Nanocomposite tantalum–carbon-based films deposited by femtosecond pulsed laser ablation
Nanostructured coatings of metal (tantalum) containing diamond-like carbon (a-C:Ta) have been prepared by femtosecond pulsed laser deposition (PLD). The films, containing 15 at.% tantalum, have been deposited by ablating sequentially graphite and metallic tantalum in vacuum conditions with an amplif...
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| Veröffentlicht in: | Thin solid films 2006-01, Vol.494 (1), p.98-104 |
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| container_title | Thin solid films |
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| creator | Benchikh, N. Garrelie, F. Wolski, K. Donnet, C. Fillit, R.Y. Rogemond, F. Subtil, J.L. Rouzaud, J.N. Laval, J.Y. |
| description | Nanostructured coatings of metal (tantalum) containing diamond-like carbon (a-C:Ta) have been prepared by femtosecond pulsed laser deposition (PLD). The films, containing 15 at.% tantalum, have been deposited by ablating sequentially graphite and metallic tantalum in vacuum conditions with an amplified Ti:sapphire laser. The coatings have been investigated by X-ray photoelectron spectroscopy, grazing angle X-ray diffraction, energy filtered transmission electron microscopy, scanning and high resolution transmission electron microscopies. Evidence of metallic α-Ta and β-Ta particles (diameter in the 100 nm range) and smaller quasi-amorphous tantalum clusters embedded in the carbonaceous matrix have been shown. A thin tantalum carbide interface between the carbon matrix and the top surface of the tantalum nodules has also been identified. The ability of femtosecond pulsed laser deposition to synthetize nanocomposite carbon-based films and to control their nanostructure is discussed. |
| doi_str_mv | 10.1016/j.tsf.2005.07.161 |
| format | Article |
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The films, containing 15 at.% tantalum, have been deposited by ablating sequentially graphite and metallic tantalum in vacuum conditions with an amplified Ti:sapphire laser. The coatings have been investigated by X-ray photoelectron spectroscopy, grazing angle X-ray diffraction, energy filtered transmission electron microscopy, scanning and high resolution transmission electron microscopies. Evidence of metallic α-Ta and β-Ta particles (diameter in the 100 nm range) and smaller quasi-amorphous tantalum clusters embedded in the carbonaceous matrix have been shown. A thin tantalum carbide interface between the carbon matrix and the top surface of the tantalum nodules has also been identified. The ability of femtosecond pulsed laser deposition to synthetize nanocomposite carbon-based films and to control their nanostructure is discussed.</description><subject>Cross-disciplinary physics: materials science; rheology</subject><subject>Doped diamond-like carbon</subject><subject>Engineering Sciences</subject><subject>Exact sciences and technology</subject><subject>Femtosecond laser</subject><subject>Laser deposition</subject><subject>Materials</subject><subject>Materials science</subject><subject>Methods of deposition of films and coatings; film growth and epitaxy</subject><subject>Nanocrystalline materials</subject><subject>Nanoscale materials and structures: fabrication and characterization</subject><subject>Optics</subject><subject>Photonic</subject><subject>Physics</subject><subject>Plasmas</subject><subject>Pulsed loser ablation</subject><issn>0040-6090</issn><issn>1879-2731</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2006</creationdate><recordtype>article</recordtype><recordid>eNp9kM1u1TAQhS0EEpeWB2CXDUgsEsb_iVhVVUsrXcEGNmwsx7GFr5z4YvtW6o536Bv2SXCUCnZdjXT0nTMzB6F3GDoMWHw6dCW7jgDwDmSHBX6BdriXQ0skxS_RDoBBK2CA1-hNzgcAwITQHfr5VS_RxPkYsy-2KXopOpzmxz8PRqcxLu2os50a58Ocm8lu2NSM942zc4nZmrhMzfEUVipUNjV6DLr4uJyjV05X_e3TPEM_rq--X960-29fbi8v9q1hvC-tY26wogegmDE7Si1Ej3vDHMejoYaP61OG1HMFcYJb7gQwNkiuiR44HegZ-rjl_tJBHZOfdbpXUXt1c7FXqwZABtKz4Q5X9sPGHlP8fbK5qNlnY0PQi42nrEgveoI5rSDeQJNizsm6f8kY1Nq4OqjauFqPUyBVbbx63j-F62x0cEkvxuf_Rskpp1JW7vPG2drKnbdJZePtYuzkkzVFTdE_s-Uv44iWgQ</recordid><startdate>20060103</startdate><enddate>20060103</enddate><creator>Benchikh, N.</creator><creator>Garrelie, F.</creator><creator>Wolski, K.</creator><creator>Donnet, C.</creator><creator>Fillit, R.Y.</creator><creator>Rogemond, F.</creator><creator>Subtil, J.L.</creator><creator>Rouzaud, J.N.</creator><creator>Laval, J.Y.</creator><general>Elsevier B.V</general><general>Elsevier Science</general><general>Elsevier</general><scope>IQODW</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7QQ</scope><scope>7SR</scope><scope>7U5</scope><scope>8BQ</scope><scope>8FD</scope><scope>JG9</scope><scope>L7M</scope><scope>1XC</scope><orcidid>https://orcid.org/0000-0003-4557-8677</orcidid></search><sort><creationdate>20060103</creationdate><title>Nanocomposite tantalum–carbon-based films deposited by femtosecond pulsed laser ablation</title><author>Benchikh, N. ; Garrelie, F. ; Wolski, K. ; Donnet, C. ; Fillit, R.Y. ; Rogemond, F. ; Subtil, J.L. ; Rouzaud, J.N. ; Laval, J.Y.</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c458t-f4f9e68003144eb7a66818c4f51bc3c5b2005c212262f65e5f6044975a2a95393</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2006</creationdate><topic>Cross-disciplinary physics: materials science; rheology</topic><topic>Doped diamond-like carbon</topic><topic>Engineering Sciences</topic><topic>Exact sciences and technology</topic><topic>Femtosecond laser</topic><topic>Laser deposition</topic><topic>Materials</topic><topic>Materials science</topic><topic>Methods of deposition of films and coatings; film growth and epitaxy</topic><topic>Nanocrystalline materials</topic><topic>Nanoscale materials and structures: fabrication and characterization</topic><topic>Optics</topic><topic>Photonic</topic><topic>Physics</topic><topic>Plasmas</topic><topic>Pulsed loser ablation</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Benchikh, N.</creatorcontrib><creatorcontrib>Garrelie, F.</creatorcontrib><creatorcontrib>Wolski, K.</creatorcontrib><creatorcontrib>Donnet, C.</creatorcontrib><creatorcontrib>Fillit, R.Y.</creatorcontrib><creatorcontrib>Rogemond, F.</creatorcontrib><creatorcontrib>Subtil, J.L.</creatorcontrib><creatorcontrib>Rouzaud, J.N.</creatorcontrib><creatorcontrib>Laval, J.Y.</creatorcontrib><collection>Pascal-Francis</collection><collection>CrossRef</collection><collection>Ceramic Abstracts</collection><collection>Engineered Materials Abstracts</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>Materials Research Database</collection><collection>Advanced Technologies Database with Aerospace</collection><collection>Hyper Article en Ligne (HAL)</collection><jtitle>Thin solid films</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Benchikh, N.</au><au>Garrelie, F.</au><au>Wolski, K.</au><au>Donnet, C.</au><au>Fillit, R.Y.</au><au>Rogemond, F.</au><au>Subtil, J.L.</au><au>Rouzaud, J.N.</au><au>Laval, J.Y.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Nanocomposite tantalum–carbon-based films deposited by femtosecond pulsed laser ablation</atitle><jtitle>Thin solid films</jtitle><date>2006-01-03</date><risdate>2006</risdate><volume>494</volume><issue>1</issue><spage>98</spage><epage>104</epage><pages>98-104</pages><issn>0040-6090</issn><eissn>1879-2731</eissn><coden>THSFAP</coden><abstract>Nanostructured coatings of metal (tantalum) containing diamond-like carbon (a-C:Ta) have been prepared by femtosecond pulsed laser deposition (PLD). The films, containing 15 at.% tantalum, have been deposited by ablating sequentially graphite and metallic tantalum in vacuum conditions with an amplified Ti:sapphire laser. The coatings have been investigated by X-ray photoelectron spectroscopy, grazing angle X-ray diffraction, energy filtered transmission electron microscopy, scanning and high resolution transmission electron microscopies. Evidence of metallic α-Ta and β-Ta particles (diameter in the 100 nm range) and smaller quasi-amorphous tantalum clusters embedded in the carbonaceous matrix have been shown. A thin tantalum carbide interface between the carbon matrix and the top surface of the tantalum nodules has also been identified. The ability of femtosecond pulsed laser deposition to synthetize nanocomposite carbon-based films and to control their nanostructure is discussed.</abstract><cop>Lausanne</cop><pub>Elsevier B.V</pub><doi>10.1016/j.tsf.2005.07.161</doi><tpages>7</tpages><orcidid>https://orcid.org/0000-0003-4557-8677</orcidid></addata></record> |
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| source | ScienceDirect Journals (5 years ago - present) |
| subjects | Cross-disciplinary physics: materials science rheology Doped diamond-like carbon Engineering Sciences Exact sciences and technology Femtosecond laser Laser deposition Materials Materials science Methods of deposition of films and coatings film growth and epitaxy Nanocrystalline materials Nanoscale materials and structures: fabrication and characterization Optics Photonic Physics Plasmas Pulsed loser ablation |
| title | Nanocomposite tantalum–carbon-based films deposited by femtosecond pulsed laser ablation |
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