Investigation of the clock transition and its pressure-dependent behavior of the trigonal 171Yb3+ centers in lithium niobate crystal
The application of rare earth (RE) doped crystals in quantum information processing has attracted more and more attention in the past decade. How to change the clock transitions of RE ion in crystal and control their lifetime of maintaining coherent quantum state is a valuable question. In this work...
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description | The application of rare earth (RE) doped crystals in quantum information processing has attracted more and more attention in the past decade. How to change the clock transitions of RE ion in crystal and control their lifetime of maintaining coherent quantum state is a valuable question. In this work, the trigonal 171Yb3+ centers in lithium niobate (LN) crystal are investigated theoretically to obtain their accurate ground and excited hyperfine sublevels under external magnetic field B by a combined method of density functional theory-based geometric optimization and parametric effective Hamiltonian modeling. An optical clock transition at |B| = 45.73 mT along the c axis of the LN crystal is successfully found by calculation. To show the pressure-dependent behavior of optical clock transition, the variation of such transition under hydrostatic pressure up to 3 GPa is also obtained theoretically. The calculated results show that applying external pressure is an effective way to control these transitions of RE ion doped crystal. Moreover, the optical coherence time T2 at zero magnetic field for 171Yb3+ ion with C3 symmetry in the LN crystal is estimated by our calculations. The calculated results indicate that if the magnetic field noise is 33 μT in the LN crystal, it is possible to find an optical clock transition with long coherence time T2 (≈382 μs) at the zero magnetic field. The present methods of seeking optical clock transition and calculating its coherence time T2 caused by a fluctuating magnetic field noise in the host crystal can be applied to other Kramers RE ions doped materials. |
doi_str_mv | 10.1063/5.0144292 |
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How to change the clock transitions of RE ion in crystal and control their lifetime of maintaining coherent quantum state is a valuable question. In this work, the trigonal 171Yb3+ centers in lithium niobate (LN) crystal are investigated theoretically to obtain their accurate ground and excited hyperfine sublevels under external magnetic field B by a combined method of density functional theory-based geometric optimization and parametric effective Hamiltonian modeling. An optical clock transition at |B| = 45.73 mT along the c axis of the LN crystal is successfully found by calculation. To show the pressure-dependent behavior of optical clock transition, the variation of such transition under hydrostatic pressure up to 3 GPa is also obtained theoretically. The calculated results show that applying external pressure is an effective way to control these transitions of RE ion doped crystal. Moreover, the optical coherence time T2 at zero magnetic field for 171Yb3+ ion with C3 symmetry in the LN crystal is estimated by our calculations. The calculated results indicate that if the magnetic field noise is 33 μT in the LN crystal, it is possible to find an optical clock transition with long coherence time T2 (≈382 μs) at the zero magnetic field. The present methods of seeking optical clock transition and calculating its coherence time T2 caused by a fluctuating magnetic field noise in the host crystal can be applied to other Kramers RE ions doped materials.</description><identifier>ISSN: 0021-8979</identifier><identifier>EISSN: 1089-7550</identifier><identifier>DOI: 10.1063/5.0144292</identifier><identifier>CODEN: JAPIAU</identifier><language>eng</language><publisher>Melville: American Institute of Physics</publisher><subject>Applied physics ; Data processing ; Density functional theory ; Doped crystals ; Electrons ; External pressure ; Hamiltonian functions ; Hydrostatic pressure ; Lithium niobates ; Magnetic fields ; Optimization ; Pressure dependence ; Quantum phenomena</subject><ispartof>Journal of applied physics, 2023-05, Vol.133 (20)</ispartof><rights>Author(s)</rights><rights>2023 Author(s). Published under an exclusive license by AIP Publishing.</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><cites>FETCH-LOGICAL-c252t-4d1068cc19bae3072b1ce02a2fce868e652340e5f8a41243905595419295c4d3</cites><orcidid>0000-0002-7183-4972 ; 0000-0002-7417-1625</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktohtml>$$Uhttps://pubs.aip.org/jap/article-lookup/doi/10.1063/5.0144292$$EHTML$$P50$$Gscitation$$H</linktohtml><link.rule.ids>314,776,780,790,4498,27901,27902,76353</link.rule.ids></links><search><creatorcontrib>Huang Gaohai</creatorcontrib><creatorcontrib>Liu, Honggang</creatorcontrib><creatorcontrib>Dong Haoran</creatorcontrib><creatorcontrib>He, Zhiyu</creatorcontrib><title>Investigation of the clock transition and its pressure-dependent behavior of the trigonal 171Yb3+ centers in lithium niobate crystal</title><title>Journal of applied physics</title><description>The application of rare earth (RE) doped crystals in quantum information processing has attracted more and more attention in the past decade. How to change the clock transitions of RE ion in crystal and control their lifetime of maintaining coherent quantum state is a valuable question. In this work, the trigonal 171Yb3+ centers in lithium niobate (LN) crystal are investigated theoretically to obtain their accurate ground and excited hyperfine sublevels under external magnetic field B by a combined method of density functional theory-based geometric optimization and parametric effective Hamiltonian modeling. An optical clock transition at |B| = 45.73 mT along the c axis of the LN crystal is successfully found by calculation. To show the pressure-dependent behavior of optical clock transition, the variation of such transition under hydrostatic pressure up to 3 GPa is also obtained theoretically. The calculated results show that applying external pressure is an effective way to control these transitions of RE ion doped crystal. Moreover, the optical coherence time T2 at zero magnetic field for 171Yb3+ ion with C3 symmetry in the LN crystal is estimated by our calculations. The calculated results indicate that if the magnetic field noise is 33 μT in the LN crystal, it is possible to find an optical clock transition with long coherence time T2 (≈382 μs) at the zero magnetic field. The present methods of seeking optical clock transition and calculating its coherence time T2 caused by a fluctuating magnetic field noise in the host crystal can be applied to other Kramers RE ions doped materials.</description><subject>Applied physics</subject><subject>Data processing</subject><subject>Density functional theory</subject><subject>Doped crystals</subject><subject>Electrons</subject><subject>External pressure</subject><subject>Hamiltonian functions</subject><subject>Hydrostatic pressure</subject><subject>Lithium niobates</subject><subject>Magnetic fields</subject><subject>Optimization</subject><subject>Pressure dependence</subject><subject>Quantum phenomena</subject><issn>0021-8979</issn><issn>1089-7550</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2023</creationdate><recordtype>article</recordtype><recordid>eNp90M9LwzAUB_AgCs7pwf8g4EmlMy9t1uQowx-DgZddPJU0TbfMLqlJOtjdP9y6TT0IngKPz3sv74vQJZARkHF6x0YEsowKeoQGQLhIcsbIMRoQQiHhIhen6CyEFSEAPBUD9DG1Gx2iWchonMWuxnGpsWqcesPRSxvMri5thU0MuPU6hM7rpNKttpW2EZd6KTfG-e_e6M3CWdlgyOG1TG-x6pX2ARuLGxOXpltja1wpY7_Hb0OUzTk6qWUT9MXhHaL548N88pzMXp6mk_tZoiijMcmq_kSuFIhS6pTktASlCZW0VpqPuR4zmmZEs5rLDGiWCsKYYBkIKpjKqnSIrvZjW-_eu_7qYuU63381FJSDAJISAb263ivlXQhe10XrzVr6bQGk-Mq4YMUh497e7G1QJu4S_MEb539h0Vb1f_jv5E9aQori</recordid><startdate>20230528</startdate><enddate>20230528</enddate><creator>Huang Gaohai</creator><creator>Liu, Honggang</creator><creator>Dong Haoran</creator><creator>He, Zhiyu</creator><general>American Institute of Physics</general><scope>AAYXX</scope><scope>CITATION</scope><scope>8FD</scope><scope>H8D</scope><scope>L7M</scope><orcidid>https://orcid.org/0000-0002-7183-4972</orcidid><orcidid>https://orcid.org/0000-0002-7417-1625</orcidid></search><sort><creationdate>20230528</creationdate><title>Investigation of the clock transition and its pressure-dependent behavior of the trigonal 171Yb3+ centers in lithium niobate crystal</title><author>Huang Gaohai ; Liu, Honggang ; Dong Haoran ; He, Zhiyu</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c252t-4d1068cc19bae3072b1ce02a2fce868e652340e5f8a41243905595419295c4d3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2023</creationdate><topic>Applied physics</topic><topic>Data processing</topic><topic>Density functional theory</topic><topic>Doped crystals</topic><topic>Electrons</topic><topic>External pressure</topic><topic>Hamiltonian functions</topic><topic>Hydrostatic pressure</topic><topic>Lithium niobates</topic><topic>Magnetic fields</topic><topic>Optimization</topic><topic>Pressure dependence</topic><topic>Quantum phenomena</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Huang Gaohai</creatorcontrib><creatorcontrib>Liu, Honggang</creatorcontrib><creatorcontrib>Dong Haoran</creatorcontrib><creatorcontrib>He, Zhiyu</creatorcontrib><collection>CrossRef</collection><collection>Technology Research Database</collection><collection>Aerospace Database</collection><collection>Advanced Technologies Database with Aerospace</collection><jtitle>Journal of applied physics</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Huang Gaohai</au><au>Liu, Honggang</au><au>Dong Haoran</au><au>He, Zhiyu</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Investigation of the clock transition and its pressure-dependent behavior of the trigonal 171Yb3+ centers in lithium niobate crystal</atitle><jtitle>Journal of applied physics</jtitle><date>2023-05-28</date><risdate>2023</risdate><volume>133</volume><issue>20</issue><issn>0021-8979</issn><eissn>1089-7550</eissn><coden>JAPIAU</coden><abstract>The application of rare earth (RE) doped crystals in quantum information processing has attracted more and more attention in the past decade. How to change the clock transitions of RE ion in crystal and control their lifetime of maintaining coherent quantum state is a valuable question. In this work, the trigonal 171Yb3+ centers in lithium niobate (LN) crystal are investigated theoretically to obtain their accurate ground and excited hyperfine sublevels under external magnetic field B by a combined method of density functional theory-based geometric optimization and parametric effective Hamiltonian modeling. An optical clock transition at |B| = 45.73 mT along the c axis of the LN crystal is successfully found by calculation. To show the pressure-dependent behavior of optical clock transition, the variation of such transition under hydrostatic pressure up to 3 GPa is also obtained theoretically. The calculated results show that applying external pressure is an effective way to control these transitions of RE ion doped crystal. Moreover, the optical coherence time T2 at zero magnetic field for 171Yb3+ ion with C3 symmetry in the LN crystal is estimated by our calculations. The calculated results indicate that if the magnetic field noise is 33 μT in the LN crystal, it is possible to find an optical clock transition with long coherence time T2 (≈382 μs) at the zero magnetic field. The present methods of seeking optical clock transition and calculating its coherence time T2 caused by a fluctuating magnetic field noise in the host crystal can be applied to other Kramers RE ions doped materials.</abstract><cop>Melville</cop><pub>American Institute of Physics</pub><doi>10.1063/5.0144292</doi><tpages>11</tpages><orcidid>https://orcid.org/0000-0002-7183-4972</orcidid><orcidid>https://orcid.org/0000-0002-7417-1625</orcidid><oa>free_for_read</oa></addata></record> |
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subjects | Applied physics Data processing Density functional theory Doped crystals Electrons External pressure Hamiltonian functions Hydrostatic pressure Lithium niobates Magnetic fields Optimization Pressure dependence Quantum phenomena |
title | Investigation of the clock transition and its pressure-dependent behavior of the trigonal 171Yb3+ centers in lithium niobate crystal |
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