Reverse bias breakdown and photocurrent gain in CH3NH3PbBr3 films
Perovskite films are promising candidates for fast, sensitive, and large area photodetectors. A gain in perovskite based detectors has been observed in several architectures, but a model describing the underlying mechanism is still missing or at least incomplete. Here, we present measurements of CH3...
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Veröffentlicht in: | Applied physics letters 2022-03, Vol.120 (11) |
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creator | Auf der Maur, M. Matteocci, F. Di Carlo, A. Testa, M. |
description | Perovskite films are promising candidates for fast, sensitive, and large area photodetectors. A gain in perovskite based detectors has been observed in several architectures, but a model describing the underlying mechanism is still missing or at least incomplete. Here, we present measurements of CH3NH3PbBr3 films under reverse bias exhibiting breakdown at 4–5 V and small photocurrent gain
≲ 2, which based on a phenomenological model, we explain tentatively by tunnel-assisted injection from the TiO2 electron transport layer and carrier multiplication, mediated by the electric field due to mobile ions. |
doi_str_mv | 10.1063/5.0082425 |
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≲ 2, which based on a phenomenological model, we explain tentatively by tunnel-assisted injection from the TiO2 electron transport layer and carrier multiplication, mediated by the electric field due to mobile ions.</description><subject>Applied physics</subject><subject>Bias</subject><subject>Breakdown</subject><subject>Electric fields</subject><subject>Electron transport</subject><subject>Multiplication</subject><subject>Perovskites</subject><subject>Photoelectric effect</subject><subject>Photoelectric emission</subject><subject>Titanium dioxide</subject><issn>0003-6951</issn><issn>1077-3118</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2022</creationdate><recordtype>article</recordtype><recordid>eNp90FFLwzAQB_AgCs7pg98g4JNC5yXXNMnjHNMKQ0X0OaRtop1bM5NO8dtb2Z6Fg-Pgx93xJ-ScwYRBgddiAqB4zsUBGTGQMkPG1CEZAQBmhRbsmJyktBxGwRFHZPrsvlxMjlatTbSKzn404bujtmvo5j30od7G6Lqevtm2o0PNSnwo8am6iUh9u1qnU3Lk7Sq5s30fk9fb-cuszBaPd_ez6SKruZB91gjX5Mo1WvNaKC_By4rbvODaK6gs146jtF5UTGoENrxaaFQatYcapNc4Jhe7vZsYPrcu9WYZtrEbThpeoFZcF5wN6nKn6hhSis6bTWzXNv4YBuYvISPMPqHBXu1sqtve9m3o_sG_pN5iqQ</recordid><startdate>20220314</startdate><enddate>20220314</enddate><creator>Auf der Maur, M.</creator><creator>Matteocci, F.</creator><creator>Di Carlo, A.</creator><creator>Testa, M.</creator><general>American Institute of Physics</general><scope>AAYXX</scope><scope>CITATION</scope><scope>8FD</scope><scope>H8D</scope><scope>L7M</scope><orcidid>https://orcid.org/0000-0001-7893-1356</orcidid><orcidid>https://orcid.org/0000-0002-4815-4485</orcidid><orcidid>https://orcid.org/0000-0001-6828-2380</orcidid><orcidid>https://orcid.org/0000-0003-1274-8967</orcidid></search><sort><creationdate>20220314</creationdate><title>Reverse bias breakdown and photocurrent gain in CH3NH3PbBr3 films</title><author>Auf der Maur, M. ; Matteocci, F. ; Di Carlo, A. ; Testa, M.</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c257t-d5ed48ed992c58f70f7b2a4629f80ba29e237af5b1793016956938939f0c07f93</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2022</creationdate><topic>Applied physics</topic><topic>Bias</topic><topic>Breakdown</topic><topic>Electric fields</topic><topic>Electron transport</topic><topic>Multiplication</topic><topic>Perovskites</topic><topic>Photoelectric effect</topic><topic>Photoelectric emission</topic><topic>Titanium dioxide</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Auf der Maur, M.</creatorcontrib><creatorcontrib>Matteocci, F.</creatorcontrib><creatorcontrib>Di Carlo, A.</creatorcontrib><creatorcontrib>Testa, M.</creatorcontrib><collection>CrossRef</collection><collection>Technology Research Database</collection><collection>Aerospace Database</collection><collection>Advanced Technologies Database with Aerospace</collection><jtitle>Applied physics letters</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Auf der Maur, M.</au><au>Matteocci, F.</au><au>Di Carlo, A.</au><au>Testa, M.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Reverse bias breakdown and photocurrent gain in CH3NH3PbBr3 films</atitle><jtitle>Applied physics letters</jtitle><date>2022-03-14</date><risdate>2022</risdate><volume>120</volume><issue>11</issue><issn>0003-6951</issn><eissn>1077-3118</eissn><coden>APPLAB</coden><abstract>Perovskite films are promising candidates for fast, sensitive, and large area photodetectors. A gain in perovskite based detectors has been observed in several architectures, but a model describing the underlying mechanism is still missing or at least incomplete. Here, we present measurements of CH3NH3PbBr3 films under reverse bias exhibiting breakdown at 4–5 V and small photocurrent gain
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subjects | Applied physics Bias Breakdown Electric fields Electron transport Multiplication Perovskites Photoelectric effect Photoelectric emission Titanium dioxide |
title | Reverse bias breakdown and photocurrent gain in CH3NH3PbBr3 films |
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