Improving the performance of ultra-flexible perovskite photodetectors through cation engineering

High performance ultra-flexible lightweight perovskite photodetectors have promising applications on a variety of substrates, including those used on unmanned aerial vehicles. Herein, we report on a facile method to improve the performance of perovskite photodetectors on flexible ultrathin (50 μm) p...

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Veröffentlicht in:Journal of physics. D, Applied physics Applied physics, 2020-06, Vol.53 (23), p.235107
Hauptverfasser: Zhang, Mingdi, Lu, Qieni, Wang, Changlei, Dai, Haitao, Xue, Yongxiang, He, Jiantao, Ge, Baozhen
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container_issue 23
container_start_page 235107
container_title Journal of physics. D, Applied physics
container_volume 53
creator Zhang, Mingdi
Lu, Qieni
Wang, Changlei
Dai, Haitao
Xue, Yongxiang
He, Jiantao
Ge, Baozhen
description High performance ultra-flexible lightweight perovskite photodetectors have promising applications on a variety of substrates, including those used on unmanned aerial vehicles. Herein, we report on a facile method to improve the performance of perovskite photodetectors on flexible ultrathin (50 μm) polyimide substrates by tuning the composition with different ratios of cations. In the presence of lead thiocyanate, the introduction of a certain amount of formamidinium could sufficiently enhance the quality of methylammonium lead triiodide perovskite film, with prolonged carrier lifetime. A perovskite photodetector with a response time of ton = 89 ms and toff = 47 ms is achieved with a very simple device architecture. In addition, our flexible photodetectors maintain good performance after rigorous folding and bending, demonstrating excellent mechanical properties, which could be very useful for a variety of applications.
doi_str_mv 10.1088/1361-6463/ab7a59
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subjects compositional engineering
mechanical stability
perovskite photodetectors
ultra-flexible detectors
title Improving the performance of ultra-flexible perovskite photodetectors through cation engineering
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