Hydrogen production from ethanol steam reforming in a micro-channel reactor
Ethanol steam reforming was studied over a supported Ir/CeO 2 catalyst in a micro-channel structured reactor. The catalyst coating was deposited on the channel walls and showed a remarkably high homogeneity and an excellent adherence to the stainless steel substrate, leading to stable performance du...
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| Veröffentlicht in: | International journal of hydrogen energy 2010-02, Vol.35 (3), p.1152-1159 |
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| container_end_page | 1159 |
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| container_issue | 3 |
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| container_title | International journal of hydrogen energy |
| container_volume | 35 |
| creator | Cai, Weijie Wang, Fagen van Veen, Andre Descorme, Claude Schuurman, Yves Shen, Wenjie Mirodatos, Claude |
| description | Ethanol steam reforming was studied over a supported Ir/CeO
2 catalyst in a micro-channel structured reactor. The catalyst coating was deposited on the channel walls and showed a remarkably high homogeneity and an excellent adherence to the stainless steel substrate, leading to stable performance during long-term runs. Hydrogen yields exceeding 40 L
H2 g
cat
−1 h
−1 were achieved during testing with partial ethanol conversion of 65% and a residence time in the order of a few milliseconds. This hydrogen productivity was found significantly higher than in a comparable conventional fixed-bed reactor hence being extremely promising for hydrogen production in micro fuel cell applications. |
| doi_str_mv | 10.1016/j.ijhydene.2009.11.104 |
| format | Article |
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2 catalyst in a micro-channel structured reactor. The catalyst coating was deposited on the channel walls and showed a remarkably high homogeneity and an excellent adherence to the stainless steel substrate, leading to stable performance during long-term runs. Hydrogen yields exceeding 40 L
H2 g
cat
−1 h
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2 catalyst in a micro-channel structured reactor. The catalyst coating was deposited on the channel walls and showed a remarkably high homogeneity and an excellent adherence to the stainless steel substrate, leading to stable performance during long-term runs. Hydrogen yields exceeding 40 L
H2 g
cat
−1 h
−1 were achieved during testing with partial ethanol conversion of 65% and a residence time in the order of a few milliseconds. This hydrogen productivity was found significantly higher than in a comparable conventional fixed-bed reactor hence being extremely promising for hydrogen production in micro fuel cell applications.</description><subject>Alternative fuels. Production and utilization</subject><subject>Applied sciences</subject><subject>Catalysis</subject><subject>Catalysts</subject><subject>Ceria</subject><subject>Chemical Sciences</subject><subject>Energy</subject><subject>Ethanol</subject><subject>Ethanol steam reforming</subject><subject>Ethyl alcohol</subject><subject>Exact sciences and technology</subject><subject>Fuels</subject><subject>Homogeneity</subject><subject>Hydrogen</subject><subject>Hydrogen production</subject><subject>Iridium</subject><subject>Micro-reactor</subject><subject>Reactors</subject><subject>Reforming</subject><subject>Walls</subject><issn>0360-3199</issn><issn>1879-3487</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2010</creationdate><recordtype>article</recordtype><recordid>eNqFkE1LAzEQhoMoWD_-guxFxMPWZDfdJDdF1IoFL3oOYzKxKbuJJluh_96UqldPgTfPzPA-hJwxOmWUdVerqV8tNxYDThtK1ZSxkvM9MmFSqLrlUuyTCW07WrdMqUNylPOKUiYoVxPyNN_YFN8xVB8p2rUZfQyVS3GocFxCiH2VR4ShSuhiGnx4r3yooBq8SbE2hQjYl08wY0wn5MBBn_H05z0mr_d3L7fzevH88Hh7s6gNF3ysWaMaabnjUgnLwNrOSCskB5StVS00zPG3N-tmXFpjccbQuJLNrALhwIn2mFzu9i6h1x_JD5A2OoLX85uF3maU8k4UNV-ssBc7ttT7XGMe9eCzwb6HgHGdtSqYEpLKQnY7sjTLufT9W82o3orWK_0rWm9Fa8ZKzsvg-c8JyAZ6lyAYn_-mm4a3XSebwl3vOCxuvjwmnY3HYND6hGbUNvr_Tn0DSaKYAg</recordid><startdate>20100201</startdate><enddate>20100201</enddate><creator>Cai, Weijie</creator><creator>Wang, Fagen</creator><creator>van Veen, Andre</creator><creator>Descorme, Claude</creator><creator>Schuurman, Yves</creator><creator>Shen, Wenjie</creator><creator>Mirodatos, Claude</creator><general>Elsevier Ltd</general><general>Elsevier</general><scope>IQODW</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7SP</scope><scope>8FD</scope><scope>L7M</scope><scope>1XC</scope><orcidid>https://orcid.org/0000-0001-9918-1769</orcidid><orcidid>https://orcid.org/0000-0002-2936-0910</orcidid></search><sort><creationdate>20100201</creationdate><title>Hydrogen production from ethanol steam reforming in a micro-channel reactor</title><author>Cai, Weijie ; Wang, Fagen ; van Veen, Andre ; Descorme, Claude ; Schuurman, Yves ; Shen, Wenjie ; Mirodatos, Claude</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c474t-12928d4f4897d1add6c8d784ae83d93a21f4bbdf548dcde51ecf21f5d9a7faf73</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2010</creationdate><topic>Alternative fuels. Production and utilization</topic><topic>Applied sciences</topic><topic>Catalysis</topic><topic>Catalysts</topic><topic>Ceria</topic><topic>Chemical Sciences</topic><topic>Energy</topic><topic>Ethanol</topic><topic>Ethanol steam reforming</topic><topic>Ethyl alcohol</topic><topic>Exact sciences and technology</topic><topic>Fuels</topic><topic>Homogeneity</topic><topic>Hydrogen</topic><topic>Hydrogen production</topic><topic>Iridium</topic><topic>Micro-reactor</topic><topic>Reactors</topic><topic>Reforming</topic><topic>Walls</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Cai, Weijie</creatorcontrib><creatorcontrib>Wang, Fagen</creatorcontrib><creatorcontrib>van Veen, Andre</creatorcontrib><creatorcontrib>Descorme, Claude</creatorcontrib><creatorcontrib>Schuurman, Yves</creatorcontrib><creatorcontrib>Shen, Wenjie</creatorcontrib><creatorcontrib>Mirodatos, Claude</creatorcontrib><collection>Pascal-Francis</collection><collection>CrossRef</collection><collection>Electronics & Communications Abstracts</collection><collection>Technology Research Database</collection><collection>Advanced Technologies Database with Aerospace</collection><collection>Hyper Article en Ligne (HAL)</collection><jtitle>International journal of hydrogen energy</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Cai, Weijie</au><au>Wang, Fagen</au><au>van Veen, Andre</au><au>Descorme, Claude</au><au>Schuurman, Yves</au><au>Shen, Wenjie</au><au>Mirodatos, Claude</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Hydrogen production from ethanol steam reforming in a micro-channel reactor</atitle><jtitle>International journal of hydrogen energy</jtitle><date>2010-02-01</date><risdate>2010</risdate><volume>35</volume><issue>3</issue><spage>1152</spage><epage>1159</epage><pages>1152-1159</pages><issn>0360-3199</issn><eissn>1879-3487</eissn><coden>IJHEDX</coden><abstract>Ethanol steam reforming was studied over a supported Ir/CeO
2 catalyst in a micro-channel structured reactor. The catalyst coating was deposited on the channel walls and showed a remarkably high homogeneity and an excellent adherence to the stainless steel substrate, leading to stable performance during long-term runs. Hydrogen yields exceeding 40 L
H2 g
cat
−1 h
−1 were achieved during testing with partial ethanol conversion of 65% and a residence time in the order of a few milliseconds. This hydrogen productivity was found significantly higher than in a comparable conventional fixed-bed reactor hence being extremely promising for hydrogen production in micro fuel cell applications.</abstract><cop>Kidlington</cop><pub>Elsevier Ltd</pub><doi>10.1016/j.ijhydene.2009.11.104</doi><tpages>8</tpages><orcidid>https://orcid.org/0000-0001-9918-1769</orcidid><orcidid>https://orcid.org/0000-0002-2936-0910</orcidid></addata></record> |
| fulltext | fulltext |
| identifier | ISSN: 0360-3199 |
| ispartof | International journal of hydrogen energy, 2010-02, Vol.35 (3), p.1152-1159 |
| issn | 0360-3199 1879-3487 |
| language | eng |
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| source | Elsevier ScienceDirect Journals |
| subjects | Alternative fuels. Production and utilization Applied sciences Catalysis Catalysts Ceria Chemical Sciences Energy Ethanol Ethanol steam reforming Ethyl alcohol Exact sciences and technology Fuels Homogeneity Hydrogen Hydrogen production Iridium Micro-reactor Reactors Reforming Walls |
| title | Hydrogen production from ethanol steam reforming in a micro-channel reactor |
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