LOGICAL-c436t-751679a70dbd9cdf26e8f736d5c091a4f781be7873827747472ca09969d3d953</cites><orcidid>0000-0003-3651-2721 ; 0000-0002-2750-9929</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktohtml>$$Uhttps://www.sciencedirect.com/science/article/pii/S0920586111005281$$EHTML$$P50$$Gelsevier$$H</linktohtml><link.rule.ids>230,309,310,314,776,780,785,786,881,3537,23909,23910,25118,27901,27902,65306</link.rule.ids><backlink>$$Uhttp://pascal-francis.inist.fr/vibad/index.php?action=getRecordDetail&idt=24741147$$DView record in Pascal Francis$$Hfree_for_read</backlink><backlink>$$Uhttps://hal.science/hal-00699704$$DView record in HAL$$Hfree_for_read</backlink></links><search><creatorcontrib>Ousmane, M.</creatorcontrib><creatorcontrib>Liotta, L.F.</creatorcontrib><creatorcontrib>Pantaleo, G.</creatorcontrib><creatorcontrib>Venezia, A.M.</creatorcontrib><creatorcontrib>Di Carlo, G.</creatorcontrib><creatorcontrib>Aouine, M.</creatorcontrib><creatorcontrib>Retailleau, L.</creatorcontrib><creatorcontrib>Giroir-Fendler, A.</creatorcontrib><title>Supported Au catalysts for propene total oxidation: Study of support morphology and gold particle size effects</title><title>Catalysis today</title><description>In this work gold nanoparticles supported over three different metal oxides, TiO
2, ZnO and Al
2O
3 were characterized by BET surface area and pore size distribution, XRD, XPS and TEM techniques and their catalytic performances were evaluated in the total oxidation of propene, chosen as model VOC molecule. Attention was focused on the evaluation of the catalytic activity by performing three consecutive catalytic runs. Characterizations by XPS and TEM were carried out on the spent catalysts after propene oxidation tests.
The results were discussed in terms of relationship between morphological, structural, electronic and catalytic properties as a function of the nature of the support.</description><subject>Al 2O 3</subject><subject>Au particle size</subject><subject>Catalysis</subject><subject>Chemical Sciences</subject><subject>Chemistry</subject><subject>Colloidal state and disperse state</subject><subject>Environment and Society</subject><subject>Environmental Sciences</subject><subject>Exact sciences and technology</subject><subject>General and physical chemistry</subject><subject>Metal–support interaction</subject><subject>Physical and chemical studies. Granulometry. Electrokinetic phenomena</subject><subject>Porous materials</subject><subject>Propene oxidation</subject><subject>Support morphology</subject><subject>Theory of reactions, general kinetics. Catalysis. Nomenclature, chemical documentation, computer chemistry</subject><subject>TiO 2</subject><subject>ZnO</subject><issn>0920-5861</issn><issn>1873-4308</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2011</creationdate><recordtype>article</recordtype><recordid>eNp9kE9LAzEQxYMoWKvfwEMuHjzsOtndbjYehCJqhYKH9h7S_GlTtpslSYv105uy0qPMYWB4v5l5D6F7AjkBUj9tcylidCovgJAcaA7ALtCINLTMqhKaSzQCVkA2aWpyjW5C2AJA01TFCHWLfd87H7XC0z1Oa0R7DDFg4zzuvet1p3F0aYrdt1UiWtc940XcqyN2BocBxjvn-41r3fqIRafw2rUK98JHK1uNg_3RWBujZQy36MqINui7vz5Gy_e35essm399fL5O55msyjpmdEJqygQFtVJMKlPUujG0rNVEAiOiMrQhK02Tv6agtEpVSAGM1UyVik3KMXoc1m5Ey3tvd8IfuROWz6ZzfpoB1IxRqA4kaatBK70LwWtzBgjwU7x8y4d4-SleDjTRLGEPA9aLIEVrvOikDWe2SE8RUtGkexl0Otk9WO15kFZ3UivrUyJcOfv_oV9wnJND</recordid><startdate>20111101</startdate><enddate>20111101</enddate><creator>Ousmane, M.</creator><creator>Liotta, L.F.</creator><creator>Pantaleo, G.</creator><creator>Venezia, A.M.</creator><creator>Di Carlo, G.</creator><creator>Aouine, M.</creator><creator>Retailleau, L.</creator><creator>Giroir-Fendler, A.</creator><general>Elsevier B.V</general><general>Elsevier</general><scope>IQODW</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>1XC</scope><orcidid>https://orcid.org/0000-0003-3651-2721</orcidid><orcidid>https://orcid.org/0000-0002-2750-9929</orcidid></search><sort><creationdate>20111101</creationdate><title>Supported Au catalysts for propene total oxidation: Study of support morphology and gold particle size effects</title><author>Ousmane, M. ; Liotta, L.F. ; Pantaleo, G. ; Venezia, A.M. ; Di Carlo, G. ; Aouine, M. ; Retailleau, L. ; Giroir-Fendler, A.</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c436t-751679a70dbd9cdf26e8f736d5c091a4f781be7873827747472ca09969d3d953</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2011</creationdate><topic>Al 2O 3</topic><topic>Au particle size</topic><topic>Catalysis</topic><topic>Chemical Sciences</topic><topic>Chemistry</topic><topic>Colloidal state and disperse state</topic><topic>Environment and Society</topic><topic>Environmental Sciences</topic><topic>Exact sciences and technology</topic><topic>General and physical chemistry</topic><topic>Metal–support interaction</topic><topic>Physical and chemical studies. Granulometry. Electrokinetic phenomena</topic><topic>Porous materials</topic><topic>Propene oxidation</topic><topic>Support morphology</topic><topic>Theory of reactions, general kinetics. Catalysis. Nomenclature, chemical documentation, computer chemistry</topic><topic>TiO 2</topic><topic>ZnO</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Ousmane, M.</creatorcontrib><creatorcontrib>Liotta, L.F.</creatorcontrib><creatorcontrib>Pantaleo, G.</creatorcontrib><creatorcontrib>Venezia, A.M.</creatorcontrib><creatorcontrib>Di Carlo, G.</creatorcontrib><creatorcontrib>Aouine, M.</creatorcontrib><creatorcontrib>Retailleau, L.</creatorcontrib><creatorcontrib>Giroir-Fendler, A.</creatorcontrib><collection>Pascal-Francis</collection><collection>CrossRef</collection><collection>Hyper Article en Ligne (HAL)</collection><jtitle>Catalysis today</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Ousmane, M.</au><au>Liotta, L.F.</au><au>Pantaleo, G.</au><au>Venezia, A.M.</au><au>Di Carlo, G.</au><au>Aouine, M.</au><au>Retailleau, L.</au><au>Giroir-Fendler, A.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Supported Au catalysts for propene total oxidation: Study of support morphology and gold particle size effects</atitle><jtitle>Catalysis today</jtitle><date>2011-11-01</date><risdate>2011</risdate><volume>176</volume><issue>1</issue><spage>7</spage><epage>13</epage><pages>7-13</pages><issn>0920-5861</issn><eissn>1873-4308</eissn><coden>CATTEA</coden><abstract>In this work gold nanoparticles supported over three different metal oxides, TiO
2, ZnO and Al
2O
3 were characterized by BET surface area and pore size distribution, XRD, XPS and TEM techniques and their catalytic performances were evaluated in the total oxidation of propene, chosen as model VOC molecule. Attention was focused on the evaluation of the catalytic activity by performing three consecutive catalytic runs. Characterizations by XPS and TEM were carried out on the spent catalysts after propene oxidation tests.
The results were discussed in terms of relationship between morphological, structural, electronic and catalytic properties as a function of the nature of the support.</abstract><cop>Amsterdam</cop><pub>Elsevier B.V</pub><doi>10.1016/j.cattod.2011.07.009</doi><tpages>7</tpages><orcidid>https://orcid.org/0000-0003-3651-2721</orcidid><orcidid>https://orcid.org/0000-0002-2750-9929</orcidid></addata></record> |
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| ispartof | Catalysis today, 2011-11, Vol.176 (1), p.7-13 |
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| language | eng |
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| source | Elsevier ScienceDirect Journals Complete |
| subjects | Al 2O 3 Au particle size Catalysis Chemical Sciences Chemistry Colloidal state and disperse state Environment and Society Environmental Sciences Exact sciences and technology General and physical chemistry Metal–support interaction Physical and chemical studies. Granulometry. Electrokinetic phenomena Porous materials Propene oxidation Support morphology Theory of reactions, general kinetics. Catalysis. Nomenclature, chemical documentation, computer chemistry TiO 2 ZnO |
| title | Supported Au catalysts for propene total oxidation: Study of support morphology and gold particle size effects |
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