WS 2 ribbon arrays with defined chirality and coherent polarity
One-dimensional transition metal dichalcogenides exhibiting an enhanced bulk photovoltaic effect have the potential to exceed the Shockley-Queisser limit efficiency in solar energy harvest within - junction architectures. However, the collective output of these prototype devices remains a challenge....
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| Veröffentlicht in: | Science (American Association for the Advancement of Science) 2024-06, Vol.384 (6700), p.1100-1104 |
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| creator | Xue, Guodong Zhou, Ziqi Guo, Quanlin Zuo, Yonggang Wei, Wenya Yang, Jiashu Yin, Peng Zhang, Shuai Zhong, Ding You, Yilong Sui, Xin Liu, Chang Wu, Muhong Hong, Hao Wang, Zhu-Jun Gao, Peng Li, Qunyang Zhang, Libo Yu, Dapeng Ding, Feng Wei, Zhongming Liu, Can Liu, Kaihui |
| description | One-dimensional transition metal dichalcogenides exhibiting an enhanced bulk photovoltaic effect have the potential to exceed the Shockley-Queisser limit efficiency in solar energy harvest within
-
junction architectures. However, the collective output of these prototype devices remains a challenge. We report on the synthesis of single-crystalline WS
ribbon arrays with defined chirality and coherent polarity through an atomic manufacturing strategy. The chirality of WS
ribbon was defined by substrate couplings into tunable armchair, zigzag, and chiral species, and the polarity direction was determined by the ribbon-precursor interfacial energy along a coherent direction. A single armchair ribbon showed strong bulk photovoltaic effect and the further integration of ~1000 aligned ribbons with coherent polarity enabled upscaling of the photocurrent. |
| doi_str_mv | 10.1126/science.adn9476 |
| format | Article |
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-
junction architectures. However, the collective output of these prototype devices remains a challenge. We report on the synthesis of single-crystalline WS
ribbon arrays with defined chirality and coherent polarity through an atomic manufacturing strategy. The chirality of WS
ribbon was defined by substrate couplings into tunable armchair, zigzag, and chiral species, and the polarity direction was determined by the ribbon-precursor interfacial energy along a coherent direction. A single armchair ribbon showed strong bulk photovoltaic effect and the further integration of ~1000 aligned ribbons with coherent polarity enabled upscaling of the photocurrent.</description><identifier>ISSN: 0036-8075</identifier><identifier>EISSN: 1095-9203</identifier><identifier>DOI: 10.1126/science.adn9476</identifier><identifier>PMID: 38843317</identifier><language>eng</language><publisher>United States</publisher><ispartof>Science (American Association for the Advancement of Science), 2024-06, Vol.384 (6700), p.1100-1104</ispartof><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><cites>FETCH-LOGICAL-c637-b47c38d7258f892af913ef99f233776749b9ef15f11ed59d263da210134b034e3</cites><orcidid>0000-0003-1262-6767 ; 0000-0002-0641-1340 ; 0000-0002-6237-0993 ; 0000-0003-2930-6970 ; 0000-0003-3607-8945 ; 0000-0001-9153-9279 ; 0000-0002-8781-2495 ; 0009-0001-8063-6345 ; 0000-0002-8227-7323 ; 0009-0000-1791-7139 ; 0000-0002-6273-6465 ; 0000-0002-6865-3863 ; 0000-0002-2946-5069 ; 0000-0003-0721-9294 ; 0009-0008-2917-0843 ; 0000-0001-5451-4144 ; 0009-0002-2195-2310 ; 0009-0006-4366-2401 ; 0000-0003-0860-5525 ; 0009-0006-9097-7529 ; 0000-0003-3244-0142</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,776,780,2871,2872,27901,27902</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/38843317$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Xue, Guodong</creatorcontrib><creatorcontrib>Zhou, Ziqi</creatorcontrib><creatorcontrib>Guo, Quanlin</creatorcontrib><creatorcontrib>Zuo, Yonggang</creatorcontrib><creatorcontrib>Wei, Wenya</creatorcontrib><creatorcontrib>Yang, Jiashu</creatorcontrib><creatorcontrib>Yin, Peng</creatorcontrib><creatorcontrib>Zhang, Shuai</creatorcontrib><creatorcontrib>Zhong, Ding</creatorcontrib><creatorcontrib>You, Yilong</creatorcontrib><creatorcontrib>Sui, Xin</creatorcontrib><creatorcontrib>Liu, Chang</creatorcontrib><creatorcontrib>Wu, Muhong</creatorcontrib><creatorcontrib>Hong, Hao</creatorcontrib><creatorcontrib>Wang, Zhu-Jun</creatorcontrib><creatorcontrib>Gao, Peng</creatorcontrib><creatorcontrib>Li, Qunyang</creatorcontrib><creatorcontrib>Zhang, Libo</creatorcontrib><creatorcontrib>Yu, Dapeng</creatorcontrib><creatorcontrib>Ding, Feng</creatorcontrib><creatorcontrib>Wei, Zhongming</creatorcontrib><creatorcontrib>Liu, Can</creatorcontrib><creatorcontrib>Liu, Kaihui</creatorcontrib><title>WS 2 ribbon arrays with defined chirality and coherent polarity</title><title>Science (American Association for the Advancement of Science)</title><addtitle>Science</addtitle><description>One-dimensional transition metal dichalcogenides exhibiting an enhanced bulk photovoltaic effect have the potential to exceed the Shockley-Queisser limit efficiency in solar energy harvest within
-
junction architectures. However, the collective output of these prototype devices remains a challenge. We report on the synthesis of single-crystalline WS
ribbon arrays with defined chirality and coherent polarity through an atomic manufacturing strategy. The chirality of WS
ribbon was defined by substrate couplings into tunable armchair, zigzag, and chiral species, and the polarity direction was determined by the ribbon-precursor interfacial energy along a coherent direction. A single armchair ribbon showed strong bulk photovoltaic effect and the further integration of ~1000 aligned ribbons with coherent polarity enabled upscaling of the photocurrent.</description><issn>0036-8075</issn><issn>1095-9203</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2024</creationdate><recordtype>article</recordtype><recordid>eNo9kE9LxDAQxYMobl09e5N8ge4mmbZJTiKL_2DBgwseS9pMaKTblqQi_fZWtnoa3rz3BuZHyC1nG85FsY21x67GjbGdzmRxRhLOdJ5qweCcJIxBkSom8xW5ivGTsdnTcElWoFQGwGVC7j_eqaDBV1XfUROCmSL99mNDLTrfoaV144Np_ThR082qbzBgN9Khb02Yt9fkwpk24s0y1-Tw9HjYvaT7t-fX3cM-rQuQaZXJGpSVIldOaWGc5oBOaycApCxkpiuNjueOc7S5tqIAawRnHLKKQYawJtvT2Tr0MQZ05RD80YSp5Kz8JVEuJMqFxNy4OzWGr-qI9j__9zr8AFSoW1A</recordid><startdate>20240607</startdate><enddate>20240607</enddate><creator>Xue, Guodong</creator><creator>Zhou, Ziqi</creator><creator>Guo, Quanlin</creator><creator>Zuo, Yonggang</creator><creator>Wei, Wenya</creator><creator>Yang, Jiashu</creator><creator>Yin, Peng</creator><creator>Zhang, Shuai</creator><creator>Zhong, Ding</creator><creator>You, Yilong</creator><creator>Sui, Xin</creator><creator>Liu, Chang</creator><creator>Wu, Muhong</creator><creator>Hong, Hao</creator><creator>Wang, Zhu-Jun</creator><creator>Gao, Peng</creator><creator>Li, Qunyang</creator><creator>Zhang, Libo</creator><creator>Yu, Dapeng</creator><creator>Ding, Feng</creator><creator>Wei, Zhongming</creator><creator>Liu, Can</creator><creator>Liu, Kaihui</creator><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><orcidid>https://orcid.org/0000-0003-1262-6767</orcidid><orcidid>https://orcid.org/0000-0002-0641-1340</orcidid><orcidid>https://orcid.org/0000-0002-6237-0993</orcidid><orcidid>https://orcid.org/0000-0003-2930-6970</orcidid><orcidid>https://orcid.org/0000-0003-3607-8945</orcidid><orcidid>https://orcid.org/0000-0001-9153-9279</orcidid><orcidid>https://orcid.org/0000-0002-8781-2495</orcidid><orcidid>https://orcid.org/0009-0001-8063-6345</orcidid><orcidid>https://orcid.org/0000-0002-8227-7323</orcidid><orcidid>https://orcid.org/0009-0000-1791-7139</orcidid><orcidid>https://orcid.org/0000-0002-6273-6465</orcidid><orcidid>https://orcid.org/0000-0002-6865-3863</orcidid><orcidid>https://orcid.org/0000-0002-2946-5069</orcidid><orcidid>https://orcid.org/0000-0003-0721-9294</orcidid><orcidid>https://orcid.org/0009-0008-2917-0843</orcidid><orcidid>https://orcid.org/0000-0001-5451-4144</orcidid><orcidid>https://orcid.org/0009-0002-2195-2310</orcidid><orcidid>https://orcid.org/0009-0006-4366-2401</orcidid><orcidid>https://orcid.org/0000-0003-0860-5525</orcidid><orcidid>https://orcid.org/0009-0006-9097-7529</orcidid><orcidid>https://orcid.org/0000-0003-3244-0142</orcidid></search><sort><creationdate>20240607</creationdate><title>WS 2 ribbon arrays with defined chirality and coherent polarity</title><author>Xue, Guodong ; 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-
junction architectures. However, the collective output of these prototype devices remains a challenge. We report on the synthesis of single-crystalline WS
ribbon arrays with defined chirality and coherent polarity through an atomic manufacturing strategy. The chirality of WS
ribbon was defined by substrate couplings into tunable armchair, zigzag, and chiral species, and the polarity direction was determined by the ribbon-precursor interfacial energy along a coherent direction. A single armchair ribbon showed strong bulk photovoltaic effect and the further integration of ~1000 aligned ribbons with coherent polarity enabled upscaling of the photocurrent.</abstract><cop>United States</cop><pmid>38843317</pmid><doi>10.1126/science.adn9476</doi><tpages>5</tpages><orcidid>https://orcid.org/0000-0003-1262-6767</orcidid><orcidid>https://orcid.org/0000-0002-0641-1340</orcidid><orcidid>https://orcid.org/0000-0002-6237-0993</orcidid><orcidid>https://orcid.org/0000-0003-2930-6970</orcidid><orcidid>https://orcid.org/0000-0003-3607-8945</orcidid><orcidid>https://orcid.org/0000-0001-9153-9279</orcidid><orcidid>https://orcid.org/0000-0002-8781-2495</orcidid><orcidid>https://orcid.org/0009-0001-8063-6345</orcidid><orcidid>https://orcid.org/0000-0002-8227-7323</orcidid><orcidid>https://orcid.org/0009-0000-1791-7139</orcidid><orcidid>https://orcid.org/0000-0002-6273-6465</orcidid><orcidid>https://orcid.org/0000-0002-6865-3863</orcidid><orcidid>https://orcid.org/0000-0002-2946-5069</orcidid><orcidid>https://orcid.org/0000-0003-0721-9294</orcidid><orcidid>https://orcid.org/0009-0008-2917-0843</orcidid><orcidid>https://orcid.org/0000-0001-5451-4144</orcidid><orcidid>https://orcid.org/0009-0002-2195-2310</orcidid><orcidid>https://orcid.org/0009-0006-4366-2401</orcidid><orcidid>https://orcid.org/0000-0003-0860-5525</orcidid><orcidid>https://orcid.org/0009-0006-9097-7529</orcidid><orcidid>https://orcid.org/0000-0003-3244-0142</orcidid></addata></record> |
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| ispartof | Science (American Association for the Advancement of Science), 2024-06, Vol.384 (6700), p.1100-1104 |
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| source | American Association for the Advancement of Science |
| title | WS 2 ribbon arrays with defined chirality and coherent polarity |
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