Modelling of the Extraction of Uranium with Supercritical Carbon Dioxide

A model is presented for the analysis of the results of extraction of uranium in a flow system by supercritical fluid modified with tributylphosphate from a nitric acid matrix, in which the extraction is not limited by the solubility of the uranium species. The model used is that of diffusion out of...

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Veröffentlicht in:Journal of nuclear science and technology 2001-06, Vol.38 (6), p.433-438
Hauptverfasser: CLIFFORD, Anthony A., ZHU, Shuang, SMART, Neil G., LIN, Yuehe, WAI, Chien M., YOSHIDA, Zenko, MEGURO, Yoshihiro, ISO, Shuichi
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container_end_page 438
container_issue 6
container_start_page 433
container_title Journal of nuclear science and technology
container_volume 38
creator CLIFFORD, Anthony A.
ZHU, Shuang
SMART, Neil G.
LIN, Yuehe
WAI, Chien M.
YOSHIDA, Zenko
MEGURO, Yoshihiro
ISO, Shuichi
description A model is presented for the analysis of the results of extraction of uranium in a flow system by supercritical fluid modified with tributylphosphate from a nitric acid matrix, in which the extraction is not limited by the solubility of the uranium species. The model used is that of diffusion out of a sphere into a medium in which the extracted uranium is infinitely dilute. Although not a completely accurate representation of the liquid-supercritical fluid system, the model is shown to be a reasonable representation and some conclusions discussed.
doi_str_mv 10.1080/18811248.2001.9715050
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source Elektronische Zeitschriftenbibliothek - Frei zugängliche E-Journals; Alma/SFX Local Collection; Free Full-Text Journals in Chemistry
subjects Applied sciences
carbon dioxide
clean technology
Energy
Exact sciences and technology
extraction
Fuels
Nuclear fuels
Preparation and processing of nuclear fuels
processing
supercritical fluid
TBP
uranium
waste minimisation
title Modelling of the Extraction of Uranium with Supercritical Carbon Dioxide
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