Source Apportionment of Dry Deposited and Airborne Coarse Particles Collected in the Chicago Area

Long-term dry deposition and dichotomous coarse particle samples were collected between November 1993 and October 1995 in Chicago, IL, as part of the Lake Michigan Mass Balance Study (LMMBS). In addition, short-term dry deposition and airborne coarse particle (Noll Rotary Impactor) samples were coll...

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Veröffentlicht in:Aerosol science and technology 1999-12, Vol.31 (6), p.473-486
Hauptverfasser: Paode, Rajendra D., Shahin, Usama M., Sivadechathep, Jakkris, Holsen, Thomas M., Franek, William J.
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container_end_page 486
container_issue 6
container_start_page 473
container_title Aerosol science and technology
container_volume 31
creator Paode, Rajendra D.
Shahin, Usama M.
Sivadechathep, Jakkris
Holsen, Thomas M.
Franek, William J.
description Long-term dry deposition and dichotomous coarse particle samples were collected between November 1993 and October 1995 in Chicago, IL, as part of the Lake Michigan Mass Balance Study (LMMBS). In addition, short-term dry deposition and airborne coarse particle (Noll Rotary Impactor) samples were collected during the Atmospheric Exchange Over Lakes and Oceans Study (AEOLOS). These samples were analyzed for trace metals and modeled using the U.S. EPA's Chemical Mass Balance (CMB) Model (Version 7) to determine the sources of these particles. The modeled source contributions were similar. The results indicate that light duty unleaded vehicles, soil dust, and heavy duty diesel vehicles were the major sources of ambient coarse and dry deposited particles in Chicago. The other sources found were lime kilns, coke dust, aluminum foundryreverberatory furnace, coal-fired power plant, paint spray booth, and municipal incineration. The results from this study indicate that the CMB approach can be used to determine the source of deposited particles.
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source IngentaConnect Free/Open Access Journals; EZB-FREE-00999 freely available EZB journals; Free Full-Text Journals in Chemistry
subjects Applied sciences
Atmospheric pollution
Earth, ocean, space
Exact sciences and technology
External geophysics
Meteorology
Particles and aerosols
Pollutants physicochemistry study: properties, effects, reactions, transport and distribution
Pollution
title Source Apportionment of Dry Deposited and Airborne Coarse Particles Collected in the Chicago Area
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