Decay Times of Fluorescent Substances Excited by High-Energy Radiation

Decay times of fluorescent light emitted by organic solutions and by onganic and inorganic solids when excited by high-energy radiation are determined under various experimental conditions. The pulse-height ratios for alpha particle and electron excitations are also found. The probabilities for radi...

Ausführliche Beschreibung

Gespeichert in:
Bibliographische Detailangaben
Veröffentlicht in:Physical Review (U.S.) Superseded in part by Phys. Rev. A, Phys. Rev. B: Solid State, Phys. Rev. C, and Phys. Rev. D Phys. Rev. B: Solid State, Phys. Rev. C, and Phys. Rev. D, 1957-12, Vol.108 (5), p.1122-1130
Hauptverfasser: Kallmann, Hartmut, Brucker, George J.
Format: Artikel
Sprache:eng
Schlagworte:
Online-Zugang:Volltext
Tags: Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
container_end_page 1130
container_issue 5
container_start_page 1122
container_title Physical Review (U.S.) Superseded in part by Phys. Rev. A, Phys. Rev. B: Solid State, Phys. Rev. C, and Phys. Rev. D
container_volume 108
creator Kallmann, Hartmut
Brucker, George J.
description Decay times of fluorescent light emitted by organic solutions and by onganic and inorganic solids when excited by high-energy radiation are determined under various experimental conditions. The pulse-height ratios for alpha particle and electron excitations are also found. The probabilities for radiative and nonradiative transitions of the light emitting molecule are estimated and compared with values obtained from absorption measurements. The time required for energy transfer is estimated. The ratio of pulse heights obtained under alpha -particle excitation to those obtained under electron excitation are found to be roughly the same for all organic solutions and solids despite wide variations in lifetime; also no difference in lifetime between alpha -particle and electron excitations is found. This is not explained by present theories. A new theory to explain these facts is outlined. (auth)
doi_str_mv 10.1103/PhysRev.108.1122
format Article
fullrecord <record><control><sourceid>crossref_osti_</sourceid><recordid>TN_cdi_crossref_primary_10_1103_PhysRev_108_1122</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>10_1103_PhysRev_108_1122</sourcerecordid><originalsourceid>FETCH-LOGICAL-c334t-b66fd76f1199d229a9cce14c2df18556f2ae29125d3efe2a9ff46bcd5a390aeb3</originalsourceid><addsrcrecordid>eNotkMFLwzAUh3NQcE7vHoP3zrwkrc1RZueEgTIneAtp8rJGtlaaTOx_b8d2-vF-7-Px-Ai5AzYDYOLhvRniGn9nwMqx4PyCTBgTkJVKfV2R6xi_GQOppJyQxTNaM9BN2GOknaeL3aHrMVpsE_041DGZ1o6b6s-GhI7WA12GbZNVLfbbga6NCyaFrr0hl97sIt6ec0o-F9VmvsxWby-v86dVZoWQKauLwrvHwgMo5ThXRlmLIC13Hso8Lzw3yBXw3An0yI3yXha1dbkRihmsxZTcn-52MQUdj0_ZxnZtizZpKUCWrBghdoJs38XYo9c_fdibftDA9FGQPgsa51IfBYl_50xdRw</addsrcrecordid><sourcetype>Open Access Repository</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype></control><display><type>article</type><title>Decay Times of Fluorescent Substances Excited by High-Energy Radiation</title><source>American Physical Society Journals</source><creator>Kallmann, Hartmut ; Brucker, George J.</creator><creatorcontrib>Kallmann, Hartmut ; Brucker, George J. ; New York Univ ; Evans Signal Lab., For Monmouth, N.J</creatorcontrib><description>Decay times of fluorescent light emitted by organic solutions and by onganic and inorganic solids when excited by high-energy radiation are determined under various experimental conditions. The pulse-height ratios for alpha particle and electron excitations are also found. The probabilities for radiative and nonradiative transitions of the light emitting molecule are estimated and compared with values obtained from absorption measurements. The time required for energy transfer is estimated. The ratio of pulse heights obtained under alpha -particle excitation to those obtained under electron excitation are found to be roughly the same for all organic solutions and solids despite wide variations in lifetime; also no difference in lifetime between alpha -particle and electron excitations is found. This is not explained by present theories. A new theory to explain these facts is outlined. (auth)</description><identifier>ISSN: 0031-899X</identifier><identifier>DOI: 10.1103/PhysRev.108.1122</identifier><language>eng</language><subject>ABSORPTION ; ALPHA PARTICLES ; DECAY ; ELECTRONS ; ENERGY ; ENERGY RANGE ; EQUATIONS ; EXCITATION ; FLUORESCENCE ; HALF-LIFE ; LIGHT ; MEASURED VALUES ; MOLECULES ; ORGANIC COMPOUNDS ; OSCILLATIONS ; PHYSICS ; RADIATIONS ; SOLIDS ; SOLUTIONS</subject><ispartof>Physical Review (U.S.) Superseded in part by Phys. Rev. A, Phys. Rev. B: Solid State, Phys. Rev. C, and Phys. Rev. D, 1957-12, Vol.108 (5), p.1122-1130</ispartof><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c334t-b66fd76f1199d229a9cce14c2df18556f2ae29125d3efe2a9ff46bcd5a390aeb3</citedby><cites>FETCH-LOGICAL-c334t-b66fd76f1199d229a9cce14c2df18556f2ae29125d3efe2a9ff46bcd5a390aeb3</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,780,784,885,2876,2877,27924,27925</link.rule.ids><backlink>$$Uhttps://www.osti.gov/biblio/4314806$$D View this record in Osti.gov$$Hfree_for_read</backlink></links><search><creatorcontrib>Kallmann, Hartmut</creatorcontrib><creatorcontrib>Brucker, George J.</creatorcontrib><creatorcontrib>New York Univ</creatorcontrib><creatorcontrib>Evans Signal Lab., For Monmouth, N.J</creatorcontrib><title>Decay Times of Fluorescent Substances Excited by High-Energy Radiation</title><title>Physical Review (U.S.) Superseded in part by Phys. Rev. A, Phys. Rev. B: Solid State, Phys. Rev. C, and Phys. Rev. D</title><description>Decay times of fluorescent light emitted by organic solutions and by onganic and inorganic solids when excited by high-energy radiation are determined under various experimental conditions. The pulse-height ratios for alpha particle and electron excitations are also found. The probabilities for radiative and nonradiative transitions of the light emitting molecule are estimated and compared with values obtained from absorption measurements. The time required for energy transfer is estimated. The ratio of pulse heights obtained under alpha -particle excitation to those obtained under electron excitation are found to be roughly the same for all organic solutions and solids despite wide variations in lifetime; also no difference in lifetime between alpha -particle and electron excitations is found. This is not explained by present theories. A new theory to explain these facts is outlined. (auth)</description><subject>ABSORPTION</subject><subject>ALPHA PARTICLES</subject><subject>DECAY</subject><subject>ELECTRONS</subject><subject>ENERGY</subject><subject>ENERGY RANGE</subject><subject>EQUATIONS</subject><subject>EXCITATION</subject><subject>FLUORESCENCE</subject><subject>HALF-LIFE</subject><subject>LIGHT</subject><subject>MEASURED VALUES</subject><subject>MOLECULES</subject><subject>ORGANIC COMPOUNDS</subject><subject>OSCILLATIONS</subject><subject>PHYSICS</subject><subject>RADIATIONS</subject><subject>SOLIDS</subject><subject>SOLUTIONS</subject><issn>0031-899X</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>1957</creationdate><recordtype>article</recordtype><recordid>eNotkMFLwzAUh3NQcE7vHoP3zrwkrc1RZueEgTIneAtp8rJGtlaaTOx_b8d2-vF-7-Px-Ai5AzYDYOLhvRniGn9nwMqx4PyCTBgTkJVKfV2R6xi_GQOppJyQxTNaM9BN2GOknaeL3aHrMVpsE_041DGZ1o6b6s-GhI7WA12GbZNVLfbbga6NCyaFrr0hl97sIt6ec0o-F9VmvsxWby-v86dVZoWQKauLwrvHwgMo5ThXRlmLIC13Hso8Lzw3yBXw3An0yI3yXha1dbkRihmsxZTcn-52MQUdj0_ZxnZtizZpKUCWrBghdoJs38XYo9c_fdibftDA9FGQPgsa51IfBYl_50xdRw</recordid><startdate>19571201</startdate><enddate>19571201</enddate><creator>Kallmann, Hartmut</creator><creator>Brucker, George J.</creator><scope>AAYXX</scope><scope>CITATION</scope><scope>OTOTI</scope></search><sort><creationdate>19571201</creationdate><title>Decay Times of Fluorescent Substances Excited by High-Energy Radiation</title><author>Kallmann, Hartmut ; Brucker, George J.</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c334t-b66fd76f1199d229a9cce14c2df18556f2ae29125d3efe2a9ff46bcd5a390aeb3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>1957</creationdate><topic>ABSORPTION</topic><topic>ALPHA PARTICLES</topic><topic>DECAY</topic><topic>ELECTRONS</topic><topic>ENERGY</topic><topic>ENERGY RANGE</topic><topic>EQUATIONS</topic><topic>EXCITATION</topic><topic>FLUORESCENCE</topic><topic>HALF-LIFE</topic><topic>LIGHT</topic><topic>MEASURED VALUES</topic><topic>MOLECULES</topic><topic>ORGANIC COMPOUNDS</topic><topic>OSCILLATIONS</topic><topic>PHYSICS</topic><topic>RADIATIONS</topic><topic>SOLIDS</topic><topic>SOLUTIONS</topic><toplevel>online_resources</toplevel><creatorcontrib>Kallmann, Hartmut</creatorcontrib><creatorcontrib>Brucker, George J.</creatorcontrib><creatorcontrib>New York Univ</creatorcontrib><creatorcontrib>Evans Signal Lab., For Monmouth, N.J</creatorcontrib><collection>CrossRef</collection><collection>OSTI.GOV</collection><jtitle>Physical Review (U.S.) Superseded in part by Phys. Rev. A, Phys. Rev. B: Solid State, Phys. Rev. C, and Phys. Rev. D</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Kallmann, Hartmut</au><au>Brucker, George J.</au><aucorp>New York Univ</aucorp><aucorp>Evans Signal Lab., For Monmouth, N.J</aucorp><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Decay Times of Fluorescent Substances Excited by High-Energy Radiation</atitle><jtitle>Physical Review (U.S.) Superseded in part by Phys. Rev. A, Phys. Rev. B: Solid State, Phys. Rev. C, and Phys. Rev. D</jtitle><date>1957-12-01</date><risdate>1957</risdate><volume>108</volume><issue>5</issue><spage>1122</spage><epage>1130</epage><pages>1122-1130</pages><issn>0031-899X</issn><abstract>Decay times of fluorescent light emitted by organic solutions and by onganic and inorganic solids when excited by high-energy radiation are determined under various experimental conditions. The pulse-height ratios for alpha particle and electron excitations are also found. The probabilities for radiative and nonradiative transitions of the light emitting molecule are estimated and compared with values obtained from absorption measurements. The time required for energy transfer is estimated. The ratio of pulse heights obtained under alpha -particle excitation to those obtained under electron excitation are found to be roughly the same for all organic solutions and solids despite wide variations in lifetime; also no difference in lifetime between alpha -particle and electron excitations is found. This is not explained by present theories. A new theory to explain these facts is outlined. (auth)</abstract><doi>10.1103/PhysRev.108.1122</doi><tpages>9</tpages></addata></record>
fulltext fulltext
identifier ISSN: 0031-899X
ispartof Physical Review (U.S.) Superseded in part by Phys. Rev. A, Phys. Rev. B: Solid State, Phys. Rev. C, and Phys. Rev. D, 1957-12, Vol.108 (5), p.1122-1130
issn 0031-899X
language eng
recordid cdi_crossref_primary_10_1103_PhysRev_108_1122
source American Physical Society Journals
subjects ABSORPTION
ALPHA PARTICLES
DECAY
ELECTRONS
ENERGY
ENERGY RANGE
EQUATIONS
EXCITATION
FLUORESCENCE
HALF-LIFE
LIGHT
MEASURED VALUES
MOLECULES
ORGANIC COMPOUNDS
OSCILLATIONS
PHYSICS
RADIATIONS
SOLIDS
SOLUTIONS
title Decay Times of Fluorescent Substances Excited by High-Energy Radiation
url https://sfx.bib-bvb.de/sfx_tum?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2024-12-21T14%3A24%3A28IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-crossref_osti_&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=Decay%20Times%20of%20Fluorescent%20Substances%20Excited%20by%20High-Energy%20Radiation&rft.jtitle=Physical%20Review%20(U.S.)%20Superseded%20in%20part%20by%20Phys.%20Rev.%20A,%20Phys.%20Rev.%20B:%20Solid%20State,%20Phys.%20Rev.%20C,%20and%20Phys.%20Rev.%20D&rft.au=Kallmann,%20Hartmut&rft.aucorp=New%20York%20Univ&rft.date=1957-12-01&rft.volume=108&rft.issue=5&rft.spage=1122&rft.epage=1130&rft.pages=1122-1130&rft.issn=0031-899X&rft_id=info:doi/10.1103/PhysRev.108.1122&rft_dat=%3Ccrossref_osti_%3E10_1103_PhysRev_108_1122%3C/crossref_osti_%3E%3Curl%3E%3C/url%3E&disable_directlink=true&sfx.directlink=off&sfx.report_link=0&rft_id=info:oai/&rft_id=info:pmid/&rfr_iscdi=true