Photoluminescence Enhancement by Surface-Plasmon Resonance: Recombination-Rate Theory and Experiments

Recombination rates were experimented with in colloidal mixtures of semiconductor/metal nanoparticles, and calculated as a function of semiconductor-metal distance. Radiative recombination rates were evaluated from the electrodynamical interactions between single-dipole emitter and a metal nanoparti...

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Veröffentlicht in:Applied physics express 2013-05, Vol.6 (5), p.052001-052001-3
Hauptverfasser: Nahm, Changwoo, Jung, Dae-Ryong, Kim, Jongmin, Nam, Seunghoon, Choi, Hongsik, Hong, Saeromi, Hwang, Taehyun, Moon, Taeho, Park, Byungwoo
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container_end_page 052001-3
container_issue 5
container_start_page 052001
container_title Applied physics express
container_volume 6
creator Nahm, Changwoo
Jung, Dae-Ryong
Kim, Jongmin
Nam, Seunghoon
Choi, Hongsik
Hong, Saeromi
Hwang, Taehyun
Moon, Taeho
Park, Byungwoo
description Recombination rates were experimented with in colloidal mixtures of semiconductor/metal nanoparticles, and calculated as a function of semiconductor-metal distance. Radiative recombination rates were evaluated from the electrodynamical interactions between single-dipole emitter and a metal nanoparticle, according to Mertens' 2007 model. Nonradiative recombination rates were obtained from the energy-transfer rate from a single exciton to the surface-plasmon band (analogous to Govorov's theory). This research verified that quantum-efficiency calculation based on carrier dynamics matches well with photoluminescence experiments by surface-plasmon resonance.
doi_str_mv 10.7567/APEX.6.052001
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title Photoluminescence Enhancement by Surface-Plasmon Resonance: Recombination-Rate Theory and Experiments
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