Electrochemical Performance of Plasma Sprayed Metal Supported Planar Solid Oxide Fuel Cells
High production cost is one of the major barriers to widespread commercialization of solid oxide fuel cells (SOFCs). Thermal spray techniques are a low cost alternative for the production of SOFCs. The objective of this work was to evaluate the electrochemical performance of cells produced by plasma...
Gespeichert in:
Veröffentlicht in: | Journal of the Electrochemical Society 2016-01, Vol.163 (9), p.F1059-F1065 |
---|---|
Hauptverfasser: | , , , |
Format: | Artikel |
Sprache: | eng |
Schlagworte: | |
Online-Zugang: | Volltext |
Tags: |
Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
|
container_end_page | F1065 |
---|---|
container_issue | 9 |
container_start_page | F1059 |
container_title | Journal of the Electrochemical Society |
container_volume | 163 |
creator | Gupta, M. Weber, A. Markocsan, N. Gindrat, M. |
description | High production cost is one of the major barriers to widespread commercialization of solid oxide fuel cells (SOFCs). Thermal spray techniques are a low cost alternative for the production of SOFCs. The objective of this work was to evaluate the electrochemical performance of cells produced by plasma spraying. The anode was deposited on a porous metallic support by atmospheric plasma spraying (APS) whereas the electrolyte was deposited by plasma spray-thin film (PS-TF) technique, which can produce thin and dense coatings at high deposition rates. The cathode was deposited by screen-printing and in-operando sintering. The electrochemical tests were performed at 650-800°C. Current-voltage characteristics and impedance spectra were measured and analyzed. The impact of electrolyte composition and layer thickness on the gas tightness of the electrolyte and the area specific resistance of the cell is discussed. The results show that the applied thermal spraying techniques are a potential alternative for producing SOFCs. |
doi_str_mv | 10.1149/2.0791609jes |
format | Article |
fullrecord | <record><control><sourceid>swepub_cross</sourceid><recordid>TN_cdi_crossref_primary_10_1149_2_0791609jes</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>oai_DiVA_org_hv_10045</sourcerecordid><originalsourceid>FETCH-LOGICAL-c412t-42ab3731414de204b6b9efe04cf4645d679ccc59235d4a7f1f316a3653e501ac3</originalsourceid><addsrcrecordid>eNpt0EFLwzAUB_AgCs7pzQ-Qo6CdeU3a2uOYmwqTDaZePIQ0fXEd6VKSVt23tzLRi6fHn_fjwfsTcg5sBCDy63jEshxSlm8wHJAB5CKJMgA4JAPGgEciTeCYnISw6SPciGxAXqcWdeudXmNdaWXpEr1xvlZbjdQZurQq1IquGq92WNJHbHuz6prG-bbP_XqrPF05W5V08VmVSGcdWjpBa8MpOTLKBjz7mUPyPJs-Te6j-eLuYTKeR1pA3EYiVgXPOAgQJcZMFGmRo0EmtBGpSMo0y7XWSR7zpBQqM2A4pIqnCceEgdJ8SC73d8MHNl0hG1_Vyu-kU5W8rV7G0vk3uX6XwJhIen2119q7EDyaXw9MftcoY_lXY88v9rxyjdy4zm_7V_6nX34mcsY</addsrcrecordid><sourcetype>Open Access Repository</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype></control><display><type>article</type><title>Electrochemical Performance of Plasma Sprayed Metal Supported Planar Solid Oxide Fuel Cells</title><source>IOP Publishing Journals</source><source>SWEPUB Freely available online</source><creator>Gupta, M. ; Weber, A. ; Markocsan, N. ; Gindrat, M.</creator><creatorcontrib>Gupta, M. ; Weber, A. ; Markocsan, N. ; Gindrat, M.</creatorcontrib><description>High production cost is one of the major barriers to widespread commercialization of solid oxide fuel cells (SOFCs). Thermal spray techniques are a low cost alternative for the production of SOFCs. The objective of this work was to evaluate the electrochemical performance of cells produced by plasma spraying. The anode was deposited on a porous metallic support by atmospheric plasma spraying (APS) whereas the electrolyte was deposited by plasma spray-thin film (PS-TF) technique, which can produce thin and dense coatings at high deposition rates. The cathode was deposited by screen-printing and in-operando sintering. The electrochemical tests were performed at 650-800°C. Current-voltage characteristics and impedance spectra were measured and analyzed. The impact of electrolyte composition and layer thickness on the gas tightness of the electrolyte and the area specific resistance of the cell is discussed. The results show that the applied thermal spraying techniques are a potential alternative for producing SOFCs.</description><identifier>ISSN: 0013-4651</identifier><identifier>ISSN: 1945-7111</identifier><identifier>EISSN: 1945-7111</identifier><identifier>DOI: 10.1149/2.0791609jes</identifier><language>eng</language><publisher>The Electrochemical Society</publisher><subject>Electrochemical testing ; Fuel Cells ; Impedance spectroscopy ; Manufacturing and materials engineering ; Metal supported cells ; Plasma spraying ; Production Technology ; Produktions- och materialteknik ; Produktionsteknik ; Solid Oxide</subject><ispartof>Journal of the Electrochemical Society, 2016-01, Vol.163 (9), p.F1059-F1065</ispartof><rights>The Author(s) 2016. Published by ECS.</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c412t-42ab3731414de204b6b9efe04cf4645d679ccc59235d4a7f1f316a3653e501ac3</citedby></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://iopscience.iop.org/article/10.1149/2.0791609jes/pdf$$EPDF$$P50$$Giop$$Hfree_for_read</linktopdf><link.rule.ids>230,314,550,776,780,881,4010,27900,27901,27902,53821</link.rule.ids><backlink>$$Uhttps://urn.kb.se/resolve?urn=urn:nbn:se:hv:diva-10045$$DView record from Swedish Publication Index$$Hfree_for_read</backlink></links><search><creatorcontrib>Gupta, M.</creatorcontrib><creatorcontrib>Weber, A.</creatorcontrib><creatorcontrib>Markocsan, N.</creatorcontrib><creatorcontrib>Gindrat, M.</creatorcontrib><title>Electrochemical Performance of Plasma Sprayed Metal Supported Planar Solid Oxide Fuel Cells</title><title>Journal of the Electrochemical Society</title><addtitle>J. Electrochem. Soc</addtitle><description>High production cost is one of the major barriers to widespread commercialization of solid oxide fuel cells (SOFCs). Thermal spray techniques are a low cost alternative for the production of SOFCs. The objective of this work was to evaluate the electrochemical performance of cells produced by plasma spraying. The anode was deposited on a porous metallic support by atmospheric plasma spraying (APS) whereas the electrolyte was deposited by plasma spray-thin film (PS-TF) technique, which can produce thin and dense coatings at high deposition rates. The cathode was deposited by screen-printing and in-operando sintering. The electrochemical tests were performed at 650-800°C. Current-voltage characteristics and impedance spectra were measured and analyzed. The impact of electrolyte composition and layer thickness on the gas tightness of the electrolyte and the area specific resistance of the cell is discussed. The results show that the applied thermal spraying techniques are a potential alternative for producing SOFCs.</description><subject>Electrochemical testing</subject><subject>Fuel Cells</subject><subject>Impedance spectroscopy</subject><subject>Manufacturing and materials engineering</subject><subject>Metal supported cells</subject><subject>Plasma spraying</subject><subject>Production Technology</subject><subject>Produktions- och materialteknik</subject><subject>Produktionsteknik</subject><subject>Solid Oxide</subject><issn>0013-4651</issn><issn>1945-7111</issn><issn>1945-7111</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2016</creationdate><recordtype>article</recordtype><sourceid>O3W</sourceid><sourceid>D8T</sourceid><recordid>eNpt0EFLwzAUB_AgCs7pzQ-Qo6CdeU3a2uOYmwqTDaZePIQ0fXEd6VKSVt23tzLRi6fHn_fjwfsTcg5sBCDy63jEshxSlm8wHJAB5CKJMgA4JAPGgEciTeCYnISw6SPciGxAXqcWdeudXmNdaWXpEr1xvlZbjdQZurQq1IquGq92WNJHbHuz6prG-bbP_XqrPF05W5V08VmVSGcdWjpBa8MpOTLKBjz7mUPyPJs-Te6j-eLuYTKeR1pA3EYiVgXPOAgQJcZMFGmRo0EmtBGpSMo0y7XWSR7zpBQqM2A4pIqnCceEgdJ8SC73d8MHNl0hG1_Vyu-kU5W8rV7G0vk3uX6XwJhIen2119q7EDyaXw9MftcoY_lXY88v9rxyjdy4zm_7V_6nX34mcsY</recordid><startdate>201601</startdate><enddate>201601</enddate><creator>Gupta, M.</creator><creator>Weber, A.</creator><creator>Markocsan, N.</creator><creator>Gindrat, M.</creator><general>The Electrochemical Society</general><scope>O3W</scope><scope>TSCCA</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>ADTPV</scope><scope>AICEO</scope><scope>AOWAS</scope><scope>D8T</scope><scope>DF5</scope><scope>ZZAVC</scope></search><sort><creationdate>201601</creationdate><title>Electrochemical Performance of Plasma Sprayed Metal Supported Planar Solid Oxide Fuel Cells</title><author>Gupta, M. ; Weber, A. ; Markocsan, N. ; Gindrat, M.</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c412t-42ab3731414de204b6b9efe04cf4645d679ccc59235d4a7f1f316a3653e501ac3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2016</creationdate><topic>Electrochemical testing</topic><topic>Fuel Cells</topic><topic>Impedance spectroscopy</topic><topic>Manufacturing and materials engineering</topic><topic>Metal supported cells</topic><topic>Plasma spraying</topic><topic>Production Technology</topic><topic>Produktions- och materialteknik</topic><topic>Produktionsteknik</topic><topic>Solid Oxide</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Gupta, M.</creatorcontrib><creatorcontrib>Weber, A.</creatorcontrib><creatorcontrib>Markocsan, N.</creatorcontrib><creatorcontrib>Gindrat, M.</creatorcontrib><collection>IOP Publishing Free Content</collection><collection>IOPscience (Open Access)</collection><collection>CrossRef</collection><collection>SwePub</collection><collection>SWEPUB Högskolan Väst full text</collection><collection>SwePub Articles</collection><collection>SWEPUB Freely available online</collection><collection>SWEPUB Högskolan Väst</collection><collection>SwePub Articles full text</collection><jtitle>Journal of the Electrochemical Society</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Gupta, M.</au><au>Weber, A.</au><au>Markocsan, N.</au><au>Gindrat, M.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Electrochemical Performance of Plasma Sprayed Metal Supported Planar Solid Oxide Fuel Cells</atitle><jtitle>Journal of the Electrochemical Society</jtitle><addtitle>J. Electrochem. Soc</addtitle><date>2016-01</date><risdate>2016</risdate><volume>163</volume><issue>9</issue><spage>F1059</spage><epage>F1065</epage><pages>F1059-F1065</pages><issn>0013-4651</issn><issn>1945-7111</issn><eissn>1945-7111</eissn><abstract>High production cost is one of the major barriers to widespread commercialization of solid oxide fuel cells (SOFCs). Thermal spray techniques are a low cost alternative for the production of SOFCs. The objective of this work was to evaluate the electrochemical performance of cells produced by plasma spraying. The anode was deposited on a porous metallic support by atmospheric plasma spraying (APS) whereas the electrolyte was deposited by plasma spray-thin film (PS-TF) technique, which can produce thin and dense coatings at high deposition rates. The cathode was deposited by screen-printing and in-operando sintering. The electrochemical tests were performed at 650-800°C. Current-voltage characteristics and impedance spectra were measured and analyzed. The impact of electrolyte composition and layer thickness on the gas tightness of the electrolyte and the area specific resistance of the cell is discussed. The results show that the applied thermal spraying techniques are a potential alternative for producing SOFCs.</abstract><pub>The Electrochemical Society</pub><doi>10.1149/2.0791609jes</doi><tpages>7</tpages><oa>free_for_read</oa></addata></record> |
fulltext | fulltext |
identifier | ISSN: 0013-4651 |
ispartof | Journal of the Electrochemical Society, 2016-01, Vol.163 (9), p.F1059-F1065 |
issn | 0013-4651 1945-7111 1945-7111 |
language | eng |
recordid | cdi_crossref_primary_10_1149_2_0791609jes |
source | IOP Publishing Journals; SWEPUB Freely available online |
subjects | Electrochemical testing Fuel Cells Impedance spectroscopy Manufacturing and materials engineering Metal supported cells Plasma spraying Production Technology Produktions- och materialteknik Produktionsteknik Solid Oxide |
title | Electrochemical Performance of Plasma Sprayed Metal Supported Planar Solid Oxide Fuel Cells |
url | https://sfx.bib-bvb.de/sfx_tum?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2025-01-31T16%3A40%3A10IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-swepub_cross&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=Electrochemical%20Performance%20of%20Plasma%20Sprayed%20Metal%20Supported%20Planar%20Solid%20Oxide%20Fuel%20Cells&rft.jtitle=Journal%20of%20the%20Electrochemical%20Society&rft.au=Gupta,%20M.&rft.date=2016-01&rft.volume=163&rft.issue=9&rft.spage=F1059&rft.epage=F1065&rft.pages=F1059-F1065&rft.issn=0013-4651&rft.eissn=1945-7111&rft_id=info:doi/10.1149/2.0791609jes&rft_dat=%3Cswepub_cross%3Eoai_DiVA_org_hv_10045%3C/swepub_cross%3E%3Curl%3E%3C/url%3E&disable_directlink=true&sfx.directlink=off&sfx.report_link=0&rft_id=info:oai/&rft_id=info:pmid/&rfr_iscdi=true |