Nonadiabatic alignment of asymmetric top molecules: field-free alignment of iodobenzene

Nonadiabatic alignment of asymmetric top molecules: field-free alignment of iodobenzene

Nonadiabatic laser alignment of an asymmetric top molecule is studied using the combination of a quantum dynamical theory and time-resolved photofragment imaging experiments. In particular, the degree of alignment of iodobenzene, induced by an intense, linearly polarized picosecond laser pulse, is c...

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Veröffentlicht in:Physical review letters 2003-07, Vol.91 (4), p.043003-043003, Article 043003
Hauptverfasser: Péronne, Emmanuel, Poulsen, Mikael D, Bisgaard, Christer Z, Stapelfeldt, Henrik, Seideman, Tamar
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container_issue 4
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container_title Physical review letters
container_volume 91
creator Péronne, Emmanuel
Poulsen, Mikael D
Bisgaard, Christer Z
Stapelfeldt, Henrik
Seideman, Tamar
description Nonadiabatic laser alignment of an asymmetric top molecule is studied using the combination of a quantum dynamical theory and time-resolved photofragment imaging experiments. In particular, the degree of alignment of iodobenzene, induced by an intense, linearly polarized picosecond laser pulse, is calculated and measured. Pronounced alignment is obtained under field-free conditions.
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title Nonadiabatic alignment of asymmetric top molecules: field-free alignment of iodobenzene
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