Fluorinated graphene nanoparticles with 1-3 nm electrically active graphene quantum dots
A new approach to creating a new and locally nanostructured graphene-based material is reported. We studied the electric and structural properties of partially fluorinated graphene (FG) films obtained from an FG-suspension and nanostructured by high-energy Xe ions. Local shock heating in ion tracks...
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| Veröffentlicht in: | Nanotechnology 2020-05, Vol.31 (29), p.295602-295602, Article 295602 |
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| container_title | Nanotechnology |
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| creator | Nebogatikova, Nadezhda A Antonova, Irina V Ivanov, Artem I Demin, Victor A Kvashnin, Dmitry G Olejniczak, Andrzej Gutakovskii, Anton K Kornieieva, Kateryna A Renault, Paul L J Skuratov, Vladimir A Chernozatonskii, Leonid A |
| description | A new approach to creating a new and locally nanostructured graphene-based material is reported. We studied the electric and structural properties of partially fluorinated graphene (FG) films obtained from an FG-suspension and nanostructured by high-energy Xe ions. Local shock heating in ion tracks is suggested to be the main force driving the changes. It was found that ion irradiation leads to the formation of locally thermally expanded FG and its cracking into nanoparticles with small (∼1.5-3 nm) graphene quantum dots (GQD), embedded in them. The bandgap of GQD was estimated as 1 -1.5 eV. A further developed approach was applied to correct the functional properties of printed FG-based crossbar memristors. Dielectric FG films with small quantum dots may offer prospects in graphene-based electronics due to their stability and promising properties. |
| doi_str_mv | 10.1088/1361-6528/ab83b8 |
| format | Article |
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We studied the electric and structural properties of partially fluorinated graphene (FG) films obtained from an FG-suspension and nanostructured by high-energy Xe ions. Local shock heating in ion tracks is suggested to be the main force driving the changes. It was found that ion irradiation leads to the formation of locally thermally expanded FG and its cracking into nanoparticles with small (∼1.5-3 nm) graphene quantum dots (GQD), embedded in them. The bandgap of GQD was estimated as 1 -1.5 eV. A further developed approach was applied to correct the functional properties of printed FG-based crossbar memristors. 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We studied the electric and structural properties of partially fluorinated graphene (FG) films obtained from an FG-suspension and nanostructured by high-energy Xe ions. Local shock heating in ion tracks is suggested to be the main force driving the changes. It was found that ion irradiation leads to the formation of locally thermally expanded FG and its cracking into nanoparticles with small (∼1.5-3 nm) graphene quantum dots (GQD), embedded in them. The bandgap of GQD was estimated as 1 -1.5 eV. A further developed approach was applied to correct the functional properties of printed FG-based crossbar memristors. Dielectric FG films with small quantum dots may offer prospects in graphene-based electronics due to their stability and promising properties.</description><subject>fluorinated graphene</subject><subject>graphene quantum dots</subject><subject>Materials Science</subject><subject>Materials Science, Multidisciplinary</subject><subject>memristor</subject><subject>molecular dynamics simulation</subject><subject>Nanoscience & Nanotechnology</subject><subject>nanostructuring</subject><subject>Physical Sciences</subject><subject>Physics</subject><subject>Physics, Applied</subject><subject>Science & Technology</subject><subject>Science & Technology - Other Topics</subject><subject>swift ion irradiation</subject><subject>Technology</subject><issn>0957-4484</issn><issn>1361-6528</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2020</creationdate><recordtype>article</recordtype><sourceid>AOWDO</sourceid><recordid>eNqNkd1L3jAUh8NwzFe3e6-kl8pWzUebppfyMt1A2I2D3YU0OdVIm9QkVfzvTal7dyMyCCQcnt_hnCcIHRF8RrAQ54RxUvKainPVCdaJD2izK-2hDW7rpqwqUe2jgxjvMSZEUPIJ7TNKM9e0G_Tncph9sE4lMMVtUNMdOCiccn5SIVk9QCyebLorSMkKNxYwgE7BajUMz4XSyT7Cv9jDrFyax8L4FD-jj70aInx5vQ_R78vvN9sf5fWvq5_bi-tSswansieccIDONKTWVDVKQYOZppRhXkOTd6J9W3GjsDGactBcCVNVTc27qiW9YYfoZO07Bf8wQ0xytFHDMCgHfo6SMlHRvDcnGcUrqoOPMUAvp2BHFZ4lwXLxKRd5cpEnV585cvzafe5GMLvAX4EZ-LoCT9D5PmoLTsMOwxjXjLGW0fzCywTi_-mtTSpZ77Z-dilHv61R6yd57-fgstX3Bj99A1_-VTIiaZtPzTGVk-nZC_KHreU</recordid><startdate>20200501</startdate><enddate>20200501</enddate><creator>Nebogatikova, Nadezhda A</creator><creator>Antonova, Irina V</creator><creator>Ivanov, Artem I</creator><creator>Demin, Victor A</creator><creator>Kvashnin, Dmitry G</creator><creator>Olejniczak, Andrzej</creator><creator>Gutakovskii, Anton K</creator><creator>Kornieieva, Kateryna A</creator><creator>Renault, Paul L J</creator><creator>Skuratov, Vladimir A</creator><creator>Chernozatonskii, Leonid A</creator><general>IOP Publishing</general><general>Iop Publishing Ltd</general><scope>AOWDO</scope><scope>BLEPL</scope><scope>DTL</scope><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7X8</scope><orcidid>https://orcid.org/0000-0003-3320-6657</orcidid><orcidid>https://orcid.org/0000-0002-6835-2737</orcidid><orcidid>https://orcid.org/0000-0001-8977-3832</orcidid><orcidid>https://orcid.org/0000-0003-3894-9396</orcidid><orcidid>https://orcid.org/0000-0002-5917-9709</orcidid><orcidid>https://orcid.org/0000-0002-4712-8736</orcidid></search><sort><creationdate>20200501</creationdate><title>Fluorinated graphene nanoparticles with 1-3 nm electrically active graphene quantum dots</title><author>Nebogatikova, Nadezhda A ; Antonova, Irina V ; Ivanov, Artem I ; Demin, Victor A ; Kvashnin, Dmitry G ; Olejniczak, Andrzej ; Gutakovskii, Anton K ; Kornieieva, Kateryna A ; Renault, Paul L J ; Skuratov, Vladimir A ; Chernozatonskii, Leonid A</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c370t-f1616eebd715c2a7aae703c223065e73b82f946da0ddc26ec6a8d44756b491fd3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2020</creationdate><topic>fluorinated graphene</topic><topic>graphene quantum dots</topic><topic>Materials Science</topic><topic>Materials Science, Multidisciplinary</topic><topic>memristor</topic><topic>molecular dynamics simulation</topic><topic>Nanoscience & Nanotechnology</topic><topic>nanostructuring</topic><topic>Physical Sciences</topic><topic>Physics</topic><topic>Physics, Applied</topic><topic>Science & Technology</topic><topic>Science & Technology - Other Topics</topic><topic>swift ion irradiation</topic><topic>Technology</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Nebogatikova, Nadezhda A</creatorcontrib><creatorcontrib>Antonova, Irina V</creatorcontrib><creatorcontrib>Ivanov, Artem I</creatorcontrib><creatorcontrib>Demin, Victor A</creatorcontrib><creatorcontrib>Kvashnin, Dmitry G</creatorcontrib><creatorcontrib>Olejniczak, Andrzej</creatorcontrib><creatorcontrib>Gutakovskii, Anton K</creatorcontrib><creatorcontrib>Kornieieva, Kateryna A</creatorcontrib><creatorcontrib>Renault, Paul L J</creatorcontrib><creatorcontrib>Skuratov, Vladimir A</creatorcontrib><creatorcontrib>Chernozatonskii, Leonid A</creatorcontrib><collection>Web of Science - Science Citation Index Expanded - 2020</collection><collection>Web of Science Core Collection</collection><collection>Science Citation Index Expanded</collection><collection>PubMed</collection><collection>CrossRef</collection><collection>MEDLINE - Academic</collection><jtitle>Nanotechnology</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Nebogatikova, Nadezhda A</au><au>Antonova, Irina V</au><au>Ivanov, Artem I</au><au>Demin, Victor A</au><au>Kvashnin, Dmitry G</au><au>Olejniczak, Andrzej</au><au>Gutakovskii, Anton K</au><au>Kornieieva, Kateryna A</au><au>Renault, Paul L J</au><au>Skuratov, Vladimir A</au><au>Chernozatonskii, Leonid A</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Fluorinated graphene nanoparticles with 1-3 nm electrically active graphene quantum dots</atitle><jtitle>Nanotechnology</jtitle><stitle>Nano</stitle><stitle>NANOTECHNOLOGY</stitle><addtitle>Nanotechnology</addtitle><date>2020-05-01</date><risdate>2020</risdate><volume>31</volume><issue>29</issue><spage>295602</spage><epage>295602</epage><pages>295602-295602</pages><artnum>295602</artnum><issn>0957-4484</issn><eissn>1361-6528</eissn><coden>NNOTER</coden><abstract>A new approach to creating a new and locally nanostructured graphene-based material is reported. We studied the electric and structural properties of partially fluorinated graphene (FG) films obtained from an FG-suspension and nanostructured by high-energy Xe ions. Local shock heating in ion tracks is suggested to be the main force driving the changes. It was found that ion irradiation leads to the formation of locally thermally expanded FG and its cracking into nanoparticles with small (∼1.5-3 nm) graphene quantum dots (GQD), embedded in them. The bandgap of GQD was estimated as 1 -1.5 eV. A further developed approach was applied to correct the functional properties of printed FG-based crossbar memristors. Dielectric FG films with small quantum dots may offer prospects in graphene-based electronics due to their stability and promising properties.</abstract><cop>BRISTOL</cop><pub>IOP Publishing</pub><pmid>32213679</pmid><doi>10.1088/1361-6528/ab83b8</doi><tpages>12</tpages><orcidid>https://orcid.org/0000-0003-3320-6657</orcidid><orcidid>https://orcid.org/0000-0002-6835-2737</orcidid><orcidid>https://orcid.org/0000-0001-8977-3832</orcidid><orcidid>https://orcid.org/0000-0003-3894-9396</orcidid><orcidid>https://orcid.org/0000-0002-5917-9709</orcidid><orcidid>https://orcid.org/0000-0002-4712-8736</orcidid></addata></record> |
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| subjects | fluorinated graphene graphene quantum dots Materials Science Materials Science, Multidisciplinary memristor molecular dynamics simulation Nanoscience & Nanotechnology nanostructuring Physical Sciences Physics Physics, Applied Science & Technology Science & Technology - Other Topics swift ion irradiation Technology |
| title | Fluorinated graphene nanoparticles with 1-3 nm electrically active graphene quantum dots |
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