Synthesis and post-synthetic modification of UiO-67 type metal-organic frameworks by mechanochemistry
[Display omitted] Herein, we report the synthesis of zirconium metal-organic frameworks by a mechanochemical route. The frameworks are obtained by the coordination of a zirconium cluster with the biphenyldicarboxylic acid linker to obtain UiO-67 or with the iso-structural 2,2′-bipyridine-5,5′-dicarb...
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| Veröffentlicht in: | Materials letters 2017-06, Vol.197, p.171-174 |
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| container_end_page | 174 |
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| container_title | Materials letters |
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| creator | Ali-Moussa, Habiba Navarro Amador, Ricardo Martinez, Jean Lamaty, Frédéric Carboni, Michaël Bantreil, Xavier |
| description | [Display omitted]
Herein, we report the synthesis of zirconium metal-organic frameworks by a mechanochemical route. The frameworks are obtained by the coordination of a zirconium cluster with the biphenyldicarboxylic acid linker to obtain UiO-67 or with the iso-structural 2,2′-bipyridine-5,5′-dicarboxylic acid to access to a functional MOF (UiO-67-bpy). In a second mechanochemical reaction, it has been possible to coordinate by post-synthetic modification a copper salt on each bipyridine site (UiO-67-bpy-Cu). Both materials exhibit crystallinity and porosity (up to 750m2/g) showing the possibility to get access to elaborated materials in a cleaner way than the classical solvothermal route in DMF. |
| doi_str_mv | 10.1016/j.matlet.2017.03.140 |
| format | Article |
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Herein, we report the synthesis of zirconium metal-organic frameworks by a mechanochemical route. The frameworks are obtained by the coordination of a zirconium cluster with the biphenyldicarboxylic acid linker to obtain UiO-67 or with the iso-structural 2,2′-bipyridine-5,5′-dicarboxylic acid to access to a functional MOF (UiO-67-bpy). In a second mechanochemical reaction, it has been possible to coordinate by post-synthetic modification a copper salt on each bipyridine site (UiO-67-bpy-Cu). Both materials exhibit crystallinity and porosity (up to 750m2/g) showing the possibility to get access to elaborated materials in a cleaner way than the classical solvothermal route in DMF.</description><identifier>ISSN: 0167-577X</identifier><identifier>EISSN: 1873-4979</identifier><identifier>DOI: 10.1016/j.matlet.2017.03.140</identifier><language>eng</language><publisher>Amsterdam: Elsevier B.V</publisher><subject>Ball milling ; Ball-mill ; Chemical Sciences ; Copper ; Functional porous material ; Inorganic chemistry ; Material chemistry ; Materials science ; Mechanochemistry ; Metal-organic framework ; Metal-organic frameworks ; Organic chemistry ; Porosity ; Solvent-free reaction ; Synthesis ; Zirconium</subject><ispartof>Materials letters, 2017-06, Vol.197, p.171-174</ispartof><rights>2017 Elsevier B.V.</rights><rights>Copyright Elsevier BV Jun 15, 2017</rights><rights>Distributed under a Creative Commons Attribution 4.0 International License</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c414t-5dccb19de79908f75ac45a3f9a96a3fa4b1184f76cc90b182cb81501ed2a623f3</citedby><cites>FETCH-LOGICAL-c414t-5dccb19de79908f75ac45a3f9a96a3fa4b1184f76cc90b182cb81501ed2a623f3</cites><orcidid>0000-0003-2213-9276 ; 0000-0002-2676-6851 ; 0000-0002-9267-4621</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktohtml>$$Uhttps://dx.doi.org/10.1016/j.matlet.2017.03.140$$EHTML$$P50$$Gelsevier$$H</linktohtml><link.rule.ids>230,314,780,784,885,3550,27924,27925,45995</link.rule.ids><backlink>$$Uhttps://cea.hal.science/cea-01997875$$DView record in HAL$$Hfree_for_read</backlink></links><search><creatorcontrib>Ali-Moussa, Habiba</creatorcontrib><creatorcontrib>Navarro Amador, Ricardo</creatorcontrib><creatorcontrib>Martinez, Jean</creatorcontrib><creatorcontrib>Lamaty, Frédéric</creatorcontrib><creatorcontrib>Carboni, Michaël</creatorcontrib><creatorcontrib>Bantreil, Xavier</creatorcontrib><title>Synthesis and post-synthetic modification of UiO-67 type metal-organic frameworks by mechanochemistry</title><title>Materials letters</title><description>[Display omitted]
Herein, we report the synthesis of zirconium metal-organic frameworks by a mechanochemical route. The frameworks are obtained by the coordination of a zirconium cluster with the biphenyldicarboxylic acid linker to obtain UiO-67 or with the iso-structural 2,2′-bipyridine-5,5′-dicarboxylic acid to access to a functional MOF (UiO-67-bpy). In a second mechanochemical reaction, it has been possible to coordinate by post-synthetic modification a copper salt on each bipyridine site (UiO-67-bpy-Cu). Both materials exhibit crystallinity and porosity (up to 750m2/g) showing the possibility to get access to elaborated materials in a cleaner way than the classical solvothermal route in DMF.</description><subject>Ball milling</subject><subject>Ball-mill</subject><subject>Chemical Sciences</subject><subject>Copper</subject><subject>Functional porous material</subject><subject>Inorganic chemistry</subject><subject>Material chemistry</subject><subject>Materials science</subject><subject>Mechanochemistry</subject><subject>Metal-organic framework</subject><subject>Metal-organic frameworks</subject><subject>Organic chemistry</subject><subject>Porosity</subject><subject>Solvent-free reaction</subject><subject>Synthesis</subject><subject>Zirconium</subject><issn>0167-577X</issn><issn>1873-4979</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2017</creationdate><recordtype>article</recordtype><recordid>eNp9kEFr3DAQhUVJoZu0_6AHQ0452NXYsmVdAiGkTWEhhzbQmxjLo662a2sjKSn-91XqkGNOD2a-95h5jH0GXgGH7su-mjAdKFU1B1nxpgLB37EN9LIphZLqhG0yJstWyl8f2GmMe865UFxsGP1Y5rSj6GKB81gcfUxl_D9KzhSTH511BpPzc-Ftce_uyk4WaTlSMVHCQ-nDb5wzaQNO9NeHP7EYlrwzO5y92dHkYgrLR_be4iHSpxc9Y_dfb35e35bbu2_fr6-2pREgUtmOxgygRpJK8d7KFo1osbEKVZcFxQDQCys7YxQfoK_N0EPLgcYau7qxzRm7WHN3eNDH4CYMi_bo9O3VVhtCzUEp2cv2CTJ7vrLH4B8eKSa9949hzudpUKLpat4olSmxUib4GAPZ11jg-rl8vddr-fq5fM0bncvPtsvVRvnbJ0dBR-NoNjS6QCbp0bu3A_4Bs6WQOg</recordid><startdate>20170615</startdate><enddate>20170615</enddate><creator>Ali-Moussa, Habiba</creator><creator>Navarro Amador, Ricardo</creator><creator>Martinez, Jean</creator><creator>Lamaty, Frédéric</creator><creator>Carboni, Michaël</creator><creator>Bantreil, Xavier</creator><general>Elsevier B.V</general><general>Elsevier BV</general><general>Elsevier</general><scope>AAYXX</scope><scope>CITATION</scope><scope>7SR</scope><scope>8BQ</scope><scope>8FD</scope><scope>JG9</scope><scope>1XC</scope><orcidid>https://orcid.org/0000-0003-2213-9276</orcidid><orcidid>https://orcid.org/0000-0002-2676-6851</orcidid><orcidid>https://orcid.org/0000-0002-9267-4621</orcidid></search><sort><creationdate>20170615</creationdate><title>Synthesis and post-synthetic modification of UiO-67 type metal-organic frameworks by mechanochemistry</title><author>Ali-Moussa, Habiba ; Navarro Amador, Ricardo ; Martinez, Jean ; Lamaty, Frédéric ; Carboni, Michaël ; Bantreil, Xavier</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c414t-5dccb19de79908f75ac45a3f9a96a3fa4b1184f76cc90b182cb81501ed2a623f3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2017</creationdate><topic>Ball milling</topic><topic>Ball-mill</topic><topic>Chemical Sciences</topic><topic>Copper</topic><topic>Functional porous material</topic><topic>Inorganic chemistry</topic><topic>Material chemistry</topic><topic>Materials science</topic><topic>Mechanochemistry</topic><topic>Metal-organic framework</topic><topic>Metal-organic frameworks</topic><topic>Organic chemistry</topic><topic>Porosity</topic><topic>Solvent-free reaction</topic><topic>Synthesis</topic><topic>Zirconium</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Ali-Moussa, Habiba</creatorcontrib><creatorcontrib>Navarro Amador, Ricardo</creatorcontrib><creatorcontrib>Martinez, Jean</creatorcontrib><creatorcontrib>Lamaty, Frédéric</creatorcontrib><creatorcontrib>Carboni, Michaël</creatorcontrib><creatorcontrib>Bantreil, Xavier</creatorcontrib><collection>CrossRef</collection><collection>Engineered Materials Abstracts</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>Materials Research Database</collection><collection>Hyper Article en Ligne (HAL)</collection><jtitle>Materials letters</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Ali-Moussa, Habiba</au><au>Navarro Amador, Ricardo</au><au>Martinez, Jean</au><au>Lamaty, Frédéric</au><au>Carboni, Michaël</au><au>Bantreil, Xavier</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Synthesis and post-synthetic modification of UiO-67 type metal-organic frameworks by mechanochemistry</atitle><jtitle>Materials letters</jtitle><date>2017-06-15</date><risdate>2017</risdate><volume>197</volume><spage>171</spage><epage>174</epage><pages>171-174</pages><issn>0167-577X</issn><eissn>1873-4979</eissn><abstract>[Display omitted]
Herein, we report the synthesis of zirconium metal-organic frameworks by a mechanochemical route. The frameworks are obtained by the coordination of a zirconium cluster with the biphenyldicarboxylic acid linker to obtain UiO-67 or with the iso-structural 2,2′-bipyridine-5,5′-dicarboxylic acid to access to a functional MOF (UiO-67-bpy). In a second mechanochemical reaction, it has been possible to coordinate by post-synthetic modification a copper salt on each bipyridine site (UiO-67-bpy-Cu). Both materials exhibit crystallinity and porosity (up to 750m2/g) showing the possibility to get access to elaborated materials in a cleaner way than the classical solvothermal route in DMF.</abstract><cop>Amsterdam</cop><pub>Elsevier B.V</pub><doi>10.1016/j.matlet.2017.03.140</doi><tpages>4</tpages><orcidid>https://orcid.org/0000-0003-2213-9276</orcidid><orcidid>https://orcid.org/0000-0002-2676-6851</orcidid><orcidid>https://orcid.org/0000-0002-9267-4621</orcidid><oa>free_for_read</oa></addata></record> |
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| subjects | Ball milling Ball-mill Chemical Sciences Copper Functional porous material Inorganic chemistry Material chemistry Materials science Mechanochemistry Metal-organic framework Metal-organic frameworks Organic chemistry Porosity Solvent-free reaction Synthesis Zirconium |
| title | Synthesis and post-synthetic modification of UiO-67 type metal-organic frameworks by mechanochemistry |
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