Boric-acid-modified Fe.sub.3O.sub.4@PDA@UiO-66 for enrichment and detection of glucose by matrix-assisted laser desorption/ionization time-of-flight mass spectrometry

Boric-acid-modified Fe.sub.3O.sub.4@PDA@UiO-66 for enrichment and detection of glucose by matrix-assisted laser desorption/ionization time-of-flight mass spectrometry

Herein, boric-acid-modified multifunctional Zr-based metal-organic frameworks (denoted as Fe.sub.3O.sub.4@PDA@B-UiO-66) were synthesized by hydrothermal reaction and surface modification. Compared to traditional matrix, Fe.sub.3O.sub.4@PDA@B-UiO-66 has the advantages of high ionization efficiency, h...

Ausführliche Beschreibung

Gespeichert in:
Bibliographische Detailangaben
Veröffentlicht in:Analytical and bioanalytical chemistry 2020-11, Vol.412 (29), p.8083
Hauptverfasser: Li, Zhijian, Huo, Panpan, Gong, Congcong, Deng, Chunhui, Pu, Shouzhi
Format: Artikel
Sprache:eng
Schlagworte:
Dextrose
Glucose
Mass spectrometry
Online-Zugang:Volltext
Tags: Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
container_end_page
container_issue 29
container_start_page 8083
container_title Analytical and bioanalytical chemistry
container_volume 412
creator Li, Zhijian
Huo, Panpan
Gong, Congcong
Deng, Chunhui
Pu, Shouzhi
description Herein, boric-acid-modified multifunctional Zr-based metal-organic frameworks (denoted as Fe.sub.3O.sub.4@PDA@B-UiO-66) were synthesized by hydrothermal reaction and surface modification. Compared to traditional matrix, Fe.sub.3O.sub.4@PDA@B-UiO-66 has the advantages of high ionization efficiency, high surface area, low matrix background, porous structure, and numerous boric-acid-active sites. By combining matrix-assisted laser desorption/ionization time-of-flight mass spectrometry (MALDI-TOF MS), Fe.sub.3O.sub.4@PDA@B-UiO-66 was used as an adsorbent and matrix for enrichment and detection of glucose, based on a specific reaction between boric acid and glucose. The limit of detection was 58.5 nM. The proposed method provides a simple and efficient approach for the sensitive and quantitative detection of glucose in complex samples based on MALDI-TOF MS.
doi_str_mv 10.1007/s00216-020-02935-8
format Article
fullrecord <record><control><sourceid>gale</sourceid><recordid>TN_cdi_gale_infotracmisc_A639327825</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><galeid>A639327825</galeid><sourcerecordid>A639327825</sourcerecordid><originalsourceid>FETCH-LOGICAL-g675-bb3aa123bf2f7acfad89929ce6a8791b2a644f54798320cf25ef6f504a416d643</originalsourceid><addsrcrecordid>eNptjMtKAzEYhbNQsFZfwFXAddrcJjOza61WhUJd1HXJ5DKNzExKkoL1gXxOY3XhQn4OB36-7wBwQ_CEYFxOI8aUCIQpzqlZgaozMCKCVIgKTi_AZYxvGJOiImIEPu98cApJ5TTqvXbWGQ2XZhIPzYStT8VnL_fz2atbIyGg9QGaISu73gwJykFDbZJRyfkBegvb7qB8NLA5wl6m4N6RjNHFlFc7GU3IdPRh_41Pc9yHPJnJ9QZ5i2zn2l3Kaoww7vNs8L1J4XgFzq3sorn-7THYLB82iye0Wj8-L-Yr1IqyQE3DpCSUNZbaUiordVXXtFZGyKqsSUOl4NwWvKwrRrGytDBW2AJzyYnQgrMxuP2ZbWVntm6wPgWpehfVdi5YzWhZ0SJTk3-ofNr0TvnBWJf_f4Qvs7Z-Lw</addsrcrecordid><sourcetype>Aggregation Database</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype></control><display><type>article</type><title>Boric-acid-modified Fe.sub.3O.sub.4@PDA@UiO-66 for enrichment and detection of glucose by matrix-assisted laser desorption/ionization time-of-flight mass spectrometry</title><source>SpringerLink Journals - AutoHoldings</source><creator>Li, Zhijian ; Huo, Panpan ; Gong, Congcong ; Deng, Chunhui ; Pu, Shouzhi</creator><creatorcontrib>Li, Zhijian ; Huo, Panpan ; Gong, Congcong ; Deng, Chunhui ; Pu, Shouzhi</creatorcontrib><description>Herein, boric-acid-modified multifunctional Zr-based metal-organic frameworks (denoted as Fe.sub.3O.sub.4@PDA@B-UiO-66) were synthesized by hydrothermal reaction and surface modification. Compared to traditional matrix, Fe.sub.3O.sub.4@PDA@B-UiO-66 has the advantages of high ionization efficiency, high surface area, low matrix background, porous structure, and numerous boric-acid-active sites. By combining matrix-assisted laser desorption/ionization time-of-flight mass spectrometry (MALDI-TOF MS), Fe.sub.3O.sub.4@PDA@B-UiO-66 was used as an adsorbent and matrix for enrichment and detection of glucose, based on a specific reaction between boric acid and glucose. The limit of detection was 58.5 nM. The proposed method provides a simple and efficient approach for the sensitive and quantitative detection of glucose in complex samples based on MALDI-TOF MS.</description><identifier>ISSN: 1618-2642</identifier><identifier>DOI: 10.1007/s00216-020-02935-8</identifier><language>eng</language><publisher>Springer</publisher><subject>Dextrose ; Glucose ; Mass spectrometry</subject><ispartof>Analytical and bioanalytical chemistry, 2020-11, Vol.412 (29), p.8083</ispartof><rights>COPYRIGHT 2020 Springer</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,780,784,27924,27925</link.rule.ids></links><search><creatorcontrib>Li, Zhijian</creatorcontrib><creatorcontrib>Huo, Panpan</creatorcontrib><creatorcontrib>Gong, Congcong</creatorcontrib><creatorcontrib>Deng, Chunhui</creatorcontrib><creatorcontrib>Pu, Shouzhi</creatorcontrib><title>Boric-acid-modified Fe.sub.3O.sub.4@PDA@UiO-66 for enrichment and detection of glucose by matrix-assisted laser desorption/ionization time-of-flight mass spectrometry</title><title>Analytical and bioanalytical chemistry</title><description>Herein, boric-acid-modified multifunctional Zr-based metal-organic frameworks (denoted as Fe.sub.3O.sub.4@PDA@B-UiO-66) were synthesized by hydrothermal reaction and surface modification. Compared to traditional matrix, Fe.sub.3O.sub.4@PDA@B-UiO-66 has the advantages of high ionization efficiency, high surface area, low matrix background, porous structure, and numerous boric-acid-active sites. By combining matrix-assisted laser desorption/ionization time-of-flight mass spectrometry (MALDI-TOF MS), Fe.sub.3O.sub.4@PDA@B-UiO-66 was used as an adsorbent and matrix for enrichment and detection of glucose, based on a specific reaction between boric acid and glucose. The limit of detection was 58.5 nM. The proposed method provides a simple and efficient approach for the sensitive and quantitative detection of glucose in complex samples based on MALDI-TOF MS.</description><subject>Dextrose</subject><subject>Glucose</subject><subject>Mass spectrometry</subject><issn>1618-2642</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2020</creationdate><recordtype>article</recordtype><sourceid/><recordid>eNptjMtKAzEYhbNQsFZfwFXAddrcJjOza61WhUJd1HXJ5DKNzExKkoL1gXxOY3XhQn4OB36-7wBwQ_CEYFxOI8aUCIQpzqlZgaozMCKCVIgKTi_AZYxvGJOiImIEPu98cApJ5TTqvXbWGQ2XZhIPzYStT8VnL_fz2atbIyGg9QGaISu73gwJykFDbZJRyfkBegvb7qB8NLA5wl6m4N6RjNHFlFc7GU3IdPRh_41Pc9yHPJnJ9QZ5i2zn2l3Kaoww7vNs8L1J4XgFzq3sorn-7THYLB82iye0Wj8-L-Yr1IqyQE3DpCSUNZbaUiordVXXtFZGyKqsSUOl4NwWvKwrRrGytDBW2AJzyYnQgrMxuP2ZbWVntm6wPgWpehfVdi5YzWhZ0SJTk3-ofNr0TvnBWJf_f4Qvs7Z-Lw</recordid><startdate>20201101</startdate><enddate>20201101</enddate><creator>Li, Zhijian</creator><creator>Huo, Panpan</creator><creator>Gong, Congcong</creator><creator>Deng, Chunhui</creator><creator>Pu, Shouzhi</creator><general>Springer</general><scope/></search><sort><creationdate>20201101</creationdate><title>Boric-acid-modified Fe.sub.3O.sub.4@PDA@UiO-66 for enrichment and detection of glucose by matrix-assisted laser desorption/ionization time-of-flight mass spectrometry</title><author>Li, Zhijian ; Huo, Panpan ; Gong, Congcong ; Deng, Chunhui ; Pu, Shouzhi</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-g675-bb3aa123bf2f7acfad89929ce6a8791b2a644f54798320cf25ef6f504a416d643</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2020</creationdate><topic>Dextrose</topic><topic>Glucose</topic><topic>Mass spectrometry</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Li, Zhijian</creatorcontrib><creatorcontrib>Huo, Panpan</creatorcontrib><creatorcontrib>Gong, Congcong</creatorcontrib><creatorcontrib>Deng, Chunhui</creatorcontrib><creatorcontrib>Pu, Shouzhi</creatorcontrib><jtitle>Analytical and bioanalytical chemistry</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Li, Zhijian</au><au>Huo, Panpan</au><au>Gong, Congcong</au><au>Deng, Chunhui</au><au>Pu, Shouzhi</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Boric-acid-modified Fe.sub.3O.sub.4@PDA@UiO-66 for enrichment and detection of glucose by matrix-assisted laser desorption/ionization time-of-flight mass spectrometry</atitle><jtitle>Analytical and bioanalytical chemistry</jtitle><date>2020-11-01</date><risdate>2020</risdate><volume>412</volume><issue>29</issue><spage>8083</spage><pages>8083-</pages><issn>1618-2642</issn><abstract>Herein, boric-acid-modified multifunctional Zr-based metal-organic frameworks (denoted as Fe.sub.3O.sub.4@PDA@B-UiO-66) were synthesized by hydrothermal reaction and surface modification. Compared to traditional matrix, Fe.sub.3O.sub.4@PDA@B-UiO-66 has the advantages of high ionization efficiency, high surface area, low matrix background, porous structure, and numerous boric-acid-active sites. By combining matrix-assisted laser desorption/ionization time-of-flight mass spectrometry (MALDI-TOF MS), Fe.sub.3O.sub.4@PDA@B-UiO-66 was used as an adsorbent and matrix for enrichment and detection of glucose, based on a specific reaction between boric acid and glucose. The limit of detection was 58.5 nM. The proposed method provides a simple and efficient approach for the sensitive and quantitative detection of glucose in complex samples based on MALDI-TOF MS.</abstract><pub>Springer</pub><doi>10.1007/s00216-020-02935-8</doi></addata></record>
fulltext fulltext
identifier ISSN: 1618-2642
ispartof Analytical and bioanalytical chemistry, 2020-11, Vol.412 (29), p.8083
issn 1618-2642
language eng
recordid cdi_gale_infotracmisc_A639327825
source SpringerLink Journals - AutoHoldings
subjects Dextrose
Glucose
Mass spectrometry
title Boric-acid-modified Fe.sub.3O.sub.4@PDA@UiO-66 for enrichment and detection of glucose by matrix-assisted laser desorption/ionization time-of-flight mass spectrometry
url https://sfx.bib-bvb.de/sfx_tum?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2025-01-05T13%3A31%3A48IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-gale&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=Boric-acid-modified%20Fe.sub.3O.sub.4@PDA@UiO-66%20for%20enrichment%20and%20detection%20of%20glucose%20by%20matrix-assisted%20laser%20desorption/ionization%20time-of-flight%20mass%20spectrometry&rft.jtitle=Analytical%20and%20bioanalytical%20chemistry&rft.au=Li,%20Zhijian&rft.date=2020-11-01&rft.volume=412&rft.issue=29&rft.spage=8083&rft.pages=8083-&rft.issn=1618-2642&rft_id=info:doi/10.1007/s00216-020-02935-8&rft_dat=%3Cgale%3EA639327825%3C/gale%3E%3Curl%3E%3C/url%3E&disable_directlink=true&sfx.directlink=off&sfx.report_link=0&rft_id=info:oai/&rft_id=info:pmid/&rft_galeid=A639327825&rfr_iscdi=true