Preparation method and application of oxygen carrier for low-temperature methane oxidation hydrogen production

The invention relates to a preparation method of an oxygen carrier for hydrogen production by low-temperature methane oxidation and application of the oxygen carrier, and belongs to the field of methane low-temperature catalysis. Magnesium oxide is prepared by adopting a homogeneous precipitation me...

Ausführliche Beschreibung

Gespeichert in:
Bibliographische Detailangaben
Hauptverfasser: HUANG ZE'AI, CHE YU'ANG, ZHOU YING, WANG JUNBU, ZHANG RUIYANG
Format: Patent
Sprache:chi ; eng
Schlagworte:
Online-Zugang:Volltext bestellen
Tags: Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
container_end_page
container_issue
container_start_page
container_title
container_volume
creator HUANG ZE'AI
CHE YU'ANG
ZHOU YING
WANG JUNBU
ZHANG RUIYANG
description The invention relates to a preparation method of an oxygen carrier for hydrogen production by low-temperature methane oxidation and application of the oxygen carrier, and belongs to the field of methane low-temperature catalysis. Magnesium oxide is prepared by adopting a homogeneous precipitation method and a high-temperature calcination method; magnesium oxide and copper salt are mixed and modified, and the composite CuMgO oxygen carrier is obtained. The preparation method of the oxygen carrier is simple, the oxygen carrier can be used in a low-temperature range, and the recycling efficiency is good. The catalyst can efficiently convert methane into hydrogen at low temperature by using lattice oxygen of the catalyst, the hydrogen selectivity is greater than 97%, and the catalyst can be regenerated in a carbon dioxide atmosphere. After a plurality of circular reactions for a long time, the oxygen carrier can still convert methane into hydrogen, and stable hydrogen production selectivity is maintained. The oxy
format Patent
fullrecord <record><control><sourceid>epo_EVB</sourceid><recordid>TN_cdi_epo_espacenet_CN114920279A</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>CN114920279A</sourcerecordid><originalsourceid>FETCH-epo_espacenet_CN114920279A3</originalsourceid><addsrcrecordid>eNqNi0EKwjAQRbtxIeod4gEKtgrSpRTFlbhwX4ZkYgNpZpimaG9vaj2Ai8-Hx3vLLNwFGQSio6A6jC0ZBSGN2Ts9Y7KK3uMTg9Ig4lCUJVGeXnnEjjHFg-A3hoBJdWbu2tEITRkLmUFPbJ0tLPgeN79fZdvL-VFfc2RqsGfQGDA29a0oDlW5K4_Vaf-P8wFUSkPL</addsrcrecordid><sourcetype>Open Access Repository</sourcetype><iscdi>true</iscdi><recordtype>patent</recordtype></control><display><type>patent</type><title>Preparation method and application of oxygen carrier for low-temperature methane oxidation hydrogen production</title><source>esp@cenet</source><creator>HUANG ZE'AI ; CHE YU'ANG ; ZHOU YING ; WANG JUNBU ; ZHANG RUIYANG</creator><creatorcontrib>HUANG ZE'AI ; CHE YU'ANG ; ZHOU YING ; WANG JUNBU ; ZHANG RUIYANG</creatorcontrib><description>The invention relates to a preparation method of an oxygen carrier for hydrogen production by low-temperature methane oxidation and application of the oxygen carrier, and belongs to the field of methane low-temperature catalysis. Magnesium oxide is prepared by adopting a homogeneous precipitation method and a high-temperature calcination method; magnesium oxide and copper salt are mixed and modified, and the composite CuMgO oxygen carrier is obtained. The preparation method of the oxygen carrier is simple, the oxygen carrier can be used in a low-temperature range, and the recycling efficiency is good. The catalyst can efficiently convert methane into hydrogen at low temperature by using lattice oxygen of the catalyst, the hydrogen selectivity is greater than 97%, and the catalyst can be regenerated in a carbon dioxide atmosphere. After a plurality of circular reactions for a long time, the oxygen carrier can still convert methane into hydrogen, and stable hydrogen production selectivity is maintained. The oxy</description><language>chi ; eng</language><subject>CHEMISTRY ; COMPOUNDS CONTAINING METALS NOT COVERED BY SUBCLASSESC01D OR C01F ; COMPOUNDS OF THE METALS BERYLLIUM, MAGNESIUM, ALUMINIUM,CALCIUM, STRONTIUM, BARIUM, RADIUM, THORIUM, OR OF THERARE-EARTH METALS ; COMPOUNDS THEREOF ; INORGANIC CHEMISTRY ; MANUFACTURE OR TREATMENT OF NANOSTRUCTURES ; MEASUREMENT OR ANALYSIS OF NANOSTRUCTURES ; METALLURGY ; NANOTECHNOLOGY ; NON-METALLIC ELEMENTS ; PERFORMING OPERATIONS ; SPECIFIC USES OR APPLICATIONS OF NANOSTRUCTURES ; TRANSPORTING</subject><creationdate>2022</creationdate><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktohtml>$$Uhttps://worldwide.espacenet.com/publicationDetails/biblio?FT=D&amp;date=20220819&amp;DB=EPODOC&amp;CC=CN&amp;NR=114920279A$$EHTML$$P50$$Gepo$$Hfree_for_read</linktohtml><link.rule.ids>230,308,776,881,25543,76293</link.rule.ids><linktorsrc>$$Uhttps://worldwide.espacenet.com/publicationDetails/biblio?FT=D&amp;date=20220819&amp;DB=EPODOC&amp;CC=CN&amp;NR=114920279A$$EView_record_in_European_Patent_Office$$FView_record_in_$$GEuropean_Patent_Office$$Hfree_for_read</linktorsrc></links><search><creatorcontrib>HUANG ZE'AI</creatorcontrib><creatorcontrib>CHE YU'ANG</creatorcontrib><creatorcontrib>ZHOU YING</creatorcontrib><creatorcontrib>WANG JUNBU</creatorcontrib><creatorcontrib>ZHANG RUIYANG</creatorcontrib><title>Preparation method and application of oxygen carrier for low-temperature methane oxidation hydrogen production</title><description>The invention relates to a preparation method of an oxygen carrier for hydrogen production by low-temperature methane oxidation and application of the oxygen carrier, and belongs to the field of methane low-temperature catalysis. Magnesium oxide is prepared by adopting a homogeneous precipitation method and a high-temperature calcination method; magnesium oxide and copper salt are mixed and modified, and the composite CuMgO oxygen carrier is obtained. The preparation method of the oxygen carrier is simple, the oxygen carrier can be used in a low-temperature range, and the recycling efficiency is good. The catalyst can efficiently convert methane into hydrogen at low temperature by using lattice oxygen of the catalyst, the hydrogen selectivity is greater than 97%, and the catalyst can be regenerated in a carbon dioxide atmosphere. After a plurality of circular reactions for a long time, the oxygen carrier can still convert methane into hydrogen, and stable hydrogen production selectivity is maintained. The oxy</description><subject>CHEMISTRY</subject><subject>COMPOUNDS CONTAINING METALS NOT COVERED BY SUBCLASSESC01D OR C01F</subject><subject>COMPOUNDS OF THE METALS BERYLLIUM, MAGNESIUM, ALUMINIUM,CALCIUM, STRONTIUM, BARIUM, RADIUM, THORIUM, OR OF THERARE-EARTH METALS</subject><subject>COMPOUNDS THEREOF</subject><subject>INORGANIC CHEMISTRY</subject><subject>MANUFACTURE OR TREATMENT OF NANOSTRUCTURES</subject><subject>MEASUREMENT OR ANALYSIS OF NANOSTRUCTURES</subject><subject>METALLURGY</subject><subject>NANOTECHNOLOGY</subject><subject>NON-METALLIC ELEMENTS</subject><subject>PERFORMING OPERATIONS</subject><subject>SPECIFIC USES OR APPLICATIONS OF NANOSTRUCTURES</subject><subject>TRANSPORTING</subject><fulltext>true</fulltext><rsrctype>patent</rsrctype><creationdate>2022</creationdate><recordtype>patent</recordtype><sourceid>EVB</sourceid><recordid>eNqNi0EKwjAQRbtxIeod4gEKtgrSpRTFlbhwX4ZkYgNpZpimaG9vaj2Ai8-Hx3vLLNwFGQSio6A6jC0ZBSGN2Ts9Y7KK3uMTg9Ig4lCUJVGeXnnEjjHFg-A3hoBJdWbu2tEITRkLmUFPbJ0tLPgeN79fZdvL-VFfc2RqsGfQGDA29a0oDlW5K4_Vaf-P8wFUSkPL</recordid><startdate>20220819</startdate><enddate>20220819</enddate><creator>HUANG ZE'AI</creator><creator>CHE YU'ANG</creator><creator>ZHOU YING</creator><creator>WANG JUNBU</creator><creator>ZHANG RUIYANG</creator><scope>EVB</scope></search><sort><creationdate>20220819</creationdate><title>Preparation method and application of oxygen carrier for low-temperature methane oxidation hydrogen production</title><author>HUANG ZE'AI ; CHE YU'ANG ; ZHOU YING ; WANG JUNBU ; ZHANG RUIYANG</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-epo_espacenet_CN114920279A3</frbrgroupid><rsrctype>patents</rsrctype><prefilter>patents</prefilter><language>chi ; eng</language><creationdate>2022</creationdate><topic>CHEMISTRY</topic><topic>COMPOUNDS CONTAINING METALS NOT COVERED BY SUBCLASSESC01D OR C01F</topic><topic>COMPOUNDS OF THE METALS BERYLLIUM, MAGNESIUM, ALUMINIUM,CALCIUM, STRONTIUM, BARIUM, RADIUM, THORIUM, OR OF THERARE-EARTH METALS</topic><topic>COMPOUNDS THEREOF</topic><topic>INORGANIC CHEMISTRY</topic><topic>MANUFACTURE OR TREATMENT OF NANOSTRUCTURES</topic><topic>MEASUREMENT OR ANALYSIS OF NANOSTRUCTURES</topic><topic>METALLURGY</topic><topic>NANOTECHNOLOGY</topic><topic>NON-METALLIC ELEMENTS</topic><topic>PERFORMING OPERATIONS</topic><topic>SPECIFIC USES OR APPLICATIONS OF NANOSTRUCTURES</topic><topic>TRANSPORTING</topic><toplevel>online_resources</toplevel><creatorcontrib>HUANG ZE'AI</creatorcontrib><creatorcontrib>CHE YU'ANG</creatorcontrib><creatorcontrib>ZHOU YING</creatorcontrib><creatorcontrib>WANG JUNBU</creatorcontrib><creatorcontrib>ZHANG RUIYANG</creatorcontrib><collection>esp@cenet</collection></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext_linktorsrc</fulltext></delivery><addata><au>HUANG ZE'AI</au><au>CHE YU'ANG</au><au>ZHOU YING</au><au>WANG JUNBU</au><au>ZHANG RUIYANG</au><format>patent</format><genre>patent</genre><ristype>GEN</ristype><title>Preparation method and application of oxygen carrier for low-temperature methane oxidation hydrogen production</title><date>2022-08-19</date><risdate>2022</risdate><abstract>The invention relates to a preparation method of an oxygen carrier for hydrogen production by low-temperature methane oxidation and application of the oxygen carrier, and belongs to the field of methane low-temperature catalysis. Magnesium oxide is prepared by adopting a homogeneous precipitation method and a high-temperature calcination method; magnesium oxide and copper salt are mixed and modified, and the composite CuMgO oxygen carrier is obtained. The preparation method of the oxygen carrier is simple, the oxygen carrier can be used in a low-temperature range, and the recycling efficiency is good. The catalyst can efficiently convert methane into hydrogen at low temperature by using lattice oxygen of the catalyst, the hydrogen selectivity is greater than 97%, and the catalyst can be regenerated in a carbon dioxide atmosphere. After a plurality of circular reactions for a long time, the oxygen carrier can still convert methane into hydrogen, and stable hydrogen production selectivity is maintained. The oxy</abstract><oa>free_for_read</oa></addata></record>
fulltext fulltext_linktorsrc
identifier
ispartof
issn
language chi ; eng
recordid cdi_epo_espacenet_CN114920279A
source esp@cenet
subjects CHEMISTRY
COMPOUNDS CONTAINING METALS NOT COVERED BY SUBCLASSESC01D OR C01F
COMPOUNDS OF THE METALS BERYLLIUM, MAGNESIUM, ALUMINIUM,CALCIUM, STRONTIUM, BARIUM, RADIUM, THORIUM, OR OF THERARE-EARTH METALS
COMPOUNDS THEREOF
INORGANIC CHEMISTRY
MANUFACTURE OR TREATMENT OF NANOSTRUCTURES
MEASUREMENT OR ANALYSIS OF NANOSTRUCTURES
METALLURGY
NANOTECHNOLOGY
NON-METALLIC ELEMENTS
PERFORMING OPERATIONS
SPECIFIC USES OR APPLICATIONS OF NANOSTRUCTURES
TRANSPORTING
title Preparation method and application of oxygen carrier for low-temperature methane oxidation hydrogen production
url https://sfx.bib-bvb.de/sfx_tum?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2025-01-26T11%3A40%3A51IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-epo_EVB&rft_val_fmt=info:ofi/fmt:kev:mtx:patent&rft.genre=patent&rft.au=HUANG%20ZE'AI&rft.date=2022-08-19&rft_id=info:doi/&rft_dat=%3Cepo_EVB%3ECN114920279A%3C/epo_EVB%3E%3Curl%3E%3C/url%3E&disable_directlink=true&sfx.directlink=off&sfx.report_link=0&rft_id=info:oai/&rft_id=info:pmid/&rfr_iscdi=true