Superconducting HfO2-YBa2Cu3O7-δ nanocomposite films deposited using ink-jet printing of colloidal solutions

To reduce the fabrication costs while maximizing the superconducting and pinning properties of YBa2Cu3O7−δ (YBCO) nanocomposite films, the drop-on-demand ink-jet printing technique was used to deposit colloidal YBCO inks onto LaAlO3 substrates. These inks containing preformed HfO2 nanocrystals were...

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Hauptverfasser: Rijckaert, Hannes, Cayado, Pablo, Nast, Rainer, Diez Sierra, Javier, Erbe, Manuela, López Domínguez, Pedro, Hänisch, Jens, De Buysser, Klaartje, Holzapfel, Bernhard, Van Driessche, Isabel
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creator Rijckaert, Hannes
Cayado, Pablo
Nast, Rainer
Diez Sierra, Javier
Erbe, Manuela
López Domínguez, Pedro
Hänisch, Jens
De Buysser, Klaartje
Holzapfel, Bernhard
Van Driessche, Isabel
description To reduce the fabrication costs while maximizing the superconducting and pinning properties of YBa2Cu3O7−δ (YBCO) nanocomposite films, the drop-on-demand ink-jet printing technique was used to deposit colloidal YBCO inks onto LaAlO3 substrates. These inks containing preformed HfO2 nanocrystals were carefully adjusted, prior to the jettability, as the droplet formation depends on the rheological properties of the inks themselves. After carefully adjusting printing parameters, 450-nm thick pristine YBCO films with a self-field critical current density (Jc) of 2.7 MA cm−² at 77 K and 500-nm thick HfO2-YBCO nanocomposite films with a self-field Jc of 3.1 MA·cm−² at 77 K were achieved. The final HfO2-YBCO nanocomposite films contained dispersed BaHfO3 particles in a YBCO matrix due to the Ba2+ reactivity with the HfO2 nanocrystals. These nanocomposite films presented a more gradual decrease of Jc with the increased magnetic field. These nanocomposite films also showed higher pinning force densities than the pristine films. This pinning enhancement was related to the favorable size and distribution of the BaHfO3 particles in the YBCO matrix.
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source MDPI - Multidisciplinary Digital Publishing Institute; Ghent University Academic Bibliography; EZB-FREE-00999 freely available EZB journals; Alma/SFX Local Collection
subjects chemical solution deposition
Chemistry
COATED CONDUCTORS
CRITICAL-CURRENT DENSITY
ink-jet printing
METAL-ORGANIC-DEPOSITION
nanocomposite
nanoparticles
OXIDE NANOCRYSTALS
Physics and Astronomy
STABILIZATION
superconductor
SURFACE-CHEMISTRY
thin film
THIN-FILMS
YBCO
title Superconducting HfO2-YBa2Cu3O7-δ nanocomposite films deposited using ink-jet printing of colloidal solutions
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